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金属氧化物基杂化型聚合物太阳电池研究

刘长文 周讯 岳文瑾 王命泰 邱泽亮 孟维利 陈俊伟 齐娟娟 董超

金属氧化物基杂化型聚合物太阳电池研究

刘长文, 周讯, 岳文瑾, 王命泰, 邱泽亮, 孟维利, 陈俊伟, 齐娟娟, 董超
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  • 以有机共轭聚合物为电子给体和无机纳米结构为电子受体组成的杂化型聚合物太阳电池(HPSC), 是一类新型的光伏器件. HPSC将有机物和无机物的光学、电学和力学等性能集成在一起, 其最显著的优点体现在材料来源丰富、性能互补且可调控、易实现低成本组装及轻便等方面. 金属氧化物纳米结构具有环境友好、可见光区透明且易合成等特点, 是很有发展前景的电子受体材料. 本文首先简要介绍了HPSC电池的研究现状、工作原理、器件结构、和稳态及动态表征方法, 然后重点综述了在基于ZnO和TiO2纳米结构的HPSC方面的研究进展, 包括载流子传输动力学理论模型、高效电池材料与器件的设计和制备、及纳米结构特性相关的器件性能等. 最后, 对我们的研究成果进行了总结, 并展望了电池的后续研究方向和发展前景.
    • 基金项目: 国家自然科学基金(批准号: 11274307, 11474286)、国家自然科学基金重大研究计划(批准号: 91333121)、国家自然科学基金青年科学基金(批准号: 51202002)和安徽省自然科学基金(批准号: 1308085ME70)资助的课题.
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    Service R F 2011 Science 332 293

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    Huynh W U, Dittmer J J, Alivisatos A P 2002 Science 295 2425

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    Mor G K, Kim S, Paulose M, Varghese O K, Shankar K, Basham J, Grimes C A 2009 Nano Lett. 9 4250

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    Dayal S, Kopidakis N, Olson D C, Ginley D S, Rumbles G 2009 Nano Lett. 10 239

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    Cui Q, Liu C, Wu F, Yue W, Qiu Z, Zhang H, Gao F, Shen W, Wang M 2013 J. Phys. Chem. C 117 5626

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  • [1]

    Green M A, Emery K, Hishikawa Y, Warta W, Dunlop E D 2013 Prog. Photovolt. Res. Appl. 21 827

    [2]

    Lewis N S 2007 Science 315 798

    [3]

    Coakley K M, McGehee M D 2004 Chem. Mater. 16 4533

    [4]

    Gnes S, Neugebauer H, Sariciftci N S 2007 Chem. Rev. 107 1324

    [5]

    Thompson B C, Fréchet J M J 2008 Angew. Chem.-Int. Edit. 47 58

    [6]

    Huang Y, Kramer E J, Heeger A J, Bazan G C 2014 Chem. Rev. 114 7006

    [7]

    Heeger A J 2014 Adv. Mater. 26 10

    [8]

    Dou L, You J, Hong Z, Xu Z, Li G, Street R A, Yang Y 2013 Adv. Mater. 25 6642

    [9]

    Krebs F C, Fyenbo J, Tanenbaum D M, Gevorgyan S A, Andriessen R, van Remoortere B, Galagan Y, Jorgensen M 2011 Energy Environ. Sci. 4 4116

    [10]

    Service R F 2011 Science 332 293

    [11]

    Huynh W U, Dittmer J J, Alivisatos A P 2002 Science 295 2425

    [12]

    Mor G K, Kim S, Paulose M, Varghese O K, Shankar K, Basham J, Grimes C A 2009 Nano Lett. 9 4250

    [13]

    Dayal S, Kopidakis N, Olson D C, Ginley D S, Rumbles G 2009 Nano Lett. 10 239

    [14]

    Chang J A, Rhee J H, Im S H, Lee Y H, Kim H J, Seok S I, Nazeeruddin M K, Grätzel M 2010 Nano Lett. 10 2609

    [15]

    Im S H, Lim C-S, Chang J A, Lee Y H, Maiti N, Kim H-J, Nazeeruddin M K, Grätzel M, Seok S I 2011 Nano Lett. 11 4789

