搜索

x

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

双色圆偏振飞秒脉冲驱动CO分子不对称解离

林康 宫晓春 宋其迎 季琴颖 马俊杨 张文斌 陆培芬 曾和平 吴健

引用本文:
Citation:

双色圆偏振飞秒脉冲驱动CO分子不对称解离

林康, 宫晓春, 宋其迎, 季琴颖, 马俊杨, 张文斌, 陆培芬, 曾和平, 吴健

Directional bond breaking of CO molecules by counter-rotating circularly polarized two-color laser fields

Lin Kang, Gong Xiao-Chun, Song Qi-Ying, Ji Qin-Ying, Ma Jun-Yang, Zhang Wen-Bin, Lu Pei-Fen, Zeng He-Ping, Wu Jian
PDF
导出引用
  • 利用反旋圆偏振双色飞秒激光脉冲,结合电子-离子三维动量符合测量,实验研究了CO分子的单电离和双电离解离过程.在激光偏振平面内观测到碳离子C+三叶草状的不对称动量分布.通过调节双色场中基频光和倍频光的相对相位,可以控制C+的出射方向,实现CO分子的二维不对称解离.
    We experimentally studied the dissociative single and double ionization of CO molecules by counter-rotating circularly polarized two-color (CRTC) laser fields. By coincidently measuring the electrons and the fragmented ions, trefoil asymmetric momentum distributions of C+ in the polarization plane were observed, which are mainly determined by the selective ionization of CO with asymmetric orbitals. The threefold pattern could rotate continuously in the two-dimensional space by finely tuning the relative phase of the CRTC fields, providing a new method to manipulate the directional bond breaking of molecules by strong laser fields.
      通信作者: 陆培芬, pflu@lps.ecnu.edu.cn
    • 基金项目: 上海市青年科技英才扬帆计划(批准号:16YF1402900)资助的课题.
      Corresponding author: Lu Pei-Fen, pflu@lps.ecnu.edu.cn
    • Funds: Project supported by the Shanghai Sailing Program, China (Grant No. 16YF1402900).
    [1]

    Zewail A H 1988Science 242 1645

    [2]

    Assion A, Baumert T, Bergt M, Brixner T, Kiefer B, Seyfried V, Strehle M, Gerber G 1998Science 282 919

    [3]

    Shapiro M, Brumer P 2012Quantum Control of Molecular Processes (New York:Wiley-VCH)

    [4]

    Kling M F, Siedschlag C, Verhoef A J, Khan J I, Schultze M, Uphues T, Ni Y, Uiberacker M, Drescher M, Krausz F, Vrakking M J J 2006Science 312 246

    [5]

    Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, Schröter C D, Moshammer R, Ullrich J 2009Phys. Rev. Lett. 103 213003

    [6]

    Fischer B, Kremer M, Pfeifer T, Feuerstein B, Sharma V, Thumm U, Schröter C D, Moshammer R, Ullrich J 2010Phys. Rev. Lett. 105 223001

    [7]

    McKenna J, Anis F, Sayler A M, Gaire B, Johnson N G, Parke E, Carnes K D, Esry B D, Ben-Itzhak I 2012Phys. Rev. A 85 023405

    [8]

    Xu H, Xu T Y, He F, Kielpinski D, Sang R T, Litvinyuk I V 2014Phys. Rev. A 89 041403

    [9]

    Rathje T, Sayler A M, Zeng S, Wustelt P, Figger H, Esry B D, Paulus G G 2013Phys. Rev. Lett. 111 093002

    [10]

    Kling N G, Betsch K J, Zohrabi M, Zeng S, Anis F, Ablikim U, Jochim B, Wang Z, Kbel M, Kling M F, Carnes K D, Esry B D, Ben-Itzhak I 2013Phys. Rev. Lett. 111 163004

    [11]

    Charron E, Giusti-Suzor A, Mies F H 1993Phys. Rev. Lett. 71 692

    [12]

