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Kinetics of solidification of liquid benzene under high pressure has attracted much attention of scientists, and it is also one of long-standing disputes. In the present work, the gas-gun technique is combined with a recently developed measurement method of light transmittance, and the time dependence of light transmittance of liquid benzene is directly observed during successive multiply shock-compressions. The analysis shows that the transmittance decrease is caused by light scattering effects in a non-uniform optical medium, which is formed by local phase transformation of liquid-solid, and that the scattering feature reflects both the time relaxation and the spacial accumulation of transition process. The argument whether the liquid-solid phase transformation happens under multi-shock compression is clarified, and important experimental evidence is provided for the study of phase transformation Kinetics.
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Keywords:
- benzene /
- multi-shock compression /
- liquid-solid phase transformations /
- light transmittance
[1] Xu Z Y 1988 Principle of phase transition (Beijing: Science Press ) p1—34,412—418 (in Chinese) [徐祖耀 1988 相变原理(北京:科学出版社)第1—34,412—418页]
[2] Tang Z P 2008 Shock-induced Phase Transformation (Beijing: Science Press) p88—105 (in Chinese) [唐志平 2008 冲击相变(北京:科学出版社)第88—105页]
[3] Zhang S L, Liu F S, Peng X J, Zhang M J, Li Y H, Ma X J, Xue X D 2010 Acta Phys. Sin. 59 (in Chinese)[张世来、刘福生、彭小娟、张明建、李永宏、马小娟、薛学东 2010 物理学报 59]
[4] Klein R M, Nourbakhsh M, Adler P M 1968 J.Mater.Sci. 3 657
[5] Dick R 1970 J. Chem. Phys. 52 6021
[6] Adams D M, Appleby 1977 Proc. R. Soc. London Ser. A 296 1896
[7] Matsuda A, Kondo K, Nakamura K G 2004 Jpn. J. Appl. Phys. Part 243 L1614
[8] Wang C, Zhang P 2010 J.Appl.Phys.107 083502
[9] Maillet J B, Pineau 2008 J. Chem. Phys. 128 224502
[10] Schmidt S C, Moore D S, Schiferl D, Shaner J W 1983 Phys. Rev. Lett. 50 661
[11] Thiery M M, Leger J M 1988 J. Chem. Phys. 89 4255
[12] Walsh J M, Rice M H 1957 J. Chem. Phys. 26 815
[13] Matsuda A, Kondo K, Nakamura K G 2006 J. Chem. Phys. 124 054501
[14] Root S, Gupta Y M 2007 Chem. Phys. Lett. 442 293
[15] Bridgman P W 1914 Phys.Rev. 3 153
[16] Akella J, Kennedy G 1971 J. Chem. Phys. 55 793
[17] Cansell F, Fabre D, Petitet J 1993 J. Chem. Phys. 99 7300
[18] Ciabini L, Gorelli F A, Santoro M, Bini R, Schettino V, Mezour M 2005 Phys. Rev. B 72 094108
[19] Block S, Weir C E, Piermarini G J 1970 Science 169 586
[20] Piermarini G J, Mighell A D, Weir C E, Block S 1969 Science 165 1250
[21] Klein R M, Nourbakhsh M, Adler P M 1968 J. Mater. Sci. 3 657
[22] Ciabini L, Santoro M, Bini R, Schettino V 2001 J.Chem.Phys. 115 3742
[23] Wang L L, Yu T X, Li Y C 1992 Advance in Shock Dynamics (Hefei:University of Science and Technology of China Press) p117—120 (in Chinese) [王礼立、余同希、李永池 1992 冲击动力学进展(合肥:中国科学技术大学出版社)第117—120页]
