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Determination of the atmospheric aerosol optical density by multi axis differential optical absorption spectroscopy

Si Fu-Qi Xie Pin-Hua Dou Ke Zhan Kai Liu Yu Xu Jin Liu Wen-Qing

Determination of the atmospheric aerosol optical density by multi axis differential optical absorption spectroscopy

Si Fu-Qi, Xie Pin-Hua, Dou Ke, Zhan Kai, Liu Yu, Xu Jin, Liu Wen-Qing
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  • In this work, a method to determine atmospheric aerosol optical density from multi axis differential optical absorption spectroscopy (MAX-DOAS) observations was described. It basically utilizes the differential absorption structures of the oxygen collision complex (O4) in the UV and visible wavelength regions to derive information on aerosol optical properties. Based on radiative transfer model with appropriate aerosol single scattering albedo, asymmetry parameter and profile, atmospheric aerosol optical density was retrieved in an iterative process by comparison with measured O4 slant column densities at 360 nm. The retrieved value was verified through comparisons with sun photometer CE318.
    • Funds:
    [1]

    [1]Platt U, Perner D 1979 J. Geophys. Res. 84 6329

    [2]

    [2]Platt U, Perner D 1980 J. Geophys. Res. 85 7453

    [3]

    [3]Zhou B, Liu W Q, Qi F, Li Z B, Cui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周斌、刘文清、齐峰、李振壁、崔延军 2001物理学报 50 1818]

    [4]

    [4]Si F Q, Liu J G, Xie P H, Zhang Y J, Dou K, Liu W Q 2006 Acta Phys. Sin. 55 3165 (in Chinese) [司福祺、刘建国、谢品华、张玉钧、窦科、刘文清 2006物理学报 55 3165]

    [5]

    [5]Wagner T, Burrows J P, Deutschmann T, Dix B, von Friedeburg C, Frie U, Hendrick F, Heue K P, Irie H, Iwabuchi H, Kanaya Y, Keller J, McLinden C A, Oetjen H, Palazzi E, Petritoli A, Platt U, Postylyakov O, Pukite J, Richter A, Roozendael M, Rozanov A, Rozanov V, Sinreich R, Sanghavi S, Wittrock F 2007 Atmos. Chem. Phys. 7 1809

    [6]

    [6]Fu Q, Liu W Q, Si F Q, Zhang Y H, Xie P H 2009 Acta Photonica Sin. 38 1216 (in Chinese) [付强、刘文清、司福祺、张英华、谢品华 2009光子学报 38 1216]

    [7]

    [7]Wagner T, von Friedeburg C, Wenig M, Otten C, Platt U 2002 J. Geophys. Res. 107 4424

    [8]

    [8]Wagner T, Dix B, von Friedeburg C, Frie U, Sanghavi S, Sinreich R, Platt U 2004 J. Geophys. Res. 109 D22205

    [9]

    [9]Frieb U, Monks P S, Remedios J J, Rozanov, Sinreich R, Wagner T, Platt U 2006 J. Geophys. Res. 111 D14203

    [10]

    ]Honninger G, von Friedeburg C V, Platt U 2004 Atmos. Chem. Phys. 4 231

    [11]

    ]Heckel A, Richter A, Tarsu T, Wittrock F, Hak C, Pundt I, Junkermann W, Burrows J P 2005 Atmos. Chem. Phys. 5 909

    [12]

    ]Irie H, Kanaya Y, Akimoto H, Iwabuchi H, Shimizu A, Aoki K 2008 Atmos. Chem. Phys. 8 341

    [13]

    ]Kondratyev K Y, Grigoryev A A, Pokrovsky O M 1982 Adv. Space Res. 2 3

    [14]

    ]von Friedeburg C 2003 Ph. D. Dissertation (Heidelberg: Heidelberg University)

    [15]

    ]Kwon H L, Li Z Q, Man S W, Xin J Y, Wang Y S, Hao W M, Zhao F S 2007 J. Geophys. Res.112 D22S15

    [16]

    ]Garland R M, Schmid O, Nowak A, Achtert P, Wiedensohler A, Gunthe S S, Takegawa N, Kita K, Kondo Y, Hu M, Shao M, Zeng L M, Zhu T, Andreae M O, Poeschl U 2009 J. Geophys. Res.114 D00G04

