Organic cations in hybrid organic-inorganic perovskite solar cells are susceptible to decomposition under high temperatures and ultraviolet light, leading their power conversion efficiency (PCE) to decrease. All-inorganic perovskite solar cells exhibit both high PCE and superior photothermal stability, making them promising candidates for single-junction and tandem photovoltaic applications. The mixed-halide perovskite CsPbI
2Br has received much attention as a top cell in semi-transparent and tandem solar cells due to its excellent thermal stability and suitable bandgap (1.90 eV). Although the PCE of CsPbI
2Br-based solar cells is approaching its theoretical limit, the energy loss caused by non-radiative recombination remains a major barrier to further improving performance. This non-radiative recombination is mainly caused by inadequate band alignment between the absorption layer and the transport layer, resulting in the loss of open-circuit voltage (
VOC) and decrease of short-circuit current density (
JSC). Two-dimensional perovskite passivation formed through solution processing can mitigate interfacial recombination, but it can also impede efficient charge transport. Constructing three-dimensional perovskite structures not only provides an effective solution to these limitations but also enhances sunlight absorption and facilitates carrier transport. In this study, we propose a dual-absorption-layer perovskite heterojunction (DPHJ) strategy, which involves integrating a staggered type-II perovskite heterojunction (p-pCsPbI
2Br-CsPbIBr
2) into the absorption layer of the top cell in an all-perovskite tandem solar cell. The simulation result indicates that stacking a 100-nm-thick CsPbIBr
2 layer atop a 300-nm-thick CsPbI
2Br layer greatly enhances the PCE of the single-junction device from 19.46% to 22.29%. This improvement is mainly attributed to band bending at the CsPbI
2Br/CsPbIBr
2 interface, which enhances the built-in electric field, facilitates carrier transport, and suppresses non-radiative recombination within the absorption layer. Compared with the tandem solar cell utilizing a single-absorption-layer CsPbI
2Br top cell, the DPHJ-based tandem solar cell significantly increases
VOC from 2.16 to 2.25 V and
JSC from 15.96 to 16.76 mA⋅cm
–2. As a result, the DPHJ-based tandem solar cell achieves a high theoretical PCE of 32.47%. In addition, the DPHJ-based tandem solar cell exhibits a significantly enhanced external quantum efficiency in a wavelength range of 500–580 nm, which can be attributed to the band-edge absorption of CsPbIBr
2. This enhanced absorption generates more photogenerated carriers, thereby significantly improving the
JSC. The
VOC and PCE values in this study exceed those experimentally reported values of current CsPbI
2Br single-junction and all-perovskite tandem solar cells. Compared with the single-layer CsPbI
2Br (
E2 = 101.9 meV, electron-phonon coupling strength \gamma _\textac = 1.2 \times 10^ - 2,\text \gamma _\textLO = 6.9 \times 10^3 ), the double-absorption-layer film exhibits a high exciton binding energy (
E2 = 110.7 meV) and reduced electron-phonon coupling strength ( \gamma _\textac = 1.1 \times 10^ - 2,\text \gamma _\textLO = 6.3 \times 10^3 ), which helps suppress phase segregation and enhance both optical and thermal stability, which is favorable for fabricating long-term stable all-perovskite tandem solar cells. This work provides new ideas and theoretical guidance for improving the efficiency and stability of all-perovskite tandem solar cells. In addition, it also proposes a universal design concept for optimizing absorption layers in all-perovskite multijunction cells, which is expected to further advance the research in this field.