Abstract Ni-FeCr multilayer films were prepared by diode sputtering technique. These multilayer films exhibit magnetic uniaxial anisotropy that is shown by fitting the anglar dependence of ferromagnetic uniform resonance field. The anisotropy energy could be expressed by EK=K1sin2θ+K2sin4θ, where K2/K1≈0.59. However the behavior of surface mode suggests that che surface and interface anisotropy of these multilayer films is not of the uniaxis type. We consider that is caused by the exchange coupling at the surface and interface.