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飞秒时间分辨质谱和光电子影像对分子激发态动力学的研究

王艳梅 唐颖 张嵩 龙金友 张冰

飞秒时间分辨质谱和光电子影像对分子激发态动力学的研究

王艳梅, 唐颖, 张嵩, 龙金友, 张冰
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  • 分子量子态的研究,特别是分子激发态演化过程的研究不仅可以了解分子量子态的基本特性和量子态之间的相互作用,而且可以了解化学反应过程和反应通道间的相互作用.飞秒时间分辨质谱和光电子影像是将飞秒抽运-探测分别与飞行时间质谱和光电子影像相结合的超快谱学方法,为实现分子内部量子态探测,研究分子量子态相互作用及超快动力学过程提供了强有力的工具,可以在飞秒时间尺度下研究单分子反应过程中的光物理或光化学机理.本文详细介绍了飞秒时间分辨质谱和光电子影像的技术原理,并结合本课题组的工作,展示了这两种方法在量子态探测及相互作用研究领域,特别是激发态电子退相、波包演化、能量转移、分子光解动力学以及分子激发态结构动力学研究中的广泛应用.最后,对该技术的发展前景以及进一步的研究工作和方向进行了展望.
      通信作者: 张冰, bzhang@wipm.ac.cn
    • 基金项目: 国家自然科学基金(批准号:21573279,11574351,11674355,21303255,91121006,21273274,21773299)和国家重点基础研究发展计划(批准号:2013CB922200)资助的课题.
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    [7]

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    [8]

    Schoenlein R W, Peteanu L A, Mathies R A, Shank C V 1991 Science 254 412

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    [10]

    Berera R, van Grondelle R, Kennis J T M 2009 Photosynth. Res. 101 105

    [11]

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    [14]

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    [15]

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    Suzuki T 2012 Int. Rev. Phys. Chem. 31 265

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    [22]

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出版历程
  • 收稿日期:  2018-07-10
  • 修回日期:  2018-08-23
  • 刊出日期:  2019-11-20

飞秒时间分辨质谱和光电子影像对分子激发态动力学的研究

  • 1. 中国科学院武汉物理与数学研究所, 波谱与原子分子物理国家重点实验室, 武汉 430071;
  • 2. 中国科学院大学, 北京 100049
  • 通信作者: 张冰, bzhang@wipm.ac.cn
    基金项目: 

    国家自然科学基金(批准号:21573279,11574351,11674355,21303255,91121006,21273274,21773299)和国家重点基础研究发展计划(批准号:2013CB922200)资助的课题.

摘要: 分子量子态的研究,特别是分子激发态演化过程的研究不仅可以了解分子量子态的基本特性和量子态之间的相互作用,而且可以了解化学反应过程和反应通道间的相互作用.飞秒时间分辨质谱和光电子影像是将飞秒抽运-探测分别与飞行时间质谱和光电子影像相结合的超快谱学方法,为实现分子内部量子态探测,研究分子量子态相互作用及超快动力学过程提供了强有力的工具,可以在飞秒时间尺度下研究单分子反应过程中的光物理或光化学机理.本文详细介绍了飞秒时间分辨质谱和光电子影像的技术原理,并结合本课题组的工作,展示了这两种方法在量子态探测及相互作用研究领域,特别是激发态电子退相、波包演化、能量转移、分子光解动力学以及分子激发态结构动力学研究中的广泛应用.最后,对该技术的发展前景以及进一步的研究工作和方向进行了展望.

English Abstract

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