    Ohmura H, Saito N, Tachiya M 2006Phys. Rev. Lett. 96 173001

    [13]

    Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406

    [14]

    Sheehy B, Walker B, DiMauro L F 1995Phys. Rev. Lett. 74 4799

    [15]

    Ray D, He F, De S, Cao W, Mashiko H, Ranitovic P, Singh K P, Znakovskaya I, Thumm U, Paulus G G, Kling M F, Litvinyuk I V, Cocke C L 2009Phys. Rev. Lett. 103 223201

    [16]

    Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002

    [17]

    Kotsina N, Kaziannis S, Danakas S, Kosmidisa C 2013J. Chem. Phys. 139 104313

    [18]

    Kaziannis S, Kotsina N, Kosmidis C 2014J. Chem. Phys. 141 104319

    [19]

    Ohmura H, Saito N 2014J. Phys. B 47 204007

    [20]

    Gong X C, He P L, Song Q Y, Ji Q Y, Pan H F, Ding J X, He F, Zeng H P, Wu J 2014Phys. Rev. Lett. 113 203001

    [21]

    Song Q Y, Gong X C, Ji Q Y, Lin K, Pan H F, Ding J X, Zeng H P, Wu J 2015J. Phys. B 48 094007

    [22]

    Lin K, Gong X C, Song Q Y, Ji Q Y, Zhang W B, Ma J Y, Lu P F, Pan H F, Ding J X, Zeng H P, Wu J 2016J. Phys. B 49 025603

    [23]

    He F, Ruiz C, Becker A 2007Phys. Rev. Lett. 99 083002

    [24]

    He F, Ruiz C, Becker A 2008J. Phys. B 41 081003

    [25]

    Singh K P, He F, Ranitovic P, Cao W, De S, Ray D, Chen S, Thumm U, Becker A, Murnane M M, Kapteyn H C, Litvinyuk I V, Cocke C L 2010Phys. Rev. Lett. 104 023001

    [26]

    Sansone G, Kelkensberg F, Pérez-Torres J F, Morales F, Kling M F, Siu W, Ghafur O, Johnsson P, Swoboda M, Benedetti E, Ferrari F, Lépine F, Sanz-Vicario J L, Zherebtsov S, Znakovskaya I, L'Huillier A, Ivanov M Y, Nisoli M, Martín F, Vrakking M J J 2010Nature 465 763

    [27]

    Wu J, Magrakvelidze M, Schmidt L P H, Kunitski M, Pfeifer T, Schöffler M, Pitzer M, Richter M, Voss S, Sann H, Kim H, Lower J, Jahnke T, Czasch A, Thumm U, Dörner R 2013Nat. Commun. 4 3177

    [28]

    Chaloupka J L, Hickstein D D 2016Phys. Rev. Lett. 116 143005

    [29]

    Mancuso C A, Dorney K M, Hickstein D D, Chaloupka J L, EllisJ L, Dollar F J, Knut R, Grychtol P, Zusin D, Gentry C, Gopalakrishnan M, Kapteyn H C, Murnane M M 2016Phys. Rev. Lett. 117 133201

    [30]

    Eckart S, Richter M, Kunitski M, Hartung A, Rist J, Henrichs K, Schlott N, Kang H, Bauer T, Sann H, Schmidt L Ph H, Schöffler M, Jahnke T, Dörner R 2016Phys. Rev. Lett. 117 133202

    [31]

    Bandrauk A D, Lu H Z 2003Phys. Rev. A 68 043408

    [32]

    Pisanty E, Sukiasyan S, Ivanov M 2014Phys. Rev. A 90 043829

    [33]

    Yuan K J, Bandrauk A D 2015Phys. Rev. A 92 063401

    [34]

    Blaga C I, Xu J, DiChiara A D, Sistrunk E, Zhang K, AgostiniP, Miller T A, DiMauro L F, Lin C D 2012Nature 483 194

