开放式法布里-珀罗光学微腔中光与单量子系统的相互作用

裴思辉; 宋子旋; 林星; 方伟

doi:10.7498/aps.71.20211970

摘要

光与物质相互作用的过程具有丰富的物理内涵, 不仅有助于理解光的本质, 更可以提供一种有效操控物质的手段. 开放式光学微腔具有光场强局域性、频率域和空间域的可调谐性以及光纤可集成性等特点, 为研究微腔内的光与物质相互作用提供了一个理想平台. 本文首先介绍基于开放式法布里-珀罗微腔的腔量子电动力学系统的基本特性, 然后介绍开放式法布里-珀罗微腔结构的制备方法, 进而从弱耦合、强耦合和差发射体三方面着重介绍近年来开放式微腔与固态单量子系统相互作用的研究工作, 最后进行了总结与展望.

关键词:

Abstract

The interaction between light and matter has attracted much attention not only for fundamental research but also for applications. The open Fabry-Perot cavity provides an excellent platform for such a study due to strong optical confinement, spectral and spatial and tunability, and the feasibility of optical fiber integration. In this review, first, the basic properties of open Fabry-Perot cavities and the fabrication techniques are introduced. Then recent progress of weak coupling, strong coupling and bad emitter regimes is discussed. Finally, the challenges to and perspectives in this respect are presented.

Keywords:

作者及机构信息

1.
浙江大学光电科学与工程学院, 现代光学仪器国家重点实验室, 杭州　310058

2.
浙江大学信息与电子工程学院, 杭州　310058

通信作者: 林星, lxing@zju.edu.cn ; 方伟, wfang08@zju.edu.cn

基金项目: 国家重点研发计划(批准号: 2018YFB2200404)、国家自然科学基金(批准号: 62035013, 61635009, 62075192)和中央高校基本科研业务费专项资金(批准号: 2021QNA5006).

Authors and contacts

1.
State Key Laboratory of Modern Optical Instrumentation, College of Optical Science and Engineering, Zhejiang University, Hangzhou 310058,China

2.
College of Information Science & Electronic Engineering, Zhejiang University,Hangzhou 310058, China

Corresponding author: Lin Xing, lxing@zju.edu.cn ; Fang Wei, wfang08@zju.edu.cn

Funds: Project supported by the National Key Research and Development Program of China (Grant No. 2018YFB2200404), the National Natural Science Foundation of China (Grant Nos. 62035013, 61635009, 62075192), and the Fundamental Research Funds for the Central Universities, China (Grant No. 2021QNA5006).

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施引文献

图 1 腔与TLS耦合的原理图. 该系统可通过3个参数进行描述: $ g, \kappa $ 和$ \gamma $, 它们分别量化了TLS与腔的耦合、腔损耗速率以及TLS的非共振自发辐射

Fig. 1. Schematic diagram of the operational principle for TLS coupling to the cavity. The system is described by three parameters:$ g $, $ \kappa $, and$ \gamma $ which quantify the cavity-TLS coupling, the photon decay from the cavity, and the non-resonant spontaneous emission of the TLS, respectively.

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图 2 JC模型下腔与TLS耦合前后的能级示意图. 当TLS与腔内光子共振时, 该系统的能级发生劈裂, 且劈裂量会随着腔内光子数的增大而增大

Fig. 2. States of the cavity-two level system coupled system described by JC model. When the TLS comes into resonance with optical modes of the cavity, a generated energy level of the system will split into two with an energy difference. The magnitude of the splitting increases with the number of photons stored in the cavity.

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图 3 开放式FP微腔的基本结构　(a), (b) 基于光纤端面的开放式FP微腔, 其中(a)光纤-光纤型^[17], (b)光纤-芯片型^[25]; (c)基于芯片的开放式FP微腔^[26]

Fig. 3. Basic structure of open FP microcavity. (a), (b) Open FP microcavity based on fiber end face: (a) Fiber-fiber type^[17]; (b) fiber-chip type^[25]. (c) chip-based open FP microcavity^[26].

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图 4 早期的开放式FP微腔结构　(a)利用湿法刻蚀制备的第一个光纤-芯片型开放式FP微腔^[36]; (b)利用气泡法制备光滑凹面结构^[37]; (c) 利用转移技术制备的光纤型开放式FP微腔^[38]; (d) 利用乳胶球辅助电化学沉积技术制备的凹面尺寸可控的微腔^[39]

Fig. 4. Early open FP microcavity structures: (a) The first fiber-chip type open FP microcavity fabricated by wet etching^[36] ; (b) preparation of smooth concave structure by bubble method^[37]; (c) fiber type FP microcavity fabricated by transfer technique^[38]; (d) microcavity with controllable concave size prepared by latex ball assisted electrochemical deposition technique^[39].

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图 5 早期利用CO₂激光烧蚀法构建光纤型FP腔的工作^[17]　(a)微腔结构示意图; (b) CO₂激光脉冲处理后光纤端面的扫描电子显微镜图; (c) 利用干涉显微镜得到的曲面形貌(实线)与理想高斯形貌(虚线)的差别

Fig. 5. Early fiber-type FP microcavity made by CO₂ laser ablation method^[17]: (a) Schematic diagram of cavity structure; (b) scanning electron microscope image of fiber endface after CO₂ laser pulse treatment; (c) surface topography (solid line) obtained by interference microscope and an ideal Gaussian profile (dotted line).

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图 6 最早利用FIB刻蚀法制备芯片型开放式FP微腔的工作^[34]　(a)腔结构示意图; (b)凹面阵列的扫描电子显微镜照片; (c)原子力显微镜得到的曲面面型(蓝线)以及拟合的光滑曲面(绿线), 面型粗糙度约0.7 nm

Fig. 6. The earliest chip-type FP microcavity made by FIB etching technique^[34]: (a) Schematic diagram of cavity structure; (b) scanning electron microscope image of the processed concave mirror array; (c) surface profile (blue line) obtained by atomic force microscope and the fitting curve (green line). The surface roughness is 0.7 nm.

