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中国物理学会期刊

α相三氧化钼中各向异性双曲声子极化激元的耦合性质

CSTR: 32037.14.aps.72.20222144

Coupling interactions of anisotropic hyperbolic phonon polaritons in double layered orthorhombic molybdenum trioxide

CSTR: 32037.14.aps.72.20222144
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  • 天然双曲声子极化激元材料-α相三氧化钼(α-MoO3)能够支持高度局域的表面声子极化激元(surface phonon polaritons, SPhPs), 达到在中红外波段对光与物质相互作用的过程进行揭示以及调节的目的. 我们理论上提出并研究了基于Kretschmann结构的单层和多层α-MoO3的面内各向异性表面声子极化激元(ASPhPs). 通过4×4传递矩阵法(TMM)快速准确地求解多层各向异性介质系统中的反射系数, 描述多层系统中激发的SPhPs及色散性质. 结果证实层间耦合可以通过多层膜的堆叠以及层厚来调制. 当入射角度大于全内反射角时, 满足SPhP激发的相位匹配条件. 在40°角范围内, SPhP谐振随着入射角度的增加迅速蓝移, 但是随后色散曲线不再随着入射角的增大而移动. 间隙层的增大会还会致使法布里-珀罗(FP)共振模式的激发. 层状异质结构中的ASPhPs是当今纳米光子技术的重要组成部分, 我们的研究有助于进一步优化和设计基于极化双曲材料的可控光电器件.

     

    The natural hyperbolic phonon polariton material-orthorhombic molybdenum trioxide (α-MoO3) has recently attracted much interest , due to the associated ultra-confinement of light and enhanced light-matter interactions. We theoretically propose and study the in-plane anisotropic phonon polaritons (APhPs) in the Kretschmann structure with monolayer and dual layers α-MoO3. The excitation of phonon polaritons and the corresponding dispersion properties in this multilayer system are studied by using a generalized 4×4 transfer matrix method (TMM). The frequency dispersions with geometrical parameters are also discussed in detail. The results confirm that the interlayer coupling can be modulated by stacking the multilayer films and regulating the thickness of each layer. More interestingly, when the distance between double α-MoO3 layers is much smaller than the propagation length of PhPs, a strong coupling phenomenon occurs, and the photon tunneling probability and intensity can be greatly improved. When the incident angle is greater than the total internal reflection angle, the phase matching condition for SPhP excitation can be satisfied. Within the 40° incident angle, the SPhP blue-shifts rapidly with the increase of incident angle. But then the dispersion curve no longer changes with increase of incidence angle. The enlargement of the interstitial layer can also lead the Fabry-Perot (FP) resonance mode to be excited. The APhP in layered heterostructure is an important part of today's nanophotonic technology, our study can help optimize and design tunable optoelectronic devices based on hyperbolic materials.

     

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