    [35]

    Kfir O, Grychtol P, Turgut E, Knut R, Zusin D, Popmintchev D, Popmintchev T, Nembach H, Shaw J M, Fleischer A, Kapteyn H, Murnane M, Cohen O 2015Nat. Photon. 9 99

    [36]

    Chen C, Wu J, Zeng H P 2010Phys. Rev. A 82 033409

    [37]

    Mancuso C A, Hickstein D D, Grychtol P, Knut R, Kfir O, Tong X M, Dollar F, Zusin D, Gopalakrishnan M, Gentry C, Turgut E, Ellis J L, Chen M C, Fleischer A, Cohen O, Kapteyn H C, Murnane M M 2015Phys. Rev. A 91 031402

    [38]

    Baykusheva D, Ahsan M S, Lin N, Wörner H J 2016Phys. Rev. Lett. 116 123001

    [39]

    Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002

    [40]

    Li H, Ray D, De S, Znakovskaya I, Cao W, Laurent G, Wang Z, Kling M F, Le A T, Cocke C L 2011Phys. Rev. A 84 043429

    [41]

    Wu J, Schmidt L Ph H, Kunitski M, Meckel M, Voss S, Sann H, Kim H, Jahnke T, Czasch A, Dörner R 2012Phys. Rev. Lett. 108 183001

    [42]

    Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406

    [43]

    Mashiko H, Gilbertson S, Li C Q, Khan S D, Shakya M M, Moon E, Chang Z 2008Phys. Rev. Lett. 100 103906

    [44]

    Chini M, Mashiko H, Wang H, Chen S, Yun C, Scott S, Gilbertson S, Chang Z 2009Opt. Express 17 21459

    [45]

    Dörner R, Mergel V, Jagutzki O, Spielberger L, Ullrich J, Moshammer R, Schmidt-Böcking H 2000Phys. Rep. 330 95

    [46]

    Ullrich J, Moshammer R, Dorn A, Dörner R, Schmidt L Ph H, Schmidt-Böcking H 2003Rep. Prog. Phys. 66 1463

    [47]

    Guo C 2006Phys. Rev. A. 73 041401

  • [1]

    Zewail A H 1988Science 242 1645

    [2]

    Assion A, Baumert T, Bergt M, Brixner T, Kiefer B, Seyfried V, Strehle M, Gerber G 1998Science 282 919

    [3]

    Shapiro M, Brumer P 2012Quantum Control of Molecular Processes (New York:Wiley-VCH)

    [4]

    Kling M F, Siedschlag C, Verhoef A J, Khan J I, Schultze M, Uphues T, Ni Y, Uiberacker M, Drescher M, Krausz F, Vrakking M J J 2006Science 312 246

    [5]

    Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, Schröter C D, Moshammer R, Ullrich J 2009Phys. Rev. Lett. 103 213003

    [6]

    Fischer B, Kremer M, Pfeifer T, Feuerstein B, Sharma V, Thumm U, Schröter C D, Moshammer R, Ullrich J 2010Phys. Rev. Lett. 105 223001

    [7]

    McKenna J, Anis F, Sayler A M, Gaire B, Johnson N G, Parke E, Carnes K D, Esry B D, Ben-Itzhak I 2012Phys. Rev. A 85 023405

    [8]

    Xu H, Xu T Y, He F, Kielpinski D, Sang R T, Litvinyuk I V 2014Phys. Rev. A 89 041403

    [9]

    Rathje T, Sayler A M, Zeng S, Wustelt P, Figger H, Esry B D, Paulus G G 2013Phys. Rev. Lett. 111 093002

    [10]

    Kling N G, Betsch K J, Zohrabi M, Zeng S, Anis F, Ablikim U, Jochim B, Wang Z, Kbel M, Kling M F, Carnes K D, Esry B D, Ben-Itzhak I 2013Phys. Rev. Lett. 111 163004

    [11]

