Magneto-electronic properties and manipulation effects of Fe-adsorbed Sb/WS<sub>2</sub> heterostructure

He Xin; Li Xin-Yan; Li Jing-Hui; Zhang Zhen-Hua

doi:10.7498/aps.71.20220949

Abstract

To study the induced magnetism mechanism and magneto-electronic properties of non-magnetic two-dimensional van der Waals heterostructure adsorbing magnetic atoms, we construct Sb/WS₂ heterostructure, and consider its adsorbed Fe atoms. The calculated adsorption energy shows that T_W, V_Sb adsorption are the most likely positions for Fe atom adsorbed below and above the heterostructure, respectively, and T_{S_M} adsorption is the most likely position for Fe atom adsorbed between two monolayers. The induced magnetism is due to the electron-spin rearrangement caused by the expansion of valence electronic configuration (VEC) and charge transfer after Fe atoms have been adsorbed. The T_W adsorption and the T_{S_M} adsorption make the nonmagnetic semiconducting heterostructure become a half-semiconductor (HSC), while V_Sb adsorption turns the heterostructure into a bipolar magnetic semiconductor (BMS). In particular, the calculated magnetized energy indicates that the interlayer T_{S_M} adsorption leads the heterostructure to holding the highest magnetic stability, which is enough to resist the influence of thermal fluctuation at room temperature. Quantum manipulation can cause the heterostructure to produce abundant magnetism, especially the flexible change of magnetic phase. For example, the application of external electric field can give rise to the magnetic phase transition among HSC, HM (half-metal) and BMS for the heterostructure, and the vertical strain can make the heterostructure realize the magnetic phase transition among HSC, HM and MM (magnetic metal). This study shows that the heterostructure can increase the adsorption region of transition metal atoms (below, interlayer and above), so as to produce rich magnetism, especially for the interlayer adsorption of transition metals, its magnetic stability against temperature is significantly enhanced.

Keywords:

two-dimensional van der Waals heterostructure /
magneto-electronic property /
magnetic stability /
quantum manipulation /
magnetic phase transition

Authors and contacts

Hunan Provincial Key Laboratory of Flexible Electronic Materials Genome Engineering, Changsha University of Science and Technology, Changsha 410114, China

Corresponding author: Zhang Zhen-Hua, zhzhang@csust.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 61771076), the Natural Science Foundation of Hunan Province, China (Grant No. 2020JJ4625), and the Scientific Research Fund of Education Department of Hunan Province, China (Grant No. 19A029).

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References

[1]	Geim A K, Grigorieva I V 2013 Nature 499 419 Google Scholar
[2]	Li X M, Tao L, Chen Z F, Fang H, Li X S, Wang X R, Xu J B, Zhu H W 2017 Appl. Phys. Rev. 4 021306 Google Scholar
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Cited By

图 1 (a)—(d) 优化之后Sb/WS₂异质结的四种堆垛方式的主视图和侧视图; (e) 优化后不同异质结的层间距与结合能; (f) 异质结单胞对应的布里渊区

Figure 1. (a)–(d) Top and side views of the four stacking patterns of optimized Sb/WS₂ heterostructures; (e) the binding energy and interlayer distance of the optimized heterostructures; (f) Brillouin zone corresponding to heterostructure unit-cell.

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图 2 PBE计算的(a) Sb单层、(b) WS₂单层和(c) Sb/WS₂异质结的能带结构; HSE06计算的(d) Sb单层、(e) WS₂单层和(f) Sb/WS₂异质结的能带结构

Figure 2. Band structures by PBE calculation: (a) Sb monolayer; (b) WS₂ monolayer; (c) Sb/WS₂ heterostructure. The band structures by HSE06 calculation: (d) Sb monolayer; (e) WS₂ monolayer; (f) Sb/WS₂ heterostructure.

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图 3 过渡金属原子Fe吸附于Sb/WS₂异质结的四个高对称位置　(a) 底层WS₂下方; (b) 两单层层间; (c)上层Sb上方

Figure 3. Four highly symmetrical adsorbed sites of Fe atom for Sb/WS₂ heterostructure: (a) Bellow the bottom WS₂ monolayer; (b) between two monolayers; (c) above the top Sb monolayer.

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图 4 FM态自旋极化密度分布, 对应的吸附方式分别为(a) T_W, (b) T_{S_m}, (c) V_Sb. 等值面取为0.002 e/A³

Figure 4. Spin-polarized density (magnetic distribution) in the FM state, and corresponding adsorbed manners are: (a) T_W; (b) T_{S_m}; (c) V_Sb. The isosurface is set as 0.002 e/A³.

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图 5 对应最稳三种吸附位置的异质结能带结构、态密度以及投影态密度　(a)—(c) 能带结构; (d)—(f) 态密度和投影态密度

Figure 5. Band structure, density of states and projected density of states of the heterostructures corresponding to three most stable adsorption sites: (a)–(c) Band structure; (d)–(f) density of states and projected density of states.