[24] Li Y H, Liu F S, Ma H Y, Cheng X L, Ma X J, Sun Y Y, Zhang M J, Xue X D 2010 Acta Phy.Sin. 59 2104 (in Chinese) [李永宏、刘福生、马海云、程小理、马小娟、孙燕云、张明建、薛学东 2010 物理学报 59 2104]
[25] Kobayashi T, Sekine T 2000 Phys.Rev. B 62 5281
[26] Jing F Q 1999 Introduction to Experimental Equation of State (Beijing: Science Press ) p204—209,352—356 (in Chinese) [经福谦 1999 实验物态方程导引(北京:科学出版社) 第204—209,352—356页]
[27] Matsuda A, Nakamura K G, Kondo K 2002 Phys. Rev. B 65 17411
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[1] Xu Z Y 1988 Principle of phase transition (Beijing: Science Press ) p1—34,412—418 (in Chinese) [徐祖耀 1988 相变原理(北京:科学出版社)第1—34,412—418页]
[2] Tang Z P 2008 Shock-induced Phase Transformation (Beijing: Science Press) p88—105 (in Chinese) [唐志平 2008 冲击相变(北京:科学出版社)第88—105页]
[3] Zhang S L, Liu F S, Peng X J, Zhang M J, Li Y H, Ma X J, Xue X D 2010 Acta Phys. Sin. 59 (in Chinese)[张世来、刘福生、彭小娟、张明建、李永宏、马小娟、薛学东 2010 物理学报 59]
[4] Klein R M, Nourbakhsh M, Adler P M 1968 J.Mater.Sci. 3 657
[5] Dick R 1970 J. Chem. Phys. 52 6021
[6] Adams D M, Appleby 1977 Proc. R. Soc. London Ser. A 296 1896
[7] Matsuda A, Kondo K, Nakamura K G 2004 Jpn. J. Appl. Phys. Part 243 L1614
[8] Wang C, Zhang P 2010 J.Appl.Phys.107 083502
[9] Maillet J B, Pineau 2008 J. Chem. Phys. 128 224502
[10] Schmidt S C, Moore D S, Schiferl D, Shaner J W 1983 Phys. Rev. Lett. 50 661
[11] Thiery M M, Leger J M 1988 J. Chem. Phys. 89 4255
[12] Walsh J M, Rice M H 1957 J. Chem. Phys. 26 815
[13] Matsuda A, Kondo K, Nakamura K G 2006 J. Chem. Phys. 124 054501
[14] Root S, Gupta Y M 2007 Chem. Phys. Lett. 442 293
[15] Bridgman P W 1914 Phys.Rev. 3 153
[16] Akella J, Kennedy G 1971 J. Chem. Phys. 55 793
[17] Cansell F, Fabre D, Petitet J 1993 J. Chem. Phys. 99 7300
[18] Ciabini L, Gorelli F A, Santoro M, Bini R, Schettino V, Mezour M 2005 Phys. Rev. B 72 094108
[19] Block S, Weir C E, Piermarini G J 1970 Science 169 586
[20] Piermarini G J, Mighell A D, Weir C E, Block S 1969 Science 165 1250
[21] Klein R M, Nourbakhsh M, Adler P M 1968 J. Mater. Sci. 3 657
[22] Ciabini L, Santoro M, Bini R, Schettino V 2001 J.Chem.Phys. 115 3742
[23] Wang L L, Yu T X, Li Y C 1992 Advance in Shock Dynamics (Hefei:University of Science and Technology of China Press) p117—120 (in Chinese) [王礼立、余同希、李永池 1992 冲击动力学进展(合肥:中国科学技术大学出版社)第117—120页]
[24] Li Y H, Liu F S, Ma H Y, Cheng X L, Ma X J, Sun Y Y, Zhang M J, Xue X D 2010 Acta Phy.Sin. 59 2104 (in Chinese) [李永宏、刘福生、马海云、程小理、马小娟、孙燕云、张明建、薛学东 2010 物理学报 59 2104]
[25] Kobayashi T, Sekine T 2000 Phys.Rev. B 62 5281
[26] Jing F Q 1999 Introduction to Experimental Equation of State (Beijing: Science Press ) p204—209,352—356 (in Chinese) [经福谦 1999 实验物态方程导引(北京:科学出版社) 第204—209,352—356页]
[27] Matsuda A, Nakamura K G, Kondo K 2002 Phys. Rev. B 65 17411
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