驱动激光波长对超短脉冲与原子相互作用产生高次谐波发射的影响

张頔玉; 蓝文迪; 李雪峰; 张稣稣; 郭福明; 杨玉军

doi:10.7498/aps.71.20220743

摘要

通过数值求解含时薛定谔方程方案, 理论研究了在有质动力能不变条件下, 不同波长超短激光辐照原子产生的高次谐波发射. 发现随着驱动激光波长的增加, 谐波发射的强度降低且发射谱中出现新的峰值结构. 通过谐波发射行为的时间频率分析, 电子密度的含时演化以及本征态布居含时分析发现, 谐波新的峰值产生根源是电子从激发态电离后返回母体离子产生的谐波发射与从基态电离产生的谐波发射之间的干涉.

关键词:

With the numerical solution of the time-dependent Schrodinger equation, we theoretically investigate the high-order harmonic emissions generated by the atoms irradiated by the ultrashort lasers with different wavelengths but the same pondermotive energy. As the driving-laser wavelength increases, the intensity of the high-harmonic emission decreases. Comparing with the harmonic spectra of atoms driven by a 1000-nm-wavelength laser pulse, a new peak structure appears in the spectra of atoms driven by a 5000-nm-wavelength laser wavelength. It is shown by the time-frequency analysis of the harmonic emission, the time-dependent evolution of the electron density, and the time-dependent population analysis of the eigenstate, that the physical mechanism behind the new peak appearing in the harmonic spectra is the interference between the harmonic emission generated by the electrons ionized out of the excited atoms returning to the parent ions and the harmonic emissions resulting from the ground state ionization.

Keywords:

作者及机构信息

1.
吉林大学原子与分子物理研究所, 长春　130012

2.
吉林省应用原子与分子光谱重点实验室, 长春　130012

通信作者: 杨玉军, yangyj@jlu.edu.cn

基金项目: 国家重大研究计划(批准号: 2019YFA0307700)和国家自然科学基金(批准号: 12074145, 11627807, 11774129)资助的课题

Authors and contacts

1.
Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China

2.
Jilin Provincial Key Laboratory of Applied Atomic and Molecular Spectroscopy, Jilin University, Changchun 130012, China

Corresponding author: Yang Yu-Jun, yangyj@jlu.edu.cn

Funds: Project supported by the National Major Research Plan of China (Grant No. 2019YFA0307700) and the National Natural Science Foundation of China (Grant Nos. 12074145, 11627807, 11774129)

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参考文献

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施引文献

图 1 波长为1000 nm (黑色点线)和5000 nm (红色实线)的驱动激光与原子作用产生的高次谐波发射

Fig. 1. High-order harmonic generated from an atom irradiated by the driving lasers with wavelengths of 1000 nm (black dotted line) and 5000 nm (red solid line)

下载: 全尺寸图片幻灯片

图 2 Keldysh参数为0.3, 波长为1000−5000 nm的驱动激光与原子作用产生的高次谐波发射随波长的改变

Fig. 2. When the Keldysh parameter is 0.3, the variation of the high-order harmonic radiation intensity with the driving laser wavelength in the 1000−5000 nm range

下载: 全尺寸图片幻灯片

图 3 波长为1000 nm的驱动激光与原子作用产生的高次谐波发射的时间行为, 图中黑色和紫色实线为经典三步模型计算的发光能量

Fig. 3. Temporal behavior of high-order harmonic generated by the atom irradiated by the driving laser with a wavelength of 1000 nm, the black and purple line represent the energy calculated by the simple man model

下载: 全尺寸图片幻灯片

图 4 (a)波长为5000 nm的驱动激光与原子作用产生的高次谐波发射的时间行为; (b)电子的概率密度随着时间的变化

Fig. 4. (a) Temporal behavior of high-order harmonic generated by the irradiated by the driving laser with a wavelength of 5000 nm; (b) variation of electron probability density with time

下载: 全尺寸图片幻灯片

图 5 (a)波长为1000 nm和(b) 5000 nm驱动激光辐照原子的激发态布居(红色点线)和电离态布居(黑色实线)随着时间的变化

Fig. 5. Variation of excited states population (red dotted line) and continuum states population (black solid line) of atoms irradiated with a driving laser at a wavelength of (a) 1000 nm and (b) 5000 nm with time

下载: 全尺寸图片幻灯片

图 6 利用谐波能量2.5—4.0 a.u.的谐波发射合成的超短脉冲强度随着时间的改变

Fig. 6. Variation of intensity of ultrashort pulses (synthesized by harmonic emission with harmonic energy 2.5–4.0 a.u.)with time

下载: 全尺寸图片幻灯片

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驱动激光波长对超短脉冲与原子相互作用产生高次谐波发射的影响