    Charron E, Giusti-Suzor A, Mies F H 1993Phys. Rev. Lett. 71 692

    [12]

    Ohmura H, Saito N, Tachiya M 2006Phys. Rev. Lett. 96 173001

    [13]

    Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406

    [14]

    Sheehy B, Walker B, DiMauro L F 1995Phys. Rev. Lett. 74 4799

    [15]

    Ray D, He F, De S, Cao W, Mashiko H, Ranitovic P, Singh K P, Znakovskaya I, Thumm U, Paulus G G, Kling M F, Litvinyuk I V, Cocke C L 2009Phys. Rev. Lett. 103 223201

    [16]

    Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002

    [17]

    Kotsina N, Kaziannis S, Danakas S, Kosmidisa C 2013J. Chem. Phys. 139 104313

    [18]

    Kaziannis S, Kotsina N, Kosmidis C 2014J. Chem. Phys. 141 104319

    [19]

    Ohmura H, Saito N 2014J. Phys. B 47 204007

    [20]

    Gong X C, He P L, Song Q Y, Ji Q Y, Pan H F, Ding J X, He F, Zeng H P, Wu J 2014Phys. Rev. Lett. 113 203001

    [21]

    Song Q Y, Gong X C, Ji Q Y, Lin K, Pan H F, Ding J X, Zeng H P, Wu J 2015J. Phys. B 48 094007

    [22]

    Lin K, Gong X C, Song Q Y, Ji Q Y, Zhang W B, Ma J Y, Lu P F, Pan H F, Ding J X, Zeng H P, Wu J 2016J. Phys. B 49 025603

    [23]

    He F, Ruiz C, Becker A 2007Phys. Rev. Lett. 99 083002

    [24]

    He F, Ruiz C, Becker A 2008J. Phys. B 41 081003

    [25]

    Singh K P, He F, Ranitovic P, Cao W, De S, Ray D, Chen S, Thumm U, Becker A, Murnane M M, Kapteyn H C, Litvinyuk I V, Cocke C L 2010Phys. Rev. Lett. 104 023001

    [26]

    Sansone G, Kelkensberg F, Pérez-Torres J F, Morales F, Kling M F, Siu W, Ghafur O, Johnsson P, Swoboda M, Benedetti E, Ferrari F, Lépine F, Sanz-Vicario J L, Zherebtsov S, Znakovskaya I, L'Huillier A, Ivanov M Y, Nisoli M, Martín F, Vrakking M J J 2010Nature 465 763

    [27]

    Wu J, Magrakvelidze M, Schmidt L P H, Kunitski M, Pfeifer T, Schöffler M, Pitzer M, Richter M, Voss S, Sann H, Kim H, Lower J, Jahnke T, Czasch A, Thumm U, Dörner R 2013Nat. Commun. 4 3177

    [28]

    Chaloupka J L, Hickstein D D 2016Phys. Rev. Lett. 116 143005

    [29]

    Mancuso C A, Dorney K M, Hickstein D D, Chaloupka J L, EllisJ L, Dollar F J, Knut R, Grychtol P, Zusin D, Gentry C, Gopalakrishnan M, Kapteyn H C, Murnane M M 2016Phys. Rev. Lett. 117 133201

    [30]

    Eckart S, Richter M, Kunitski M, Hartung A, Rist J, Henrichs K, Schlott N, Kang H, Bauer T, Sann H, Schmidt L Ph H, Schöffler M, Jahnke T, Dörner R 2016Phys. Rev. Lett. 117 133202

    [31]

    Bandrauk A D, Lu H Z 2003Phys. Rev. A 68 043408

    [32]

    Pisanty E, Sukiasyan S, Ivanov M 2014Phys. Rev. A 90 043829

    [33]

    Yuan K J, Bandrauk A D 2015Phys. Rev. A 92 063401

    [34]

    Blaga C I, Xu J, DiChiara A D, Sistrunk E, Zhang K, AgostiniP, Miller T A, DiMauro L F, Lin C D 2012Nature 483 194