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图 6 (a) 外加电场示意图; (b) 电场能、带隙值及磁性随加电场变化; (c)—(j) E_ext = –0.1, –0.3, –0.7, –1, 0.2, 0.5, 0.8 和1.0 V/Å时的能带结构, 其中图(d)中绿色区域代表该阴影部分的能带放大图

Figure 6. (a) Schematic diagram of applied external electric field on heterostructure. (b) Electric field energy, band gap, and magnetic phase versus the external electric field. (c)–(j) The band structures for E_ext = –0.1, –0.3, –0.7, –1, 0.2, 0.5, 0.8, and 1.0 V/Å, where the green region in panel (d) represents the enlarged partial band structure.

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图 7 (a)施加的拉力与压力示意图; (b) 应变能、带隙及磁相随应变变化; (c)—(f) ε = –0.3, 0.2, 0.35 和 0.4 Å时的能带结构, 其中图(e)与图(f)中绿色区域代表该部分的能带放大图

Figure 7. (a) Schematic diagram of stretching and compressing heterostructure; (b) the strain energy, band gap and magnetic phase as versus strain; (c)–(f) band structure at ε = –0.3, 0.2, 0.35, and 0.4 Å, where the green region in panel (e) and (f) represent the enlarged partial band structure.

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表 1 磁矩、TM原子电子构型、电荷转移和磁化能. μ₀ 为孤立Fe原子的磁矩, μ为Fe原子吸附后磁矩, 括号中M为超元胞磁矩. VEC 为孤立Fe原子价电子构型(valence electron configuration), VEC^*为Fe原子吸附后价电子构型. ΔQ为吸附之后Fe原子所转移的电荷, “–”代表 Fe原子失去电荷. E_M为磁化能

Table 1. Magnetic moment, electron configuration of TM atom, charge transfer and magnetization energy. μ₀ is the magnetic moment of isolated Fe atoms, μ is the magnetic moment after adsorption of Fe atoms, M in parentheses is the magnetic moment of the supercell. VEC is the valence electron configuration of isolated Fe atoms, and VEC* is the valence electron configuration of Fe atoms after adsorption. ΔQ is the charge transferred by Fe atom after adsorption, where “–” means that the Fe atom loses its charge. E_M is the magnetization energy.

Adsorbed site	μ₀/μ_B	μ/μ_B (M/μ_B)	VEC	VEC^*	ΔQ/\|e\|	E_M/meV
T_W	4	2.002 (2.023)	3d/4s 6/2	3d/4s/4p 6.923/0.354/0.304	–0.423	75.3
T_{S_m}	4	2.002 (2.290)	3d/4s 6/2	3d/4s/4p 7.011/0.568/0.304	–0.119	146.46
V_Sb	4	2.004 (2.313)	3d/4s 6/2	3d/4s/4p 7.030/0.577/0.330	–0.065	10.02