    [16]

    Chang J A, Im S H, Lee Y H, Kim H J, Lim C S, Heo J H, Seok S I 2012 Nano Lett. 12 1863

    [17]

    Liu C, Qiu Z, Li F, Meng W, Yue W, Zhang F, Qiao Q, Wang, M 2014 Nano Energy DOI: 10.1016/j.nanoen.2014.09.028

    [18]

    Zhou Y, Eck M, Krger M 2010 Energy Environ. Sci. 3 1851

    [19]

    Reiss P, Couderc E, De Girolamo J, Pron A 2011 Nanoscale 3 446

    [20]

    Xu T, Qiao Q 2011 Energy Environ. Sci. 4 2700

    [21]

    Moule A J, Chang L, Thambidurai C, Vidu R, Stroeve P 2012 J. Mater. Chem. 22 2351

    [22]

    Wright M, Uddin A 2012 Sol Energy Mater. Sol. Cells 107 87

    [23]

    Fan X, Zhang M, Wang X, Yang F, Meng X 2013 J. Mater. Chem. A 1 8694

    [24]

    He M, Qiu F, Lin Z 2013 J. Phys. Chem. Lett. 4 1788

    [25]

    Gao F, Ren S, Wang J 2013 Energy Environ. Sci. 6 2020

    [26]

    Li S S, Chen C W 2013 J. Mater. Chem. A 1 10574

    [27]

    Patel J, Mighri F, Ajji A, Chaudhuri T K 2014 Nano Energy 5 36

    [28]

    Freitas J N, Goncalves A S, Nogueira A F 2014 Nanoscale 6 6371

    [29]

    Miranda P B, Moses D, Heeger A J 2001 Phys. Rev. B 64 081201

    [30]

    Gregg B A, Hanna M C 2003 J. Appl. Phys. 93 3605

    [31]

    Gregg B A 2003 J. Phys. Chem. B 107 4688

    [32]

    Dloczik L, Ileperuma O, Lauermann I, Peter L M, Ponomarev E A, Redmond G, Shaw N J, Uhlendorf I 1997 J. Phys. Chem. B 101 10281

    [33]

    Chen C, Peng R, Wu H, Wang M 2009 J. Phys. Chem. C 113 12608

    [34]

    de Jongh P E, Vanmaekelbergh D 1996 Phys. Rev. Lett. 77 3427

    [35]

    Haque S A, Tachibana Y, Klug D R, Durrant J R 1998 J. Phys. Chem. B 102 1745

    [36]

    Bisquert J, Zaban A, Salvador P 2002 J. Phys. Chem. B 106 8774

    [37]

    Kannan B, Castelino K, Majumdar A 2003 Nano Lett. 3 1729

    [38]

    Kirchartz T, Mattheis J, Rau U 2008 Phys. Rev. B 78 235320

    [39]

    Bi D, Wu F, Yue W, Guo Y, Shen W, Peng R, Wu H, Wang X, Wang M 2010 J. Phys. Chem. C 114 13846

    [40]

    Potscavage W J Jr, Sharma A, Kippelen B 2009 Acc. Chem. Res. 42 1758

    [41]

    Qi B, Wang J 2013 Phys. Chem. Chem. Phys. 15 8972

    [42]

    Schilinsky P, Waldauf C, Hauch J, Brabec C J 2004 J. Appl. Phys. 95 2816

    [43]

    Wu F, Yue W, Cui Q, Liu C, Qiu Z, Shen W, Zhang H, Wang M 2012 Sol. Energy 86 1459

    [44]

    Bi D, Wu F, Qu Q, Yue W, Cui Q, Shen W, Chen R, Liu C, Qiu Z, Wang M 2011 J. Phys. Chem. C 115 3745

    [45]

    Cui Q, Liu C, Wu F, Yue W, Qiu Z, Zhang H, Gao F, Shen W, Wang M 2013 J. Phys. Chem. C 117 5626

    [46]

    Wu F, Cui Q, Qiu Z, Liu C, Zhang H, Shen W, Wang M 2013 ACS Appl. Mater. Interfaces 5 3246

    [47]

    Rauh D, Wagenpfahl A, Deibel C, Dyakonov V 2011 Appl. Phys. Lett. 98 133301

    [48]