    [35]

    Kfir O, Grychtol P, Turgut E, Knut R, Zusin D, Popmintchev D, Popmintchev T, Nembach H, Shaw J M, Fleischer A, Kapteyn H, Murnane M, Cohen O 2015Nat. Photon. 9 99

    [36]

    Chen C, Wu J, Zeng H P 2010Phys. Rev. A 82 033409

    [37]

    Mancuso C A, Hickstein D D, Grychtol P, Knut R, Kfir O, Tong X M, Dollar F, Zusin D, Gopalakrishnan M, Gentry C, Turgut E, Ellis J L, Chen M C, Fleischer A, Cohen O, Kapteyn H C, Murnane M M 2015Phys. Rev. A 91 031402

    [38]

    Baykusheva D, Ahsan M S, Lin N, Wörner H J 2016Phys. Rev. Lett. 116 123001

    [39]

    Betsch K J, Pinkham D W, Jones R R 2010Phys. Rev. Lett. 105 223002

    [40]

    Li H, Ray D, De S, Znakovskaya I, Cao W, Laurent G, Wang Z, Kling M F, Le A T, Cocke C L 2011Phys. Rev. A 84 043429

    [41]

    Wu J, Schmidt L Ph H, Kunitski M, Meckel M, Voss S, Sann H, Kim H, Jahnke T, Czasch A, Dörner R 2012Phys. Rev. Lett. 108 183001

    [42]

    Wu J, Vredenborg A, Schmidt L P H, Jahnke T, Czasch A, Dörner R 2013Phys. Rev. A 87 023406

    [43]

    Mashiko H, Gilbertson S, Li C Q, Khan S D, Shakya M M, Moon E, Chang Z 2008Phys. Rev. Lett. 100 103906

    [44]

    Chini M, Mashiko H, Wang H, Chen S, Yun C, Scott S, Gilbertson S, Chang Z 2009Opt. Express 17 21459

    [45]

    Dörner R, Mergel V, Jagutzki O, Spielberger L, Ullrich J, Moshammer R, Schmidt-Böcking H 2000Phys. Rep. 330 95

    [46]

    Ullrich J, Moshammer R, Dorn A, Dörner R, Schmidt L Ph H, Schmidt-Böcking H 2003Rep. Prog. Phys. 66 1463

    [47]