  • [1]

    [1]Platt U, Perner D 1979 J. Geophys. Res. 84 6329

    [2]

    [2]Platt U, Perner D 1980 J. Geophys. Res. 85 7453

    [3]

    [3]Zhou B, Liu W Q, Qi F, Li Z B, Cui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周斌、刘文清、齐峰、李振壁、崔延军 2001物理学报 50 1818]

    [4]

    [4]Si F Q, Liu J G, Xie P H, Zhang Y J, Dou K, Liu W Q 2006 Acta Phys. Sin. 55 3165 (in Chinese) [司福祺、刘建国、谢品华、张玉钧、窦科、刘文清 2006物理学报 55 3165]

    [5]

    [5]Wagner T, Burrows J P, Deutschmann T, Dix B, von Friedeburg C, Frie U, Hendrick F, Heue K P, Irie H, Iwabuchi H, Kanaya Y, Keller J, McLinden C A, Oetjen H, Palazzi E, Petritoli A, Platt U, Postylyakov O, Pukite J, Richter A, Roozendael M, Rozanov A, Rozanov V, Sinreich R, Sanghavi S, Wittrock F 2007 Atmos. Chem. Phys. 7 1809

    [6]

    [6]Fu Q, Liu W Q, Si F Q, Zhang Y H, Xie P H 2009 Acta Photonica Sin. 38 1216 (in Chinese) [付强、刘文清、司福祺、张英华、谢品华 2009光子学报 38 1216]

    [7]

    [7]Wagner T, von Friedeburg C, Wenig M, Otten C, Platt U 2002 J. Geophys. Res. 107 4424

    [8]

    [8]Wagner T, Dix B, von Friedeburg C, Frie U, Sanghavi S, Sinreich R, Platt U 2004 J. Geophys. Res. 109 D22205

    [9]

    [9]Frieb U, Monks P S, Remedios J J, Rozanov, Sinreich R, Wagner T, Platt U 2006 J. Geophys. Res. 111 D14203

    [10]

    ]Honninger G, von Friedeburg C V, Platt U 2004 Atmos. Chem. Phys. 4 231

    [11]

    ]Heckel A, Richter A, Tarsu T, Wittrock F, Hak C, Pundt I, Junkermann W, Burrows J P 2005 Atmos. Chem. Phys. 5 909

    [12]

    ]Irie H, Kanaya Y, Akimoto H, Iwabuchi H, Shimizu A, Aoki K 2008 Atmos. Chem. Phys. 8 341

    [13]

    ]Kondratyev K Y, Grigoryev A A, Pokrovsky O M 1982 Adv. Space Res. 2 3

    [14]

    ]von Friedeburg C 2003 Ph. D. Dissertation (Heidelberg: Heidelberg University)

    [15]

    ]Kwon H L, Li Z Q, Man S W, Xin J Y, Wang Y S, Hao W M, Zhao F S 2007 J. Geophys. Res.112 D22S15

    [16]

    ]Garland R M, Schmid O, Nowak A, Achtert P, Wiedensohler A, Gunthe S S, Takegawa N, Kita K, Kondo Y, Hu M, Shao M, Zeng L M, Zhu T, Andreae M O, Poeschl U 2009 J. Geophys. Res.114 D00G04

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  • Received Date:  13 July 2009
  • Accepted Date:  30 July 2009
  • Published Online:  15 April 2010

Determination of the atmospheric aerosol optical density by multi axis differential optical absorption spectroscopy

  • 1. 中国科学院安徽光学精密机械研究所,中国科学院环境光学与技术重点实验室,合肥 230031

Abstract: In this work, a method to determine atmospheric aerosol optical density from multi axis differential optical absorption spectroscopy (MAX-DOAS) observations was described. It basically utilizes the differential absorption structures of the oxygen collision complex (O4) in the UV and visible wavelength regions to derive information on aerosol optical properties. Based on radiative transfer model with appropriate aerosol single scattering albedo, asymmetry parameter and profile, atmospheric aerosol optical density was retrieved in an iterative process by comparison with measured O4 slant column densities at 360 nm. The retrieved value was verified through comparisons with sun photometer CE318.

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