    Potscavage W J Jr, Yoo S, Kippelen B 2008 Appl. Phys. Lett. 93 193308

    [49]

    Vandewal K, Tvingstedt K, Gadisa A, Inganäs O, Manca J V 2010 Phys. Rev. B 81 125204

    [50]

    Ruankham P, Macaraig L, Sagawa T, Nakazumi H, Yoshikawa S 2011 J. Phys. Chem. C 115 23809

    [51]

    Gupta D, Bag M, Narayan K S 2008 Appl. Phys. Lett. 93 163301

    [52]

    Jeong W I, Lee J, Park S Y, Kang J W, Kim J J 2011 Adv. Funct. Mater. 21 343

    [53]

    Liao K S, Yambem S D, Haldar A, Alley N J, Curran S A 2010 Energies 3 1212

    [54]

    Burschka J, Dualeh A, Kessler F, Baranoff E, Cevey-Ha N L, Yi C Y, Nazeeruddin M K, Grätzel M 2011 J. Am. Chem. Soc. 133 18042

    [55]

    Choi S, Potscavage W J, Kippelen B 2009 J. Appl. Phys. 106 054507

    [56]

    Dunn H K, Peter L M 2009 J. Phys. Chem. C 113 4726

    [57]

    Chen C, Wang M, Wang K 2009 J. Phys. Chem. C 113 1624

    [58]

    Geng H, Wang M, Han S, Peng R 2010 Sol. Energy Mater. Sol. Cells 94 547

    [59]

    Geng H, Guo Y, Peng R, Han S, Wang M 2010 Sol. Energy Mater. Sol. Cells 94 1293

    [60]

    Wu F, Shen W, Cui Q, Bi D, Yue W, Qu Q, Wang M 2010 J. Phys. Chem. C 114 20225

    [61]

    Peng R, Chen C, Shen W, Wang M, Guo Y, Geng H 2009 Acta Phys. Sin. 58 6582 (in Chinese) [彭瑞祥, 陈冲, 沈薇, 王命泰, 郭颖, 耿宏伟 2009 物理学报 58 6582]

    [62]

    Krger J, Plass R, Grätzel M, Cameron P J, Peter L M 2003 J. Phys. Chem. B 107 7536

    [63]

    Chen C, Wu F, Geng1 H, Shen W, Wang M 2011 Nanoscale Res. Lett. 6 350

    [64]

    Takanezawa K, Hirota K, Wei Q S, Tajima K, Hashimoto K 2007 J. Phys. Chem. C 111 7218

    [65]

    Lin Y Y, Chu T H, Li S S, Chuang C H, Chang C H, Su W F, Chang C P, Chu M W, Chen C W 2009 J. Am. Chem. Soc. 131 3644

    [66]

    Xi J, Wiranwetchayan O, Zhang Q, Liang Z, Sun Y, Cao G 2012 J. Mater Sci: Mater. Electron. 23 1657

    [67]

    Yue W, Han S, Peng R, Shen W, Geng H, Wu F, Tao S, Wang M 2010 J. Mater. Chem. 20 7570

    [68]

    Yue W, Wu F, Liu C, Qiu Z, Cui Q, Zhang H, Gao F, Shen W, Qiao Q, Wang M 2013 Sol. Energy Mater. Sol. Cells 114 43

    [69]

    Ravirajan P, Peiró A M, Nazeeruddin M K, Graetzel M, Bradley D D C, Durrant J R, Nelson J 2006 J. Phys. Chem. B 110 7635

    [70]

    Lin Y Y, Lee Y Y, Chang L, Wu J J, Chen C W 2009 Appl. Phys. Lett. 94 063308

    [71]

    Liu Y, Scully S R, McGehee M D, Liu J, Luscombe C K, Fréchet J M J, Shaheen S E, Ginley D S 2006 J. Phys. Chem. B 110 3257

    [72]

    Qu Q, Geng H, Peng R, Cui Q, Gu X, Li F, Wang M 2010 Langmuir 26 9539

    [73]

    Greene L E, Law M, Yuhas B D, Yang P 2007 J. Phys. Chem. C 111 18451

    [74]