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图 7 可实现强耦合的典型量子点-腔系统^[80]　(a)量子点-腔系统结构; (b)为了控制量子点的电荷, 量子点层下面的n掺杂GaAs层与其上面的p掺杂GaAs层一起形成p-i-n二极管结构; (c)通过调节腔长优化量子点和腔之间的耦合, 基于该平台得到了具有反交叉特征的共振透射光谱

Fig. 7. Typical quantum dot (QD)-cavity system in which the strong coupling could be observed^[80]: (a) Setup of the QD-cavity system; (b) the n-doped GaAs layer below the QD layer and the p-doped GaAs layer above forming a p-i-n diode structure, which is used to control the charge state of the QDs; (c) the cavity length is adjusted to optimize the coupling between the QD and the cavity, an anti-crossing in resonant transmission spectroscopy is observed.

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图 8 差发射体区域Purcell因子与模式体积的关系^[14], 其中离散点为实验数据, 实线是将有效$ Q $值代入(14)式计算得到

Fig. 8. Purcell enhancement as a function of mode volume in bad emitter regime^[14]. The discrete points are derived from the experimental data, and the solid line is calculated by substituting the effective Q value into Eq.(14).

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表 1 开放式FP微腔的性能比较

Table 1. Performance comparison of open FP microcavities.

制备方法	反射膜层	结构	年份	$\mathit{L}/\text{μm }$	$\mathit{R}/\text{μm }$	$ \mathit{F} $	文献
湿法刻蚀	Au	光纤型	2005	$ 20—200 $	$ 185 $	$ ~100 $	[36]
气泡法	DBR	芯片型	2006	$ 40—60 $	$ 40—100 $	$ 200 $	[37]
转移法	DBR	光纤型	2006	$ 27 $	$ 1000 $	$ 1050 $	[38]
电化学沉积	Au	芯片型	2007	$ 6.5—9.7 $	$ 10 $	$ ~15 $	[39]
CO₂激光烧蚀	DBR	光纤型	2007	$ 38.6 $	$ 150 $	$ 37000 $	[46]
	DBR	光纤型	2010	$ 20—60 $	$ 40—2000 $	$ 38600 $	[17]
	DBR	光纤型	2012	$ 20—2000 $	$ 20—2000 $	$ 100000 $	[47]
	DBR	光纤型	2013	$ 206 $	$ 209 $	$ 45000 $	[48]
	DBR	芯片型	2014	$ 1.34 $	$ 10 $	$ 15000 $	[26]
	DBR	芯片型	2017	$ 1.33 $	$ ~5 $	$ 25000 $	[49]
	DBR	光纤型	2017	$ 100 $	$ 200—360 $	$ 1300 $	[29]
	DBR	光纤型	2018	$ 20 $	$ 66 $	$ 40000 $	[50]
	DBR	光纤型	2019	$ 4 $	$ 43 $	$ ~60 $	[25]
FIB刻蚀	DBR	芯片型	2010	$ 3—13 $	$ 5—25 $	$ 460 $	[34]
	DBR	芯片型	2012	$ 1.6 $	$ 7 $	$ ~1280 $	[14]
	DBR	光纤型	2014	$ 5.6 $	$ 14.1 $	$ 3600 $	[51]*
	DBR	芯片型	2015	$ 1.55 $	$ 4.3 $	$ ~1000 $	[33]
	DBR	芯片型	2016	$ 3 $	$ 6 $	$ ~1000 $	[32]
	DBR	芯片型	2018	$ 2.2 $	$ ~10 $	—	[52]
	DBR	芯片型	2021	1	—	$ 2500 $	[53]
注: 1)所选取微腔参数范围是对应文献典型微腔的参数, 并非涉及文献中所有微腔; 2)部分文献未直接给出F的值, 这里根据(3)式和(4)式进行换算; 3)带*标注是指文献[51]引用参数对应微腔一个端镜由FIB刻蚀产生, 另一个由CO₂激光烧蚀产生; 4)这里R指的是微腔两面端镜的曲率半径中较小的.

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表 2 开放式FP微腔在弱耦合中的典型应用

Table 2. Typical applications of open FP microcavity in weak coupling regime.

年份	结构	加工方法	量子体系	$ {F}_{\mu } $	文献
2009	光纤型	转移法	InAs量子点	—	[12]
2011	芯片型	激光烧蚀	AlGaAs量子点	1.6	[13]
2015	芯片型	FIB刻蚀	InGaAs量子点	2.54	[55]
2015	芯片型	FIB刻蚀	NV色心	6.25^*	[62]
2017	芯片型	激光烧蚀	NV色心	>30^*	[63]
2021	芯片型	激光烧蚀	InGaAs量子点	12	[5]
注: 针对NV色心零声子线辐射速率的增强倍率.

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表 3 开放式FP微腔在强耦合中的典型应用

Table 3. Typical applications of open FP microcavity in strong coupling regime.

年份	结构	加工方法	量子体系	$ \mathrm{协}\mathrm{同}\mathrm{参}\mathrm{数}C $	$ Q $	文献
2013	光纤型	激光烧蚀	InGaAs量子点	2.0±1.3	30000	[80]
2015	光纤型	激光烧蚀	InAs量子点	5.5	60000	[81]
2019	芯片型	激光烧蚀	InAs量子点	150	170000	[59]
2019	光纤型	FIB刻蚀	DBT分子	12.7	120000	[31]
2021	光纤型	FIB刻蚀	DBT分子	45	120000	[82]

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