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新型偶氮苯衍生物的三阶非线性光学特性

李梦梦 朱宝华 冉霞 刘波 郭立俊

新型偶氮苯衍生物的三阶非线性光学特性

李梦梦, 朱宝华, 冉霞, 刘波, 郭立俊
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  • 本文以30 ps的脉冲激光为激发光源, 用Z扫描技术研究了偶氮苯类材料4-羟基-4'-羧基偶氮苯(BN)和N-(3, 4, 5-辛氧基苯基)-N'-4-[(4-羟基苯)偶氮苯]1, 3, 4-恶二唑(AOB-t8) 及金属复合物(Au/AOB-t8)的三阶非线性光学性质, 并从理论上进行了分析和计算. 结果表明, AOB-t8的三阶非线性极化率是BN的1.38倍, 其非线性光学效应的增大是由共轭链增长、大 键增多引起的. 结果同时给出, AOB-t8的三阶非线性极化率是其与金纳米颗粒复合物的4.7倍, 这种与金属复合产生的非线性光学效应的减弱是金属引入的局域场效应与有机分子大键作用之间相互抵消导致的.
    [1]

    Bhagavannarayana G, Riscob B, Shakir M 2011 Mater. Chem. Phys. 126 20

    [2]

    Harutyunyan H, Volpe G, Quidant R, Novotny L 2012 Phys. Rev. Lett. 108 217403

    [3]

    Zhu B H, Wang F F, Zhang K, Ma G H, Guo L J, Qian S X 2007 Acta Phys.Sin. 56 4024 (in Chinese) [朱宝华, 王芳芳, 张琨, 马国宏, 郭立俊, 钱世雄 2007 物理学报 56 4024]

    [4]

    Tabiryan N, Hrozhyk U, Serak S 2004 Phys. Rev. Lett. 93 113901

    [5]

    Jaunet-Lahary T, Chantzis A, Chen K J, Laurent A D, Jacquemin D 2014 J. Phys. Chem. C 118 28831

    [6]

    Zhao F, Wang C, Zeng Y, Jin Z, Ma G 2013 Chem. Phys. Lett. 558 100

    [7]

    Virkki M, Tuominen O, Forni A, Saccone M, Metrangolo P, Resnati G, Priimagi A 2015 J. Mater. Chem. C 3 3003

    [8]

    Brzozowski L, Sargent E H 2001 J. Mater. Sci. Mater. Elect. 12 483

    [9]

    Bandara H M D, Burdette S C 2012 Chem. Soc. Rev. 41 1809

    [10]

    Papagiannouli I, Iliopoulos K, Gindre D, Sahraoui B, Krupka O, Smokal V, Couris S 2012 Chem. Phys. Lett. 554 107

    [11]

    El Ouazzani H, Iliopoulos K, Pranaitis M, Krupka O, Smokal V, Kolendo A, Sahraoui B 2011 J. Phys. Chem. B 115 1944

    [12]

    Li N J, Lu J M, Li H, Kang E T 2011 Dyes Pigments 88 18

    [13]

    Yan Z Q, Guang S Y, Xu H Y, Liu X Y 2013 Dyes Pigments 99 720

    [14]

    Zeng Y, Pan Z H, Zhao F L, Qin M, Zhou Y, Wang C S 2014 Chin. Phys. B 23 024212

    [15]

    Papagiannouli I, Iliopoulos K, Gindre D, Sahraoui B, Krupka O, Smokal V, Kolendo A, Couris S 2012 Chem. Phys. Lett. 554 107

    [16]

    Kerasidou A P, Khammar F, Iliopoulos K, Ayadi A, El-Ghayoury A, Zouari N, Mhiri T, Sahraoui B 2014 Chem. Phys. Lett. 597 106

    [17]

    Liaros N, Couris S, Maggini L, De Leo F, Cattaruzza F, Aurisicchio C, Bonifazi D 2013 Chem. Phys. Chem. 14 2961

    [18]

    El Ouazzani H, Iliopoulos K, Pranaitis M, Krupka O, Smokal V, Kolendo A, Sahraoui B 2011 J. Phys. Chem. B 115 1944

    [19]

    Qian Y, Xiao G M, Wang G, Lin B P, Cui Y, Sun Y M 2007 Dyes Pigments 75 218

    [20]

    Wu S J, Qian W, Xia Z J, Zou Y H, Wang S Q, Shen S Y, Xu H J 2000 Chem. Phys. Lett. 330 535

    [21]

    Zhu B H, Wang F F, Zhang K, Ma G H, Gu Y Z, Guo L J, Qian S X 2008 Acta Phys. Sin. 57 3085 (in Chinese) [朱宝华, 王芳芳, 张琨, 马国宏, 顾玉宗, 郭立俊, 钱世雄 2008 物理学报 57 3085]

    [22]

    Ran X, Wang H, Lou J, Shi L L, Liu B, Li M, Guo L J 2014 Soft Mater. 12 396

    [23]

    Ji X H, Song X, Li J, Bai Y, Yang W, Peng X 2007 J. Am. Chem. Soc. 129 13939

    [24]

    Sheik-Bahae M, SAID A A, WEI T, Hagan D J, Vanstryland E W 1990 IEEE J. Quant. Elect. 26 760

    [25]

    Agrawal G P, Cojan C, Flytzanis C 1978 Phys. Rev. B 17 776

    [26]

    Sipe J E, Boyd R W 1992 Phys. Rev. A 46 1614

  • [1]

