合成参数对气-液-固法低温生长MgO纳米线的影响

赖云锋

doi:10.7498/aps.59.8814

摘要

将Mg(C11H19O2)2(即双(2, 2, 6, 6,-四甲基-3, 5-庚二酮酸)镁)作为反应前驱体,用脉冲液滴注入式金属有机物化学气相沉积法,在较低温度(T=600 ℃)下合成MgO纳米线.纳米线沿着[001]方向生长且Au催化剂位于纳米线顶端,这表明纳米线是由气-液-固机制诱导生长的.通过改变前驱体注入的脉冲周期或周期注入剂量能够控制纳米线的生长模式,使之垂直或平行于样品表面生长.

关键词:

纳米线 /
气-液-固机制 /
MgO

MgO nanowires are synthesized at a lower temperature (T=600 ℃) by pulsed liquid injection metal-organic chemical vapor deposition with Mg(C11H19O2)2 (magnesium bis (2, 2, 6, 6-tetramethyl-3, 5-heptanedionate)) as precursor. The MgO nanowires grow along the [001] direction with gold nanoparticles on the tips, which leads to the vapor-liquid-solid growth mechanism. The growth mode of nanowires (vertical growth to the substrate or parallel growth to the substrate) can be controlled by adjusting the injection period or the injection mass/period.

Keywords:

作者及机构信息

赖云锋

1.
福州大学物理与信息工程学院,微纳器件与太阳能电池研究所,福州 350108

基金项目: 国家自然科学基金(批准号:61006003)、福建省自然科学基金(批准号:2010J05134)、福州大学引进人才科研启动基金(批准号:0460022216)和福州大学科技发展基金(批准号:2009-XQ-32)资助的课题.

Authors and contacts

Lai Yun-Feng

1.
Institute of Micro-Nano Devices and Solar Cells, School of Physics and Information Engineering, Fuzhou University, Fuzhou 350108, China

参考文献

[1]	Ferry D K 2008 Science 319 579
[2]	Thelander C, Agarwal P, Brongersma S, Eymery J, Feiner L F, Forchel A, Scheffler M, Riess W, Ohlsson B J, Gosele U, Samuelson L 2006 Mater. Today 9 28
[3]	Jaey A, Nam S W, Friedman R S, Yan H, Lieber C M 2007 Nano Lett. 7 773
[4]	Zhanf F C, Zhang Z Y, Zhang W H, Yan J F, Yong J N 2009 Chin. Phys. B 18 2508
[5]	Zhang W, Li M K, Wei Q, Cao L, Yang Z, Qiao S S 2008 Acta Phys. Sin. 57 5887 (in Chinese) [张威、李梦轲、魏强、曹璐、杨志、乔双双 2008 物理学报 57 5887]
[6]	Zhang J Y, Deng T S, Shen X, Zhu K T, Zhang Q F, Wu J L 2009 Acta Phys. Sin. 58 4156 (in Chinese) [张俊艳、邓天松、沈昕、朱孔涛、张琦锋、吴锦雷 2009 物理学报 58 4156]
[7]	Yin Y D, Zhang G T, Xia Y N 2002 Adv. Funct. Mater. 12 293
[8]	Han S, Li C, Liu Z Q, Lei B, Zhang D H, Jin W, Liu X L, Tang T, Zhou C W 2004 Nano Lett. 4 1241
[9]	Kim H W, Shim S H 2006 Chem. Phys. Lett. 422 165
[10]	Nagashima K, Yanagida T, Tanaka H, Kawai T 2007 J. Appl. Phys. 101 124304
[11]	Yanagida T, Nagashima K, Tanaka H, Kawai T 2007 Appl. Phys. Lett. 91 061502
[12]	Kim G, Martens R L, Thompson G B, Kim B C, Gupta A 2007 J. Appl. Phys. 102 104906
[13]	Yang P D, Lieber C M 1997 J. Mater. Res. 12 2981
[14]	Xing H Y, Fan G H, Yang X L, Zhang G Y 2010 Acta Phys. Sin. 59 504 (in Chinese) [刑海英、范广涵、杨学林、张国义 2010 物理学报 59 504]
[15]	Zhang Z, Zhang R, Xie Z L, Liu B, Xiu X Q, Li Y, Fu D Y, Lu H, Chen P, Han P, Zheng Y D, Tang C G, Chen Y H, Wang Z G 2009 Acta Phys. Sin. 58 3416 (in Chinese) [张〖16] Senateur J P, Dubourdieu C, Weiss F, Rosina M, Abrutis A 2000 Adv. Mater. Opt. Electron. 10 155
[16]	Wagner R S, Ellis W C 1964 Appl. Phys. Lett. 4 89
[17]	Hanson M 1958 Constitution of Binary Alloys (New York: McGraw-Hill) p214
[18]	Givargizov E I 1975 J. Cryst. Growth 31 20
[19]	Blakely J M, Jackson K A 1962 J. Chem. Phys. 37 428
[20]	Dubrovskii V G, Cirlin G E, Soshnikov I P, Tokikh A A, Sibirev N V, Samsonenko Y B, Ustinov V M 2005 Phys. Rev. B 71 205325

