磁空混合约束激光诱导Cu等离子体光谱特性

李百慧; 高勋; 宋超; 林景全

doi:10.7498/aps.65.235201

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磁空混合约束激光诱导Cu等离子体光谱特性

李百慧 , 高勋 , 宋超 , 林景全

磁空混合约束激光诱导Cu等离子体光谱特性

李百慧, 高勋, 宋超, 林景全

物理学报. 2016, 65(23): 235201.

doi: 10.7498/aps.65.235201.

摘要

本文基于发射光谱法对磁空混合约束铜等离子体光谱特性进行了研究，分析了磁空混合约束条件下铜等离子体光谱强度演化过程以及等离子体光谱轴向和横向分布.实验结果表明，在磁空混合约束和空间约束条件下等离子体光谱均出现增强，对原子光谱Cu I 521.8 nm的最大增强因子分别为2和1.2，磁空混合作用等离子体离子光谱增强效果大于纯空间约束情形.在磁空混合约束作用下，光谱增强在小延时来源于磁场约束产生，而大延时为空间约束产生.结合光学阴影成像法，分析了Cu I 521.8 nm谱线强度的轴向和横向空间强度分布，由于空间约束作用的冲击波反射压缩，使等离子体羽横向膨胀方向存在约束，使等离子体内原子数密度最大空间位置前移，造成了磁空混合约束下Cu I 521.8 nm谱线强度的轴向最大空间位置远离铜表面.

关键词:

作者及机构信息

1.
长春理工大学理学院, 长春 130022;

2.
长春理工大学化学与环境工程学院, 长春 130022

通信作者: 高勋, lasercust@163.com

基金项目: 国家自然科学基金（批准号：61575030）资助的课题.

参考文献

[1]	Hemmerlin M, Meilland R, Falk H, Wintjens P, Paulard L 2001 Spectrochim. Acta Part B At. Spectrosc. 56 661
[2]	Michel A P, Lawrencesnyder M, Angel S M, Chave A D 2007 Appl. Opt. 46 2507
[3]	Hanafi M, Omar M M, Gamal E D 2000 Radiat. Phys. Chem. 57 11
[4]	Asimellis G, Hamilton S, Giannoudakos A, Kompitsas M 2005 Spectrochim. Acta Part B At. Spectrosc. 60 1132
[5]	Du C, Gao X, Shao Y, Song X W, Zhao Z M, Hao Z Q, Lin J Q 2013 Acta Phys. Sin. 62 045202 (in Chinese)[杜闯, 高勋, 邵妍, 宋晓伟, 赵振明, 郝作强, 林景全2013物理学报62 045202]
[6]	Harilal S S, Tillack M S, O'Shay B, Bindhu C V, Najmabadi F 2004 Phys. Rev. E 69 026413
[7]	Gao X, Liu L, Song C, Lin J Q 2015 J. Phys. D:Appl. Phys. 48 175205
[8]	Li C, Gao X, Liu L, Lin J Q 2014 Acta Phys. Sin. 63 145203 (in Chinese)[李丞, 高勋, 刘潞, 林景全2014物理学报63 145203]
[9]	Wang Z, Hou Z, Lui S L, Jiang D, Liu J, Li Z 2012 Opt. Express 20 1011
[10]	Shen X K, Sun J, Ling H, Lu Y F 2007 Appl. Phys. Lett. 91 081501
[11]	Guo L B, Hu W, Zhang B Y, He X N, Li C M, Zhou Y S, Cai Z X, Zeng X Y, Lu Y F 2011 Opt. Express 19 14067
[12]	Li Y, Hu C, Zhang H, Jiang Z, Li Z 2009 Appl. Opt. 48 B105
[13]	Pagano C, Hafeez S, Lunney J G 2009 J. Phys. D:Appl. Phys. 42 155205
[14]	Li C, Zhang L Y, Qian S W 1979 Thermology (Beijing:Higher Education Press) p72(in Chinese)[李椿, 章立源, 钱尚武1979热学(北京:高等教育出版社)第72页]
[15]	Qindeel R, Bidin N, Zia R, Daud Y M 2011 Optoelectron. Adv. Mat. Rapid Commun. 5 331
[16]	Tillack M S, Harilal S S, Najmabadi F, O'Shay J 2005 IFSA 5 45

施引文献

[1]	Hemmerlin M, Meilland R, Falk H, Wintjens P, Paulard L 2001 Spectrochim. Acta Part B At. Spectrosc. 56 661
[2]	Michel A P, Lawrencesnyder M, Angel S M, Chave A D 2007 Appl. Opt. 46 2507
[3]	Hanafi M, Omar M M, Gamal E D 2000 Radiat. Phys. Chem. 57 11
[4]	Asimellis G, Hamilton S, Giannoudakos A, Kompitsas M 2005 Spectrochim. Acta Part B At. Spectrosc. 60 1132
[5]	Du C, Gao X, Shao Y, Song X W, Zhao Z M, Hao Z Q, Lin J Q 2013 Acta Phys. Sin. 62 045202 (in Chinese)[杜闯, 高勋, 邵妍, 宋晓伟, 赵振明, 郝作强, 林景全2013物理学报62 045202]
[6]	Harilal S S, Tillack M S, O'Shay B, Bindhu C V, Najmabadi F 2004 Phys. Rev. E 69 026413
[7]	Gao X, Liu L, Song C, Lin J Q 2015 J. Phys. D:Appl. Phys. 48 175205
[8]	Li C, Gao X, Liu L, Lin J Q 2014 Acta Phys. Sin. 63 145203 (in Chinese)[李丞, 高勋, 刘潞, 林景全2014物理学报63 145203]
[9]	Wang Z, Hou Z, Lui S L, Jiang D, Liu J, Li Z 2012 Opt. Express 20 1011
[10]	Shen X K, Sun J, Ling H, Lu Y F 2007 Appl. Phys. Lett. 91 081501
[11]	Guo L B, Hu W, Zhang B Y, He X N, Li C M, Zhou Y S, Cai Z X, Zeng X Y, Lu Y F 2011 Opt. Express 19 14067
[12]	Li Y, Hu C, Zhang H, Jiang Z, Li Z 2009 Appl. Opt. 48 B105
[13]	Pagano C, Hafeez S, Lunney J G 2009 J. Phys. D:Appl. Phys. 42 155205
[14]	Li C, Zhang L Y, Qian S W 1979 Thermology (Beijing:Higher Education Press) p72(in Chinese)[李椿, 章立源, 钱尚武1979热学(北京:高等教育出版社)第72页]
[15]	Qindeel R, Bidin N, Zia R, Daud Y M 2011 Optoelectron. Adv. Mat. Rapid Commun. 5 331
[16]	Tillack M S, Harilal S S, Najmabadi F, O'Shay J 2005 IFSA 5 45

