Exotic states in moiré superlattices of twisted semiconducting transition metal dichalcogenides

Tang Yan-Hao

doi:10.7498/aps.72.20222080

Abstract

Moiré superlattices formed by van der Waals materials with small lattice mismatch or twist angle open an unprecedented approach to generate flat bands that don’t exist in the “parent” materials, which provides a controllable platform for exploring quantum many body physics. Owing to the wide angle range for the existence of flat bands, as well as the valley-spin-locking band structure and the excellent optical properties, twisted semiconducting transition metal dichalcogenides (TMDs) heterostructures have recently attracted lots of attention. In this review, we discuss the exotic states discovered in the twisted TMDs heterostructures, including Mott insulator, generalized Wigner crystals, topological non-trivial states, and moiré excitons, how to manipulate these exotic states and related mechanisms, and finally some perspectives on the opportunities and challenges in this field.

Keywords:

Authors and contacts

Tang Yan-Hao

Interdisciplinary Center for Quantum Information, Zhejiang Province Key Laboratory of Quantum Technology, Department of Physics, Zhejiang University, Hangzhou 310063, China

Corresponding author: Tang Yan-Hao, yanhaotc@zju.edu.cn

Funds: Project supported by the National Basic Research Program of China (Grant Nos. 2022YFA1405400, 2022YFA1402403) and the National Natural Science Foundation of China (Grant No. 12274365).

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Cited By

图 1 转角TMDs的晶格和能带结构0°转角 (a)和60°转角 (b) TMDs异质结的晶格结构示意图; (c)转角WSe₂/MoSe₂的能带图^[17]; (d)不同晶格位之间跃迁的动能随莫尔晶格常数的依赖关系^[17]

Figure 1. Crystal structure and band structure in twisted TMDs: The crystal structure in 0° (a) and 60° (b) twisted TMDs heterobilayer; (c) the moiré band structure of low-energy electrons in 2° twisted WSe₂/MoSe₂ heterobilayer^[17]; (d) the kinetic energy of electrons hopping between different moiré sites as a function of the moiré lattice constant^[17].

DownLoad: Full-Size Img PowerPoint

图 2 转角TMDs中的关联绝缘态的电荷分布示意图

Figure 2. The schematic of the correlated states in twisted TMDs.

DownLoad: Full-Size Img PowerPoint

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