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The experimental technique and results from measuring spin-lattice relaxation times by the pulse saturation method at X band are described. Double frequency is used to synchronize the oscilloscope in order to measure T1 more precisely. The spin lattice relaxation times of Cr3+ in ruby have been measured for several different concentrations. It is concluded that T1 of various transitions are nearly the same, but become shorter apparently with increasing Cr3+ concentration.
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