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First-order and second-order infrared quantum cutting of Ho3+ Yb3+ doped oxyfluoride vitroceramics

Chen Xiao-Bo Yang Guo-Jian Li Song Sawanobori N. Xu Yi-Zhuang Chen Xiao-Duan Zhou Gu

First-order and second-order infrared quantum cutting of Ho3+ Yb3+ doped oxyfluoride vitroceramics

Chen Xiao-Bo, Yang Guo-Jian, Li Song, Sawanobori N., Xu Yi-Zhuang, Chen Xiao-Duan, Zhou Gu
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  • Infrared quantum cutting is an international hot research field nowadays. Comparitive research between first-order and second-order quantum cutting of Ho3+ Yb3+ doped oxyfluoride vitroceramics is reported in present paper. It is found that most population can easily non-radiativly relax to (5F45S2) energy level when the energy levels between 5G5 and 5S2 are excited. For (5F45S2) level, the population of Ho3+ ion can be cross-transferred to 5I6 level by strong ETr7-ETaYb {5F4(Ho) 5I6 (Ho), 2F7/2(Yb) 2F5/2(Yb)} cross energy transfer passage; meanwhile, Yb3+ ion is excited to 2F5/2 level from 2F7/2 ground state. It results in the two infrared photons which can be absorbed by crystal Si, that is, one is (1153 nm, 1188 nm) infrared photon and the other is (973.0 nm, 1002.0 nm) infrared photon. Therefore, it results in two-photon first-order infrared quantum cutting. Finally, the cross energy transfer efficiency tr, 1%Yb(5F45S2)=29.2%, tr, 10.5%Yb(5F45S2)=99.2%. and cooperative energy transfer efficiency tr, 1%Yb(5F3)=4.18%, tr, 10.5%Yb(5F3)=75.3% of Ho(0.5)Yb(1):FOV and Ho(0.5)Yb(10.5):FOV are calculated. Their quantum efficiency up-limits of two-photon quantum cutting are CR, 1%Yb(5F45S2)=129.2%, CR, 10.5% Yb(5F45S2)=199.2 and CO, 1%Yb(5F3)=104.18%, CO, 10.5% Yb(5F3)=175.3% respectively. That is to say, the probability of first-order infrared quantum cutting is larger than that of second-order infrared quantum cutting. The present research is of significance for enhancing solar cell efficiency.
    • Funds: Project supported by the National Natural Science Foundation of China (Grant No. 10674019 ), and by the Fundamental Research Funds for the Central Universities of China (212-105560GK).
    [1]

    Yang G Z 1995 Optical Physics (Beijing: Science Press) (in Chinese) [杨国桢, 1995 光物理科学 (北京: 科学出版社)]

    [2]

    Wegh R T, Donker H, Oskam K D, Meijerink A 1999 Science 283 663

    [3]

    Eliseeva S V, Bunzli J C G 2010 Chem. Soc. Rev. 39 189

    [4]

    Rodrguez V D, Tikhomirov V K, Mendez-Ramos J, Yanes A C, Moshchalkov V V 2010 Solar Energy Materials & Solar Cells 94 1612

    [5]

    Vergeer P, Vlugt T J H, Kox M H F, den Hertog M I, van der Eerden J P J M, Meijerink A 2005 Phys. Rev. B 71 014119

    [6]

    Lin H, Chen D Q, Yu Y L, Yang A P, and Wang Y S 2010 Opt. Lett. 36 876

    [7]

    Deng K M, Gong T, Hu L X, Wei X T, Chen Y H, Yin M 2011 Opt. Express 19 1749

    [8]

    Chen X B, Wu J G, Xu X L, Zhang Y Z, Sawanobori N, Zhang C L, Pan Q H, Salamo G J 2009 Opt. Lett. 34 887

    [9]

    Zhou J J, Teng Y, Liu X F, Ye S, Ma Z J, Qiu J R 2010 Phys. Chem. Chem. Phys. 12 13759

    [10]

    van der Ende B M, Aarts L, Meijerink A 2009 Phys. Chem. Chem. Phys. 11 11081

    [11]

    Chen J D, Guo H, Li Z Q, Zhang H, Zhuang Y X 2010 Opt. Materials 32 998

    [12]

    Zhou J J, Teng Y, Liu X F, Ye S, Xu X Q, Ma Z J, Qiu J R 2010 Opt. Express 18 21663