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[1]	Geim A K, Grigorieva I V 2013 Nature 499 419 Google Scholar
[2]	Li X M, Tao L, Chen Z F, Fang H, Li X S, Wang X R, Xu J B, Zhu H W 2017 Appl. Phys. Rev. 4 021306 Google Scholar
[3]	Novoselov K S, Mishchenko A, Carvalho A, Neto A H C 2016 Science 353 aac9439 Google Scholar
[4]	Shang J M, Pan L F, Wang X T, Li J B, Deng H X, Wei Z M 2018 J. Mater. Chem. C 6 7201 Google Scholar
[5]	Idrees M, Fawad M, Bilal M, Saeed Y, Nguyen C, Amin B 2020 RSC Adv. 10 25801 Google Scholar
[6]	Ozcelik V O, Azadani J G, Yang C, Koester S J, Low T 2016 Phys. Rev. B 94 035125 Google Scholar
[7]	Liu C H, Clark G, Fryett T, Wu S F, Zheng J J, Hatami F, Xu X D, Majumdar A 2017 Nano Lett. 17 200 Google Scholar
[8]	Binder J, Withers F, Molas M R, Faugeras C, Nogajewski K, Watanabe K, Taniguchi T, Kozikov A, Geim A K, Novoselov K S, Potemski M 2017 Nano Lett. 17 1425 Google Scholar
[9]	He X, Deng X Q, Sun L, Zhang Z H, Fan Z Q 2022 Appl. Surf. Sci. 578 151844 Google Scholar
[10]	Huang L, Huo N J, Li Y, Chen H, Yang J H, Wei Z M, Li J B, Li S S 2015 J. Phys. Chem. Lett. 6 2483 Google Scholar
[11]	Xiao W Z, Xu L, Rong Q Y, Dai X Y, Cheng C P, Wang L L 2020 Appl. Surf. Sci. 504 144425 Google Scholar
[12]	Huang L, Li Y, Wei Z M, Li J B 2015 Sci. Rep. 5 16448 Google Scholar
[13]	Lei C G, Ma Y D, Xu X L, Zhang T, Huang B B, Dai Y 2019 J. Phys. Chem. C 123 23089 Google Scholar
[14]	Yan R S, Fathipour S, Han Y M, Song B, Xiao S D, Li M D, Ma N, Protasenko V, Muller D A, Jena D, Xing H G 2015 Nano Lett. 15 5791 Google Scholar
[15]	Shim J, Oh S, Kang D H, Jo S H, Ali M H, Choi W Y, Heo K, Jeon J, Lee S, Kim M, Song Y J, Park J H 2016 Nat. Commun. 7 13413 Google Scholar
[16]	Xia C X, Du J, Li M, Li X P, Zhao X, Wang T X, Li J B 2018 Phy. Rev. A 10 054064 Google Scholar
[17]	Wu Y B, Huang Z Y, Liu H T, He C Y, Xue L, Qi X, Zhong J X 2018 Phys. Chem. Chem. Phys. 20 17387 Google Scholar
[18]	Bian H, Duan H, Li J, Chen F, Cao B, Long M 2019 AIP Adv. 9 065207 Google Scholar
[19]	Kundu S, Naik M H, Jain M 2020 Phy. Rev. Mater. 4 054004 Google Scholar
[20]	Luo M, Xu Y E, Song Y X 2018 J. Supercond. Novel Magn. 31 449 Google Scholar
[21]	Ding Y M, Shi J J, Zhang M, Zhu Y H, Wu M, Wang H, Cen Y L, Guo W H, Pan S H 2018 Physica E 101 245 Google Scholar
[22]	Chen HL, Han J N, Deng X Q, Fan Z Q, Sun L, Zhang Z H 2022 Appl. Surf. Sci. 598 153756 Google Scholar
[23]	Han J N, Zhang Z H, Fan Z Q, Zhou R L 2020 Nanotechnology 31 315206 Google Scholar
[24]	Hu R, Wang D, Fan Z Q, Zhang Z H 2018 Phys. Chem. Chem. Phys. 20 13574 Google Scholar
[25]	Chen H L, Zhang L, Deng X Q, Sun L, Zhang Z H, Fan Z Q 2021 J. Mater. Chem. C 9 12904 Google Scholar
[26]	Zhao T, Fan Z Q, Zhang Z H, Zhou R L 2019 J. Phys. D: Appl. Phys. 52 475301 Google Scholar
[27]	Hu R, Li Y H, Zhang Z H, Fan Z Q, Sun L 2019 J. Mater. Chem. C 7 7745 Google Scholar
[28]	Dong Q X, Hu R, Fan Z Q, Zhang Z H 2018 Carbon 130 206 Google Scholar
[29]	Hu J K, Zhang Z H, Fan Z Q, Zhou R L 2019 Nanotechnology 30 485703 Google Scholar
[30]	Han J N, He X, Fan Z Q, Zhang Z H 2019 Phys. Chem. Chem. Phys. 21 1830 Google Scholar
[31]	Grimme S 2006 J. Comput. Chem. 27 1787 Google Scholar
[32]	Yang Y Y, Gong P, Ma W D, Hao R, Fang X Y 2021 Chin. Phys. B 30 067803 Google Scholar
[33]	Jia Y H, Gong P, Li S L, Ma W D, Fang X Y, Yang Y Y 2020 Phys. Lett. A 384 126106 Google Scholar
[34]	吴甜, 姚梦丽, 龙孟秋 2021 物理学报 70 056301 Google Scholar Wu T, Yao M L, Long M Q 2021 Acta Phys. Sin. 70 056301 Google Scholar
[35]	Gong P, Yang Y Y, Ma W D, Fang X Y, Jing X L, Jia Y H, Cao M S 2021 Physica E 128 114578 Google Scholar
[36]	Xie Z J, Zhang B, Ge Y Q, Zhu Y, Nie G H, Song Y F, Lim C K, Zhang H, Prasad P N 2021 Chem. Rev. 122 1127 Google Scholar
[37]	He X, Fan Z Q, Zhang Z H 2020 Phys. Chem. Chem. Phys. 22 23665 Google Scholar

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Magneto-electronic properties and manipulation effects of Fe-adsorbed Sb/WS₂ heterostructure

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Corresponding author: Zhang Zhen-Hua, zhzhang@csust.edu.cn

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Magneto-electronic properties and manipulation effects of Fe-adsorbed Sb/WS2 heterostructure

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Corresponding author: Zhang Zhen-Hua, zhzhang@csust.edu.cn

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Magneto-electronic properties and manipulation effects of Fe-adsorbed Sb/WS₂ heterostructure