    Lee Y J, Davis R J, Lloyd M T, Provencio P P, Prasankumar R P, Hsu J W P 2010 IEEE J. Sel. Top. Quantum Electron. 16 1587

    [75]

    Wang L, Zhao D, Su Z, Li B, Zhang Z, Shen D 2011 J. Electrochem. Soc. 158 H804

    [76]

    Krger J, Bach U, Grätzel M 2000 Adv. Mater. 12 447

    [77]

    Goh C, Scully S R, McGehee M D 2007 J. Appl. Phys. 101 114503

    [78]

    Chen Z L, Zhang H, Du X H, Cheng X, Chen X G, Jiang Y Y, Yang B 2013 Energy Environ. Sci. 6 1597

    [79]

    Heeger H J, Sariciftci N S, Namdas E B (translated by Shuai Z G, Cao Y et al.) 2010 Semiconducting and Metallic Polymers (Beijing: Science Press) p17-28 (in Chinese) [Heeger H J, Sariciftci N S, Namdas E B (帅志刚, 曹镛等译)2010 半导性和金属性聚合物 (北京: 科学出版社)第17–28页]

    [80]

    Mihailetchi V D, Koster L J A, Hummelen J C, Blom P W M 2004 Phys. Rev. Lett. 93 216601

    [81]

    Yin C, Pieper B, Stiller B, Kietzke T, Neher D 2007 Appl. Phys. Lett. 90 133502

    [82]

    Marsh R A, McNeill C R, Abrusci A, Campbell A R, Friend R H 2008 Nano Lett. 8 1393

    [83]

    Olson C, Shaheen S E, White M S, Mitchell W J, van Hest M F A M, Collins R T, Ginley D S 2007 Adv. Funct. Mater. 17 264

    [84]

    Schlichthörl G, Huang S Y, Sprague J, Frank A J 1997 J. Phys. Chem. B 101 8141

    [85]

    Adebanjo O, Maharjan P P, Adhikary P, Wang M, Yang S, Qiao Q 2013 Energy Environ. Sci. 6 3150

    [86]

    Ameri T, Li N, Brabec C J 2013 Energy Environ. Sci. 6 2390

    [87]

    Chen C C, Chang W H, Yoshimura K, Ohya K, You J, Gao J, Hong Z, Yang Y 2014 Adv. Mater. 26 5670

    [88]

    Winder C, Sariciftci N S 2004 J. Mater. Chem. 14 1077

    [89]

    Bundgaard E, Krebs F C 2007 Sol. Energy Mater. Sol. Cells 91 954

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    Li Y 2012 Acc. Chem. Res. 45 723

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  • 收稿日期:  2014-10-22
  • 修回日期:  2014-11-27
  • 刊出日期:  2015-02-05

金属氧化物基杂化型聚合物太阳电池研究

  • 1. 中国科学院等离子体物理研究所, 合肥 230031;
  • 2. 安徽工程大学生物与化学工程学院, 芜湖 241000
    基金项目: 

    国家自然科学基金(批准号: 11274307, 11474286)、国家自然科学基金重大研究计划(批准号: 91333121)、国家自然科学基金青年科学基金(批准号: 51202002)和安徽省自然科学基金(批准号: 1308085ME70)资助的课题.

摘要: 以有机共轭聚合物为电子给体和无机纳米结构为电子受体组成的杂化型聚合物太阳电池(HPSC), 是一类新型的光伏器件. HPSC将有机物和无机物的光学、电学和力学等性能集成在一起, 其最显著的优点体现在材料来源丰富、性能互补且可调控、易实现低成本组装及轻便等方面. 金属氧化物纳米结构具有环境友好、可见光区透明且易合成等特点, 是很有发展前景的电子受体材料. 本文首先简要介绍了HPSC电池的研究现状、工作原理、器件结构、和稳态及动态表征方法, 然后重点综述了在基于ZnO和TiO2纳米结构的HPSC方面的研究进展, 包括载流子传输动力学理论模型、高效电池材料与器件的设计和制备、及纳米结构特性相关的器件性能等. 最后, 对我们的研究成果进行了总结, 并展望了电池的后续研究方向和发展前景.

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