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超分子凝胶与介观结构

林乃波 林友辉 黄巧玲 刘向阳

超分子凝胶与介观结构

林乃波, 林友辉, 黄巧玲, 刘向阳
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  • 从介观结构角度综述了超分子凝胶晶体网络结构的形成机理、结构特性对宏观性能的影响以及超分子凝胶的设计与调控,系统总结了超分子凝胶的表征方法. 超分子凝胶的性能由层级结构决定,介观结构可大幅提高材料的宏观性能,其结构与性能可以通过四个因素相关联:拓扑结构,相关长度,对称性/有序性和晶体网络间的结合力. 基于对超分子凝胶的介观概念更深、更新的理解,该类材料的研究和开发将被推向新的阶段.
      通信作者: 刘向阳, phyliuxy@nus.edu.sg
    • 基金项目: 111计划(批准号:B16029)、国家自然科学基金(批准号:21404087,U1405226 21401154)和国家高技术研究发展计划(批准号:2011AA06Z228)、福建省科技厅项目(批准号:2014H6022,2015J05109)、广东省自然科学基金(批准号:2015A030310007,2014A030310005)、 中组部千人计划项目和厦门大学校长基金(批准号:20720160088,20720150218,20720140528)资助的课题.
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  • [1]

    Li J L, Liu X Y 2013 Soft Fibrillar Materials: fabrication and applications (Vol. 1) (Weinheim, Germany: Wiley-VCH Verlag GmbH Co. KGaA) p163

    [2]

    Hemminger J 2012 From Quanta to the Continuum: Opportunities for Mesoscale Science (Vol. 1) (U.S. Department of Energy: Basic Energy Sciences Advisory Committee)

    [3]

    Xu G, Gong L, Yang Z, Liu X 2014 Soft Matt. 10 2116

    [4]

    Lin N, Liu X Y 2015 Chem. Soc. Rev. 44 7881

    [5]

    Sangeetha N M, Maitra U 2005 Chem. Soc. Rev. 34 821

    [6]

    Foster J A, Steed J W 2010 Angew. Chem. Int. Ed. 49 6718

    [7]

    Yu G, Yan X, Han C, Huang F 2013 Chem. Soc. Rev. 42 6697

    [8]

    Xiong J Y, Liu X Y, Li J L, Vallon M W 2007 J. Phys. Chem. B 111 5558

    [9]

    Estroff L A, Hamilton A D 2004 Chem. Rev. 104 1201

    [10]

    Garlaschelli L, Ramaccini F, Delia Sala S 1991 Nature 353 507

    [11]

    Lipowitz A 1841 Justus Liebigs Ann. Chem. 38 348

    [12]

    Lin N, Toh G W, Feng Y, Liu X Y, Xu H 2014 J. Mater. Chem. B 2 2136

    [13]

    Seiffert S, Anthamatten M 2015 Supramolecular Polymer Networks and Gels (Vol. 268) (Switzerland: Springer) p1

    [14]

    Nguyen A T, Huang Q L, Yang Z, Lin N, Xu G, Liu X Y 2015 Small 11 1039

    [15]

    Li J L, Liu X Y 2009 J. Phys. Chem. B,113 15467

    [16]

    Liu X Y, Sawant P D, Tan W B, Noor I, Pramesti C, Chen B 2002 J. Am. Chem. Soc. 124 15055

    [17]

    Liu X Y, Sawant P D 2001 Appl. Phys. Lett. 79 3518

    [18]

    Liu X Y, Sawant P D 2002 Chemphyschem. 3 374

    [19]

    Liu X Y, Sawant P D 2002 Adv. Mater. 14 421

    [20]

    Sawant P D, Liu X Y 2002 Chem. Mater. 14 3793

    [21]

    Albert R, Barabsi A L 2002 Rev. Mod. Phys. 74 47

    [22]

    Yu R, Lin N, Yu W D, Liu X Y 2015 Cryst. Eng. Comm. 17 7986

    [23]

    Li J L, Liu X Y 2010 Adv. Funct. Mater. 20 3196

    [24]

    Xiong J Y, Liu X Y, Li J L, Vallon M W 2007 J. Phys. Chem. B 111 5558

    [25]

    Yuan B, Li J L, Liu X Y, Ma Y Q, Xu H Y 2011 Chem. Commun. 47 2793

    [26]

    Yuan B, Li J L, Liu X Y, Ma Y Q, Wang Y J 2012 Soft Matt. 8 5187

    [27]

    Li J L, Liu X Y, Wang R Y, Xiong J Y 2005 J. Phys. Chem. B 109 24231

    [28]

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    [29]

    Vandewalle N, Ausloos M 1997 Phys. Rev. E 55 94

    [30]

    Avrami M 1939 J. Chem. Phys. 7 1103

    [31]

    Witten Jr T, Sander L M 1981 Phys. Rev. Lett. 47 1400

    [32]

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    [34]

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    Diao Y Y, Liu X Y 2012 Adv. Funct. Mater. 22 1354

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    [38]

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    [39]

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    [40]

    Yu R, Lin N, Yu W D, Liu X Y 2015 Cryst. Eng. Comm. 17 7986

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    [42]

    Liu X Y, 2005 Low Molecular Mass Gelators: Design, Self-Assembly, Function (Vol. 256) (Berlin: Springer) p1

    [43]

    Xiong J Y, Narayanan J, Liu X Y, Chong T K, Chen S B, Chung T S 2005 J. Phys. Chem. B 109 5638

    [44]

    Xiong J, Liu X, Li J, Narayanan J, Wang R 2006 Appl. Phys. Lett. 89 083106

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    Tang S, Liu X Y, Strom C S 2009 Adv. Funct. Mater. 19 2252

