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High-sensitive off-axis integrated cavity output spectroscopy and its measurement of ambient CO2 at 2 μm

Li Zhi-Bin Ma Hong-Liang Cao Zhen-Song Sun Ming-Guo Huang Yin-Bo Zhu Wen-Yue Liu Qiang

High-sensitive off-axis integrated cavity output spectroscopy and its measurement of ambient CO2 at 2 μm

Li Zhi-Bin, Ma Hong-Liang, Cao Zhen-Song, Sun Ming-Guo, Huang Yin-Bo, Zhu Wen-Yue, Liu Qiang
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  • Received Date:  11 July 2015
  • Accepted Date:  15 December 2015
  • Published Online:  05 March 2016

High-sensitive off-axis integrated cavity output spectroscopy and its measurement of ambient CO2 at 2 μm

    Corresponding author: Cao Zhen-Song, zscao@aiofm.ac.cn
  • 1. Key Laboratory of Atmospheric Composition and Optical Radiation, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 220031, China;
  • 2. University of Chinese Academy of Sciences, Beijing 100049, China
Fund Project:  Project supported by the National Natural Science Foundation of China (Grant No. 41205021)

Abstract: An off-axis integrated cavity output spectroscopy (OA-ICOS) is established by using a fiber-coupled distributed feedback diode laser operating near 2 μm. Its performances are evaluated and optimized through experimental investigation via detecting the pure CH4 absorptions at different pressures. The reflectivity of the cavity mirror is measured to be 0.99865, which results in the effective total optical pathlength of up to 407.4 m based on a 55 cm cavity. It is shown that the OA-ICOS configuration can be used to obtain very long optical pathlength, leading to pretty high sensitive monitoring of atmospheric trace gases. Based on the developed OA-ICOS, the atmospheric CO2 measurements are made and its performance is improved by using the wavelet denoising approach. The CO2 absorption line at 4993.7431 cm-1 is used for measuring the concentration. The measured results are compared with the results obtaind by a commercial H2O/CO2 analyzer. Agreement and disagreement are briefly discussed, and the results show that the OA-ICOS is reliable for detecting the atmospheric trace gases. The limitation of the developed OA-ICOS and the further steps towards the improvement in precision and accuracy are also presented.

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