施引文献

[1]	Ferry D K 2008 Science 319 579
[2]	Thelander C, Agarwal P, Brongersma S, Eymery J, Feiner L F, Forchel A, Scheffler M, Riess W, Ohlsson B J, Gosele U, Samuelson L 2006 Mater. Today 9 28
[3]	Jaey A, Nam S W, Friedman R S, Yan H, Lieber C M 2007 Nano Lett. 7 773
[4]	Zhanf F C, Zhang Z Y, Zhang W H, Yan J F, Yong J N 2009 Chin. Phys. B 18 2508
[5]	Zhang W, Li M K, Wei Q, Cao L, Yang Z, Qiao S S 2008 Acta Phys. Sin. 57 5887 (in Chinese) [张威、李梦轲、魏强、曹璐、杨志、乔双双 2008 物理学报 57 5887]
[6]	Zhang J Y, Deng T S, Shen X, Zhu K T, Zhang Q F, Wu J L 2009 Acta Phys. Sin. 58 4156 (in Chinese) [张俊艳、邓天松、沈昕、朱孔涛、张琦锋、吴锦雷 2009 物理学报 58 4156]
[7]	Yin Y D, Zhang G T, Xia Y N 2002 Adv. Funct. Mater. 12 293
[8]	Han S, Li C, Liu Z Q, Lei B, Zhang D H, Jin W, Liu X L, Tang T, Zhou C W 2004 Nano Lett. 4 1241
[9]	Kim H W, Shim S H 2006 Chem. Phys. Lett. 422 165
[10]	Nagashima K, Yanagida T, Tanaka H, Kawai T 2007 J. Appl. Phys. 101 124304
[11]	Yanagida T, Nagashima K, Tanaka H, Kawai T 2007 Appl. Phys. Lett. 91 061502
[12]	Kim G, Martens R L, Thompson G B, Kim B C, Gupta A 2007 J. Appl. Phys. 102 104906
[13]	Yang P D, Lieber C M 1997 J. Mater. Res. 12 2981
[14]	Xing H Y, Fan G H, Yang X L, Zhang G Y 2010 Acta Phys. Sin. 59 504 (in Chinese) [刑海英、范广涵、杨学林、张国义 2010 物理学报 59 504]
[15]	Zhang Z, Zhang R, Xie Z L, Liu B, Xiu X Q, Li Y, Fu D Y, Lu H, Chen P, Han P, Zheng Y D, Tang C G, Chen Y H, Wang Z G 2009 Acta Phys. Sin. 58 3416 (in Chinese) [张〖16] Senateur J P, Dubourdieu C, Weiss F, Rosina M, Abrutis A 2000 Adv. Mater. Opt. Electron. 10 155
[16]	Wagner R S, Ellis W C 1964 Appl. Phys. Lett. 4 89
[17]	Hanson M 1958 Constitution of Binary Alloys (New York: McGraw-Hill) p214
[18]	Givargizov E I 1975 J. Cryst. Growth 31 20
[19]	Blakely J M, Jackson K A 1962 J. Chem. Phys. 37 428
[20]	Dubrovskii V G, Cirlin G E, Soshnikov I P, Tokikh A A, Sibirev N V, Samsonenko Y B, Ustinov V M 2005 Phys. Rev. B 71 205325

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