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    Huang X, Terech P, Raghavan S R, Weiss R G 2005 J. Am. Chem. Soc. 127 4336

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    Huang X, Raghavan S R, Terech P, Weiss R G 2006 J. Am. Chem. Soc. 128 15341

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    Lam R, Quaroni L, Pedersen T, Rogers M A 2010 Soft Matt. 6 404

    [52]

    Terech P, Wade R 1988 J. Colloid Interface Sci. 125 542

    [53]

    George S J, Ajayaghosh A 2005 Chemistry 11 3217

    [54]

    Abdallah D J, Weiss R G 2000 Langmuir 16 352

    [55]

    Sakurai K, Ono Y, Jung J H, Okamoto S, Sakurai S, Shinkai S 2001 Journal of the Chemical Society, Perkin Transactions 2 108

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    Sakurai K, Jeong Y, Koumoto K, Friggeri A, Gronwald O, Sakurai S, Okamoto S, Inoue K, Shinkai S 2003 Langmuir 19 8211

    [57]

    Jeong Y, Hanabusa K, Masunaga H, Akiba I, Miyoshi K, Sakurai S, Sakurai K 2005 Langmuir 21 586

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    Takeno H, Mochizuki T, Yoshiba K, Kondo S, Dobashi T 2009 Gels: Structures, Properties, and Functions (Vol. 136) (Berlin: Springer) pp47-53

    [59]

    Wilder E A, Hall C K, Spontak R J 2003 J. Colloid Interface Sci. 267 509

    [60]

    Wilder E A, Braunfeld M B, Jinnai H, Hall C K, Agard D A, Spontak R J 2003 J. Phys. Chem. B 107 11633

    [61]

    Xu D H, Wang Z G, Douglas J F 2008 Macromolecules 41 815

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    Schnablegger H, Singh Y 2013 The SAXS Guide (Vol. 1) (Austria: Anton Paar GmbH)

    [63]

    Weiss R G, Terech P 2006 Molecular Gels: Materials with Self-assembled Fibrillar Networks (Vol. 1) (Dordrecht: Springer) p1

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    Bouas-Laurent H, Desvergne J P 2006 Optical Spectroscopic Methods as Tools to Investigate Gel Structures (Vol. 1) (Amsteldam: Springer) p363

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    Kotova O, Daly R, dos Santos C M, Boese M, Kruger P E, Boland J J, Gunnlaugsson T 2012 Angew. Chem. Int. Ed. 51 7208

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    Liao X, Chen G, Liu X, Chen W, Chen F, Jiang M 2010 Angew. Chem. 122 4511

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    Carretti E, Bonini M, Dei L, Berrie B H, Angelova L V, Baglioni P, Weiss R G 2010 Acc. Chem. Res. 43 751

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    Yuan B, Liu X Y, Li J L, Xu H Y 2011 Soft Matt. 7 1708

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    Wu X, Liu X Y, Du N, Xu G, Li B 2009 Appl. Phys. Lett. 95 093703

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    Nguyen A T, Huang Q L, Yang Z, Lin N, Xu G, Liu X Y 2015 Small 11 1013

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    Wrthner F, Hanke B, Lysetska M, Lambright G, Harms G S 2005 Org. Lett. 7 967

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    Lan Y, Corradini M G, Weiss R G, Raghavan S R, Rogers M A 2015 Chem. Soc. Rev. 44 6035

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    Liu X Y, Sawant P D 2002 Angew. Chem. Int. Ed. 114 3793

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    Zhan C, Wang J, Yuan J, Gong H, Liu Y, Liu M 2003 Langmuir 19 9440

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    Li J L, Liu X Y, Strom C S, Xiong J Y 2006 Adv. Mater. 18 2574

    [84]

    Hanabusa K, Matsumoto M, Kimura M, Kakehi A, Shirai H 2000 J. Colloid Interface Sci. 224 231

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    Makarević J, Jokić M, Perić B, Tomiić V, Kojić-Prodić B, Žinić M 2001 Chemistry 7 3328

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    Zhao C X, Wang H T, Li M 2014 Acta Phys.-Chim. Sin. 30 2197 (in Chinese) [赵呈孝, 王海涛, 李敏 2014 物理化学学报 30 2197]

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  • 收稿日期:  2016-04-22
  • 修回日期:  2016-05-26
  • 刊出日期:  2016-09-05

超分子凝胶与介观结构

  • 1. 厦门大学材料学院, 物理科学与技术学院, 生物仿生及软物质研究院, 福建省柔性功能材料重点实验室, 厦门 361005;
  • 2. 新加坡国立大学物理系, 新加坡 117542
  • 通信作者: 刘向阳, phyliuxy@nus.edu.sg
    基金项目: 

    111计划(批准号:B16029)、国家自然科学基金(批准号:21404087,U1405226 21401154)和国家高技术研究发展计划(批准号:2011AA06Z228)、福建省科技厅项目(批准号:2014H6022,2015J05109)、广东省自然科学基金(批准号:2015A030310007,2014A030310005)、 中组部千人计划项目和厦门大学校长基金(批准号:20720160088,20720150218,20720140528)资助的课题.

摘要: 从介观结构角度综述了超分子凝胶晶体网络结构的形成机理、结构特性对宏观性能的影响以及超分子凝胶的设计与调控,系统总结了超分子凝胶的表征方法. 超分子凝胶的性能由层级结构决定,介观结构可大幅提高材料的宏观性能,其结构与性能可以通过四个因素相关联:拓扑结构,相关长度,对称性/有序性和晶体网络间的结合力. 基于对超分子凝胶的介观概念更深、更新的理解,该类材料的研究和开发将被推向新的阶段.

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