Influence of driving-laser wavelength on emission of high-order harmonic wave generated by atoms irradiated by ultrashort laser pulse

Zhang Di-Yu; Lan Wen-Di; Li Xue-Feng; Zhang Su-Su; Guo Fu-Ming; Yang Yu-Jun

doi:10.7498/aps.71.20220743

Abstract

With the numerical solution of the time-dependent Schrodinger equation, we theoretically investigate the high-order harmonic emissions generated by the atoms irradiated by the ultrashort lasers with different wavelengths but the same pondermotive energy. As the driving-laser wavelength increases, the intensity of the high-harmonic emission decreases. Comparing with the harmonic spectra of atoms driven by a 1000-nm-wavelength laser pulse, a new peak structure appears in the spectra of atoms driven by a 5000-nm-wavelength laser wavelength. It is shown by the time-frequency analysis of the harmonic emission, the time-dependent evolution of the electron density, and the time-dependent population analysis of the eigenstate, that the physical mechanism behind the new peak appearing in the harmonic spectra is the interference between the harmonic emission generated by the electrons ionized out of the excited atoms returning to the parent ions and the harmonic emissions resulting from the ground state ionization.

Keywords:

Authors and contacts

1.
Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China
2.
Jilin Provincial Key Laboratory of Applied Atomic and Molecular Spectroscopy, Jilin University, Changchun 130012, China

Corresponding author: Yang Yu-Jun, yangyj@jlu.edu.cn

Funds: Project supported by the National Major Research Plan of China (Grant No. 2019YFA0307700) and the National Natural Science Foundation of China (Grant Nos. 12074145, 11627807, 11774129)

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References

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Cited By

图 1 波长为1000 nm (黑色点线)和5000 nm (红色实线)的驱动激光与原子作用产生的高次谐波发射

Figure 1. High-order harmonic generated from an atom irradiated by the driving lasers with wavelengths of 1000 nm (black dotted line) and 5000 nm (red solid line)

DownLoad: Full-Size Img PowerPoint

图 2 Keldysh参数为0.3, 波长为1000−5000 nm的驱动激光与原子作用产生的高次谐波发射随波长的改变

Figure 2. When the Keldysh parameter is 0.3, the variation of the high-order harmonic radiation intensity with the driving laser wavelength in the 1000−5000 nm range

DownLoad: Full-Size Img PowerPoint

图 3 波长为1000 nm的驱动激光与原子作用产生的高次谐波发射的时间行为, 图中黑色和紫色实线为经典三步模型计算的发光能量

Figure 3. Temporal behavior of high-order harmonic generated by the atom irradiated by the driving laser with a wavelength of 1000 nm, the black and purple line represent the energy calculated by the simple man model

DownLoad: Full-Size Img PowerPoint

图 4 (a)波长为5000 nm的驱动激光与原子作用产生的高次谐波发射的时间行为; (b)电子的概率密度随着时间的变化

Figure 4. (a) Temporal behavior of high-order harmonic generated by the irradiated by the driving laser with a wavelength of 5000 nm; (b) variation of electron probability density with time

DownLoad: Full-Size Img PowerPoint

图 5 (a)波长为1000 nm和(b) 5000 nm驱动激光辐照原子的激发态布居(红色点线)和电离态布居(黑色实线)随着时间的变化

Figure 5. Variation of excited states population (red dotted line) and continuum states population (black solid line) of atoms irradiated with a driving laser at a wavelength of (a) 1000 nm and (b) 5000 nm with time

DownLoad: Full-Size Img PowerPoint

图 6 利用谐波能量2.5—4.0 a.u.的谐波发射合成的超短脉冲强度随着时间的改变

Figure 6. Variation of intensity of ultrashort pulses (synthesized by harmonic emission with harmonic energy 2.5–4.0 a.u.)with time

DownLoad: Full-Size Img PowerPoint

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