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物理学报. 2016, 65(23): 235201.

doi: 10.7498/aps.65.235201.

磁空混合约束激光诱导Cu等离子体光谱特性

1. 长春理工大学理学院, 长春 130022;
2. 长春理工大学化学与环境工程学院, 长春 130022

通信作者: 高勋, lasercust@163.com

基金项目:

国家自然科学基金（批准号：61575030）资助的课题.

收稿日期: 2016-08-07
修回日期: 2016-09-05
刊出日期: 2016-12-05

摘要: 本文基于发射光谱法对磁空混合约束铜等离子体光谱特性进行了研究，分析了磁空混合约束条件下铜等离子体光谱强度演化过程以及等离子体光谱轴向和横向分布.实验结果表明，在磁空混合约束和空间约束条件下等离子体光谱均出现增强，对原子光谱Cu I 521.8 nm的最大增强因子分别为2和1.2，磁空混合作用等离子体离子光谱增强效果大于纯空间约束情形.在磁空混合约束作用下，光谱增强在小延时来源于磁场约束产生，而大延时为空间约束产生.结合光学阴影成像法，分析了Cu I 521.8 nm谱线强度的轴向和横向空间强度分布，由于空间约束作用的冲击波反射压缩，使等离子体羽横向膨胀方向存在约束，使等离子体内原子数密度最大空间位置前移，造成了磁空混合约束下Cu I 521.8 nm谱线强度的轴向最大空间位置远离铜表面.

关键词:

English Abstract

Laser induced plasma spectral characteristics of Cu with magnetically and spatially combined confinement

1.
School of Science, Changchun University of Science and Technology, Changchun 130022, China;

2.
School of Chemistry and Environmental Engineering, Changchun University of Science and Technology, Changchun 130022, China

Fund Project:
Project supported by the National Natural Science Foundation of China (Grant No. 61575030).

Received Date: 07 August 2016
Accepted Date: 05 September 2016
Published Online: 05 December 2016

Abstract: In order to explore and understand the spectroscopic characteristics of laser induced plasma and spectral intensity distribution under magnetic-spatially combined confinement,in this paper,the laser induced breakdown plasma spectral characteristics of Cu with magnetic-spatially combined confinement,obtained by the optical emission spectroscopy and the optical shadow graph are studied.The temporal evolutions of spectral intensity and the axial and transversal distributions of Cu I 521.8 nm plasma spectrum with magnetic-spatially combined confinement are analyzed.The experimental results show that the laser induced Cu plasma spectra are all enhanced under the conditions of magneticspatially combined confinement and spatial confinement.In addition,the maximum enhancement factors of Cu I 521.8 nm in these two kinds of confinement conditions are 2 and 1.2,respectively.The enhanced effect of plasma ion spectrum in the magnetic-spatial field is stronger than that of spatial confinement.Under the effect of magnetic-spatially combined confinement,spectral enhancement mechanisms are derived from the magnetic field and spatial mixed actions.At the early stage of plasma expansion,the magnetic field action is a dominant factor.The charged particles in plasma are affected by the Lorenz force in the magnetic field which induces the charged particles to do the Lamor cyclotron motion, then the plasma expansion is restrained and the plasma volume decreases.The frequency of collisions between the electron and ion in the plasma increases.Therefore,the spectral intensities of atoms and ions are strengthened.For the case of the larger delay time,the spectral enhancement is caused by the spatial confinement.The axial and transversal spatial intensity distributions of Cu I 521.8 nm are analyzed by the optical shadow graph method.The plasma is compressed by the shock wave because the shock wave generated by the Cu plasma is reflected by the space plate.The transversal expansion of plasma plume is constrained by the spatial confinement,which causes the spatial position of the plasma internal atoms with high densityto move forward,and also induces the maximum axial spatial location of Cu I 521.8 nm spectral intensity to be far from the Cu metal surface.The results indicate that the axial distribution of plasma plume,obtained from the optical shadow graph is corresponding to the axial distribution of plasma spectrum obtained by the optical emission spectroscopy.In summary,the spectrum enhancement of laser induced plasma with the magnetic-spatial combined confinement is influenced by two forces:one is the magnetic force and the other is the compressive force caused by the shock wave.The study of the laser induced breakdown plasma spectral characteristics of Cu with magnetic-spatially combined confinement provides a simple and powerful tool for improving the sensitivity of laser induced breakdown spectroscopy.

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