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The ionization time-delay in atoms and molecules detected through strong-field multiphoton transition interferometry

Wei Menghao Li Xing Luo Sizuo He Lanhai Dajun Ding

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The ionization time-delay in atoms and molecules detected through strong-field multiphoton transition interferometry

Wei Menghao, Li Xing, Luo Sizuo, He Lanhai, Dajun Ding
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  • Attosecond ionization dynamics, as a key research direction in ultrafast science, relies critically on breakthroughs in both experimental techniques and theoretical models to reveal the fundamental processes underlying ultrafast matter evolution. Among the cutting-edge approaches in this field, the strong-field multiphoton transition interferometry (SFMPTI) method stands out for its ability to achieve attosecond time-resolved probing of multiphoton ionization dynamics via quantum path interference. This technique has been widely applied to attosecond-scale measurements and characterizations of ionization time delays with quantum state resolution, ranging from atomic systems to complex molecules, offering a novel time-resolved perspective for strong-field physics.This article focuses on the application of the SFMPTI method in probing strong-field multiphoton ionization time delays in atoms and molecules. We systematically present the quantum interference mechanisms underlying the method, summarize recent progress in attosecond-resolved studies of above-threshold ionization dynamics and resonance-state-mediated delays, and discuss the prospective applications and challenges that lie ahead for this emerging technique.
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