    [13]

    Richards B S 2006 Solar Energy Materials & Solar Cells 90 1189

    [14]

    Yu D C, Huang X Y, Ye S, Zhang Q Y 2011 J. Alloys and Compounds 509 9919

    [15]

    Reisfeld R 1977 Lasers and excited states of rare-earth (New York: Springer-Verlag, Berlin Heidelberg, )

    [16]

    Wei X T, Zhao J B, Chen Y H, Yin M, and Li Y 2010 Chin. Phys. B 19 077804

    [17]

    Chen X Y, Luo Z D 1998 Chin. Phys. 7 773

    [18]

    Song Z F, Lian S R, Wang S K 1982 Acta Phys. Sin. 31 772 (in Chinese) [宋增福, 连绍仁, 王淑坤 1982 物理学报 31 772]

    [19]

    Trupke T, Green M, Wurfel P 2002 J. Appl. Phys. 92 1668

    [20]

    Trupke T, Green M, Wurfel P 2002 J. Appl. Phys. 92 4117

    [21]

    Xu X R, Shu M Z 2003 Science of Luminescence and Luminescent Material (Beijing: The Publish Center of Material Science and Engineering)(in Chinese) [徐叙瑢, 苏勉曾 2003 发光学与发光材料 (北京: 材料科学与工程出版中心)]

    [22]

    Zhang X G, Yang B J 2002 Acta Phys. Sin. 51 2745 [张晓光, 杨伯君 2002 物理学报 51 2745]

    [23]

    Hao H Y, Kong G L, Zeng X B, Diao H W, Liao X B 2005 Acta Phys. Sin. 54 3327 [郝会颖, 孔光临, 曾湘波, 刁宏伟, 廖显伯 2005 物理学报 54 3327]

    [24]

    Zhao H, Wang Y S, Hou Y B, Xu Z, Xu X R 2000 Acta Phys. Sin. 49 954 [赵 辉, 王永生, 侯延冰, 徐 征, 徐叙瑢 2000 物理学报 49 954]

    [25]

    Zhao Z X 1979 Acta Phys. Sin. 28 222 [赵忠贤 1979 物理学报 28 222]

  • [1]

    Yang G Z 1995 Optical Physics (Beijing: Science Press) (in Chinese) [杨国桢, 1995 光物理科学 (北京: 科学出版社)]

    [2]

    Wegh R T, Donker H, Oskam K D, Meijerink A 1999 Science 283 663

    [3]

    Eliseeva S V, Bunzli J C G 2010 Chem. Soc. Rev. 39 189

    [4]

    Rodrguez V D, Tikhomirov V K, Mendez-Ramos J, Yanes A C, Moshchalkov V V 2010 Solar Energy Materials & Solar Cells 94 1612

    [5]

    Vergeer P, Vlugt T J H, Kox M H F, den Hertog M I, van der Eerden J P J M, Meijerink A 2005 Phys. Rev. B 71 014119

    [6]

    Lin H, Chen D Q, Yu Y L, Yang A P, and Wang Y S 2010 Opt. Lett. 36 876

    [7]

    Deng K M, Gong T, Hu L X, Wei X T, Chen Y H, Yin M 2011 Opt. Express 19 1749

    [8]

    Chen X B, Wu J G, Xu X L, Zhang Y Z, Sawanobori N, Zhang C L, Pan Q H, Salamo G J 2009 Opt. Lett. 34 887

    [9]

    Zhou J J, Teng Y, Liu X F, Ye S, Ma Z J, Qiu J R 2010 Phys. Chem. Chem. Phys. 12 13759

    [10]

    van der Ende B M, Aarts L, Meijerink A 2009 Phys. Chem. Chem. Phys. 11 11081

    [11]

    Chen J D, Guo H, Li Z Q, Zhang H, Zhuang Y X 2010 Opt. Materials 32 998

    [12]

    Zhou J J, Teng Y, Liu X F, Ye S, Xu X Q, Ma Z J, Qiu J R 2010 Opt. Express 18 21663

    [13]

    Richards B S 2006 Solar Energy Materials & Solar Cells 90 1189

    [14]

    Yu D C, Huang X Y, Ye S, Zhang Q Y 2011 J. Alloys and Compounds 509 9919

    [15]

    Reisfeld R 1977 Lasers and excited states of rare-earth (New York: Springer-Verlag, Berlin Heidelberg, )

