Research progress of low-dimensional semiconductor materials in field of nonlinear optics

Bai Rui-Xue; Yang Jue-Han; Wei Da-Hai; Wei Zhong-Ming

doi:10.7498/aps.69.20200206

Abstract

Since the first ruby laser was invented, researchers have focused their attention on how to achieve a strong laser light source, which cannot be produced by the ordinary light sources. Since then, the rich and colorful characteristics of nonlinear optical materials have been discovered, such as the saturation absorption, reverse saturation absorption and nonlinear refraction. They are applied to optoelectronic devices, optical switching devices and optical communication. At the same time, with the increase of the requirements for device integration performance in industrial production, ordinary three-dimensional devices are difficult to meet the production requirements, and the advent of low-dimensional semiconductor devices effectively solves this problem. Therefore, the combination of nonlinear optics and low-dimensional semiconductor materials is a general trend. The emergence of quantum dots, quantum wire lasers, and amplifiers confirms this. In this paper, we summarize the frontier work on nonlinear optics by selecting several special low-dimensional structures and several materials, providing some references for future research. However, due to the fact that the instability and low filling ratio of low-dimensional materials remain to be improved, further relevant research is still required.

Keywords:

Authors and contacts

1.
State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083, China
2.
College of Materials Science and Opto-Electronic Technology, University of Chinese Academy of Sciences, Beijing 100049, China

Corresponding author: Wei Zhong-Ming, zmwei@semi.ac.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 61622406)

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Cited By

图 1 (a)双层石墨烯调制器结构示意图^[44]; (b)单分子光开关示意图^[45]; (c)双层石墨烯双光子吸收和双层石墨烯4个可能的过渡^[46]; (d)用于石墨烯包裹的光纤(GCM)透射率测量的实验装置^[47]

Figure 1. (a) Schematic of the structure for the double layer graphene modulator (reproduced with permission^[44], Copyright 2012 American Chemical Society); (b) single-molecule optical switch (reproduced with permission^[45], Copyright 2005 American Physical Society); (c) two-photon absorption in bilayer graphene and four possible transitions in bilayer graphene (reproduced with permission^[46], Copyright 2011 American Chemical Society); (d) experimental setup for transmittance measurements of GCMs (reproduced with permission^[47], Copyright 2014 American Chemical Society).

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图 2 (a)相干非线性光学响应测量装置图^[53]; (b)可饱和的透射SWCNT的透射光谱^[55]; (c) 基于单壁碳纳米管饱和吸收体的超快激光器装置图^[56]; (d) Z扫描系统装置图^[54]

Figure 2. (a) Schematic of coherent nonlinear optical response measurement setup (reproduced with permission^[53], Copyright 2010 The American Physical Society); (b) transmission spectra of transmissive SWCNT saturable absorbers (reproduced with permission^[55], Copyright © 2010 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim; (c) experimental setup of the ultrafast-laser based on SWNT SAs (reproduced with permission^[56], Copyright 2016 Springer Nature); (d) schematic diagram of the Z-scan setup (reproduced with permission^[54], Copyright 2019, Springer Nature).

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图 3 基于石墨烯-Bi₂Te₃异质结的饱和吸收体^[103]　(a)光纤连接器端面上的石墨烯-Bi₂Te₃异质结构示意图; (b)双探测器测量实验装置的示意图; (c)石墨烯-Bi₂Te₃异质结构中光学跃迁的示意图; (d)石墨烯-Bi₂Te₃异质结构的拉曼光谱

Figure 3. Saturable absorber based on graphene-Bi₂Te₃ heterojunction (reproduced with permission^[103], Copyright 2015, American Chemical Society): (a) Schematic of graphene-Bi₂Te₃ heterostructure on the end-facet of fiber connector; (b) schematic diagram of the twin-detector measurement experimental setup; (c) schematic diagram showing the optical transitions in graphene-Bi₂Te₃ heterostructure; (d) Raman spectrum of the graphene-Bi₂Te₃ heterostructure.

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图 4 (a) MoS₂中的THG^[113]; (b) 2D (TMD)光发射器^[114]; (c)少层MoS₂不同的非线性光学现象^[35]; (d) SHG和THG的极坐标图^[115]

Figure 4. (a) Third harmonic generation in MoS₂ (reproduced with permission^[113], Copyright 2014 American Chemical Society); (b) 2D (TMD) optical emitter (reproduced with permission^[114], Copyright 2018 American Physical Society); (c) different nonlinear optical phenomenon of few-layer MoS₂ (reproduced with permission^[35], Copyright 2016, American Chemical Society); (d) polar plots of normalized SHG and THG (reproduced with permission^[115], Copyright 2018 American Physical Society).

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图 5 (a)铋的线性色散价和导带中载流子的开关和信号^[124]; (b)开关和信号的叠加原理^[124]; (c) BP调Q光纤激光器输出偏振特性^[127]; (d) 磷烯的透射率与飞秒激光强度之间的关系^[104]

Figure 5. (a) Switch and signal of carriers in the linearly dispersive valence and conduction bands of bismuthine (reproduced with permission^[124], Copyright 2017, American Chemical Society); (b) superposition principle of switch and signal light (reproduced with permission^[124], Copyright 2017, American Chemical Society); (c) output polarization characteristics of BP Q-switched fiber laser (reproduced with permission^[127], Copyright 2015, Springer Nature); (d) relationship between transmittance of the phosphorene dispersions and intensity of the femtosecond laser (reproduced with permission^[104], Copyright 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim).

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图 6 (a)沉积有黑磷量子点的微纤维照片^[138]; (b)黑磷量子点饱和吸收体SA特征^[138]; (c)线性、非线性和总折射率变化随光子能量的变化(对于0s—1p跃迁)^[139]; (d)微腔中的非对称量子点作为非线性光学元件^[140]

Figure 6. (a) Photograph of the microfiber deposited with PQDs, (b) saturable absorption property of the PQD-SA device (reproduced with permission^[138], Copyright 2017 Springer Nature); (c) the linear, nonlinear and total refractive index changes with photon energy for 0s–1p transitions (reproduced with permission^[139], Copyright 2011 American Institute of Physics); (d) asymmetric quantum dot in a microcavity as a nonlinear optical element (reproduced with permission^[140], ©2012 American Physical Society).

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