    Bhagavannarayana G, Riscob B, Shakir M 2011 Mater. Chem. Phys. 126 20

    [2]

    Harutyunyan H, Volpe G, Quidant R, Novotny L 2012 Phys. Rev. Lett. 108 217403

    [3]

    Zhu B H, Wang F F, Zhang K, Ma G H, Guo L J, Qian S X 2007 Acta Phys.Sin. 56 4024 (in Chinese) [朱宝华, 王芳芳, 张琨, 马国宏, 郭立俊, 钱世雄 2007 物理学报 56 4024]

    [4]

    Tabiryan N, Hrozhyk U, Serak S 2004 Phys. Rev. Lett. 93 113901

    [5]

    Jaunet-Lahary T, Chantzis A, Chen K J, Laurent A D, Jacquemin D 2014 J. Phys. Chem. C 118 28831

    [6]

    Zhao F, Wang C, Zeng Y, Jin Z, Ma G 2013 Chem. Phys. Lett. 558 100

    [7]

    Virkki M, Tuominen O, Forni A, Saccone M, Metrangolo P, Resnati G, Priimagi A 2015 J. Mater. Chem. C 3 3003

    [8]

    Brzozowski L, Sargent E H 2001 J. Mater. Sci. Mater. Elect. 12 483

    [9]

    Bandara H M D, Burdette S C 2012 Chem. Soc. Rev. 41 1809

    [10]

    Papagiannouli I, Iliopoulos K, Gindre D, Sahraoui B, Krupka O, Smokal V, Couris S 2012 Chem. Phys. Lett. 554 107

    [11]

    El Ouazzani H, Iliopoulos K, Pranaitis M, Krupka O, Smokal V, Kolendo A, Sahraoui B 2011 J. Phys. Chem. B 115 1944

    [12]

    Li N J, Lu J M, Li H, Kang E T 2011 Dyes Pigments 88 18

    [13]

    Yan Z Q, Guang S Y, Xu H Y, Liu X Y 2013 Dyes Pigments 99 720

    [14]

    Zeng Y, Pan Z H, Zhao F L, Qin M, Zhou Y, Wang C S 2014 Chin. Phys. B 23 024212

    [15]

    Papagiannouli I, Iliopoulos K, Gindre D, Sahraoui B, Krupka O, Smokal V, Kolendo A, Couris S 2012 Chem. Phys. Lett. 554 107

    [16]

    Kerasidou A P, Khammar F, Iliopoulos K, Ayadi A, El-Ghayoury A, Zouari N, Mhiri T, Sahraoui B 2014 Chem. Phys. Lett. 597 106

    [17]

    Liaros N, Couris S, Maggini L, De Leo F, Cattaruzza F, Aurisicchio C, Bonifazi D 2013 Chem. Phys. Chem. 14 2961

    [18]

    El Ouazzani H, Iliopoulos K, Pranaitis M, Krupka O, Smokal V, Kolendo A, Sahraoui B 2011 J. Phys. Chem. B 115 1944

    [19]

    Qian Y, Xiao G M, Wang G, Lin B P, Cui Y, Sun Y M 2007 Dyes Pigments 75 218

    [20]

    Wu S J, Qian W, Xia Z J, Zou Y H, Wang S Q, Shen S Y, Xu H J 2000 Chem. Phys. Lett. 330 535

    [21]

    Zhu B H, Wang F F, Zhang K, Ma G H, Gu Y Z, Guo L J, Qian S X 2008 Acta Phys. Sin. 57 3085 (in Chinese) [朱宝华, 王芳芳, 张琨, 马国宏, 顾玉宗, 郭立俊, 钱世雄 2008 物理学报 57 3085]

    [22]

    Ran X, Wang H, Lou J, Shi L L, Liu B, Li M, Guo L J 2014 Soft Mater. 12 396

    [23]

    Ji X H, Song X, Li J, Bai Y, Yang W, Peng X 2007 J. Am. Chem. Soc. 129 13939

    [24]

    Sheik-Bahae M, SAID A A, WEI T, Hagan D J, Vanstryland E W 1990 IEEE J. Quant. Elect. 26 760

    [25]

    Agrawal G P, Cojan C, Flytzanis C 1978 Phys. Rev. B 17 776

    [26]

    Sipe J E, Boyd R W 1992 Phys. Rev. A 46 1614

  • 引用本文:
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出版历程
  • 收稿日期:  2015-07-09
  • 修回日期:  2015-09-18
  • 刊出日期:  2016-01-20

新型偶氮苯衍生物的三阶非线性光学特性

摘要: 本文以30 ps的脉冲激光为激发光源, 用Z扫描技术研究了偶氮苯类材料4-羟基-4'-羧基偶氮苯(BN)和N-(3, 4, 5-辛氧基苯基)-N'-4-[(4-羟基苯)偶氮苯]1, 3, 4-恶二唑(AOB-t8) 及金属复合物(Au/AOB-t8)的三阶非线性光学性质, 并从理论上进行了分析和计算. 结果表明, AOB-t8的三阶非线性极化率是BN的1.38倍, 其非线性光学效应的增大是由共轭链增长、大 键增多引起的. 结果同时给出, AOB-t8的三阶非线性极化率是其与金纳米颗粒复合物的4.7倍, 这种与金属复合产生的非线性光学效应的减弱是金属引入的局域场效应与有机分子大键作用之间相互抵消导致的.

English Abstract

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