    [16]

    Wei X T, Zhao J B, Chen Y H, Yin M, and Li Y 2010 Chin. Phys. B 19 077804

    [17]

    Chen X Y, Luo Z D 1998 Chin. Phys. 7 773

    [18]

    Song Z F, Lian S R, Wang S K 1982 Acta Phys. Sin. 31 772 (in Chinese) [宋增福, 连绍仁, 王淑坤 1982 物理学报 31 772]

    [19]

    Trupke T, Green M, Wurfel P 2002 J. Appl. Phys. 92 1668

    [20]

    Trupke T, Green M, Wurfel P 2002 J. Appl. Phys. 92 4117

    [21]

    Xu X R, Shu M Z 2003 Science of Luminescence and Luminescent Material (Beijing: The Publish Center of Material Science and Engineering)(in Chinese) [徐叙瑢, 苏勉曾 2003 发光学与发光材料 (北京: 材料科学与工程出版中心)]

    [22]

    Zhang X G, Yang B J 2002 Acta Phys. Sin. 51 2745 [张晓光, 杨伯君 2002 物理学报 51 2745]

    [23]

    Hao H Y, Kong G L, Zeng X B, Diao H W, Liao X B 2005 Acta Phys. Sin. 54 3327 [郝会颖, 孔光临, 曾湘波, 刁宏伟, 廖显伯 2005 物理学报 54 3327]

    [24]

    Zhao H, Wang Y S, Hou Y B, Xu Z, Xu X R 2000 Acta Phys. Sin. 49 954 [赵 辉, 王永生, 侯延冰, 徐 征, 徐叙瑢 2000 物理学报 49 954]

    [25]

    Zhao Z X 1979 Acta Phys. Sin. 28 222 [赵忠贤 1979 物理学报 28 222]

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  • Received Date:  17 March 2012
  • Accepted Date:  30 May 2012
  • Published Online:  05 November 2012

First-order and second-order infrared quantum cutting of Ho3+ Yb3+ doped oxyfluoride vitroceramics

  • 1. Applied Optics Beijing Area Major Laboratory and Analysis and Testing Center, Beijing Normal University, Beijing, 100875, China;
  • 2. Sumita Optical Glass, Inc., 4-7-25 Harigaya, Urawa, Saitama, 338, Japan;
  • 3. The Chemistry and the Molecular Engineer College, Peking University, Beijing 100871, China
Fund Project:  Project supported by the National Natural Science Foundation of China (Grant No. 10674019 ), and by the Fundamental Research Funds for the Central Universities of China (212-105560GK).

Abstract: Infrared quantum cutting is an international hot research field nowadays. Comparitive research between first-order and second-order quantum cutting of Ho3+ Yb3+ doped oxyfluoride vitroceramics is reported in present paper. It is found that most population can easily non-radiativly relax to (5F45S2) energy level when the energy levels between 5G5 and 5S2 are excited. For (5F45S2) level, the population of Ho3+ ion can be cross-transferred to 5I6 level by strong ETr7-ETaYb {5F4(Ho) 5I6 (Ho), 2F7/2(Yb) 2F5/2(Yb)} cross energy transfer passage; meanwhile, Yb3+ ion is excited to 2F5/2 level from 2F7/2 ground state. It results in the two infrared photons which can be absorbed by crystal Si, that is, one is (1153 nm, 1188 nm) infrared photon and the other is (973.0 nm, 1002.0 nm) infrared photon. Therefore, it results in two-photon first-order infrared quantum cutting. Finally, the cross energy transfer efficiency tr, 1%Yb(5F45S2)=29.2%, tr, 10.5%Yb(5F45S2)=99.2%. and cooperative energy transfer efficiency tr, 1%Yb(5F3)=4.18%, tr, 10.5%Yb(5F3)=75.3% of Ho(0.5)Yb(1):FOV and Ho(0.5)Yb(10.5):FOV are calculated. Their quantum efficiency up-limits of two-photon quantum cutting are CR, 1%Yb(5F45S2)=129.2%, CR, 10.5% Yb(5F45S2)=199.2 and CO, 1%Yb(5F3)=104.18%, CO, 10.5% Yb(5F3)=175.3% respectively. That is to say, the probability of first-order infrared quantum cutting is larger than that of second-order infrared quantum cutting. The present research is of significance for enhancing solar cell efficiency.

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