    Guo C 2006Phys. Rev. A. 73 041401

  • [1] 冯凯源, 邵福球, 蒋祥瑞, 邹德滨, 胡理想, 张国博, 杨晓虎, 银燕, 马燕云, 余同普. 双束对射激光驱动超薄靶的超短脉冲中子源. 物理学报, 2023, 72(18): 185201. doi: 10.7498/aps.72.20230706
    [2] 沈环, 胡春龙, 邓绪兰. 超短脉冲激光场中间二氯苯的激发态动力学. 物理学报, 2017, 66(15): 157801. doi: 10.7498/aps.66.157801
    [3] 夏彦文, 申淼, 孙志红, 彭志涛, 卢宗贵, 周松, 张波, 粟敬钦. 超短激光脉冲波形的单次测量技术. 物理学报, 2017, 66(4): 044204. doi: 10.7498/aps.66.044204
    [4] 白春江, 崔万照, 余金清. 超短超强激光脉冲辐照超薄碳膜电离状态研究. 物理学报, 2016, 65(11): 113201. doi: 10.7498/aps.65.113201
    [5] 刘玉柱, 陈云云, 郑改革, 金峰, Gregor Knopp. 氟利昂F113分子在飞秒激光作用下的多光子电离解离动力学. 物理学报, 2016, 65(5): 053302. doi: 10.7498/aps.65.053302
    [6] 陆莹瑛, 曾志男, 郑颖辉, 邹璞, 刘灿东, 龚成, 李儒新, 徐至展. 双色光场驱动产生单个阿秒脉冲过程中的宏观效应. 物理学报, 2011, 60(10): 103202. doi: 10.7498/aps.60.103202
    [7] 许慎跃, 马新文, 任雪光, T. Pflüger, A. Dorn, J. Ullrich. 甲烷分子电子碰撞电离和解离的实验研究. 物理学报, 2011, 60(9): 093401. doi: 10.7498/aps.60.093401
    [8] 李洪玉, 刘建胜. 超短强激光脉冲激励甲烷团簇的内电离机理. 物理学报, 2010, 59(11): 7850-7856. doi: 10.7498/aps.59.7850
    [9] 苗泉, 赵鹏, 孙玉萍, 刘纪彩, 王传奎. 超短脉冲激光在DBASVP分子中传播时的双光子面积演化和光限幅效应. 物理学报, 2009, 58(8): 5455-5461. doi: 10.7498/aps.58.5455
    [10] 陆剑清, 张向韵, 张诗按, 贾天卿, 孙真荣, 王祖赓. 超短激光脉冲在多能级系统中的传输特性. 物理学报, 2009, 58(12): 8212-8216. doi: 10.7498/aps.58.8212
    [11] 张秋菊, 武慧春, 王兴海, 盛政明, 张 杰. 超短激光脉冲在等离子体中的分裂以及类孤子结构的形成. 物理学报, 2007, 56(12): 7106-7113. doi: 10.7498/aps.56.7106
    [12] 刘运全, 张 杰, 武慧春, 盛政明. 超短电子脉冲在聚焦强激光场中的三维有质动力散射. 物理学报, 2006, 55(3): 1176-1180. doi: 10.7498/aps.55.1176
    [13] 唐荣荣. 超短超强脉冲激光产生的电离通道的存活性态分析. 物理学报, 2006, 55(2): 494-498. doi: 10.7498/aps.55.494
    [14] 王晓峰, 贾天卿, 徐至展. 周期量级超短激光脉冲作用下导带电子的光吸收与碰撞电离. 物理学报, 2005, 54(7): 3451-3456. doi: 10.7498/aps.54.3451
    [15] 陈晓伟, 朱 毅, 刘 军, 冷雨欣, 葛晓春, 李儒新, 徐至展. 飞秒激光脉冲在正色散固体材料中的自压缩. 物理学报, 2005, 54(11): 5178-5183. doi: 10.7498/aps.54.5178
    [16] 华剑飞, 霍裕昆, 林郁正, 陈 钊, 谢永杰, 张绍银, 阎 峥, 徐俊杰. 电子在超短激光脉冲修正场中的动力学特性研究. 物理学报, 2005, 54(2): 653-657. doi: 10.7498/aps.54.653
    [17] 鲁 欣, 奚婷婷, 李英竣, 张 杰. 超短超强脉冲激光在空气中产生的电离通道的寿命研究. 物理学报, 2004, 53(10): 3404-3408. doi: 10.7498/aps.53.3404
    [18] 张秋菊, 盛政明, 张 杰. 周期量级超短激光脉冲在近临界密度等离子体中形成的光孤子. 物理学报, 2004, 53(3): 798-802. doi: 10.7498/aps.53.798
    [19] 王迎松, 徐至展. 初始位相对超短脉冲强激光场高次谐波辐射的影响. 物理学报, 1999, 48(6): 1023-1029. doi: 10.7498/aps.48.1023
    [20] 陈荣清, 徐至展, 孙岚, 姚关华, 张文琦, 李萍. 激光方脉冲作用下强场自电离过程. 物理学报, 1991, 40(10): 1584-1589. doi: 10.7498/aps.40.1584
计量
  • 文章访问数:  5238
  • PDF下载量:  321
  • 被引次数: 0
出版历程
  • 收稿日期:  2016-09-26
  • 修回日期:  2016-11-04
  • 刊出日期:  2016-11-05

/

返回文章
返回