搜索

x

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

机载多轴差分吸收光谱技术获取对流层NO2垂直柱浓度的研究

徐晋 谢品华 司福祺 李昂 刘文清

引用本文:
Citation:

机载多轴差分吸收光谱技术获取对流层NO2垂直柱浓度的研究

徐晋, 谢品华, 司福祺, 李昂, 刘文清

Determination of tropospheric NO2 by airborne multi axis differential optical absorption spectroscopy

Xu Jin, Xie Pin-Hua, Si Fu-Qi, Li Ang, Liu Wen-Qing
PDF
导出引用
  • 介绍了一种基于机载平台获取对流层NO2垂直柱浓度的多轴差分吸收光谱技术. 研究了利用差分吸收光谱技术结合不同观测角度的测量光谱反演差分斜柱浓度, 并利用辐射传输模型SCIATRAN计算对流层NO2垂直柱浓度的方法. 研究了不同海拔高度、不同地面反照率以及不同太阳天顶角等条件对天顶和天底两个观测角度的大气质量因子的影响. 报道了该系统在2008年12月10日在珠三角地区的实验结果, 结合天顶和天底两个方向反演得到了珠三角地区对流层NO2垂直柱浓度的分布信息. 同时还将机载测量结果跟安装在珠海市的一台地基多轴差分吸收光谱仪的结果进行了对比, 二者相差仅为8%. 实验结果表明, 机载多轴DOAS技术可以实现对大区域对流层NO2浓度的快速获取.
    The airborne multi axis differential optical absorption spectroscopy (AMAXDOAS) is employed to retrieve tropospheric vertical columns of NO2. The differential slant columns of NO2 are retrieved combined with the spectra in different viewing directions by the DOAS method and the vertical columns are calculated with the radiative transfer model SCIATRAN. The dependences of AMF on altitude, surface albedo, and solar zenith angle are studied. The measurement campaign in pearl region delta region on December 10 in 2008 is reported. The NO2 vertical column distribution is obtained in zenith and nadir directions. The results from airborne multi axis DOAS are compared with those from a ground-based multi axis DOAS in Zhuhai, with a deviation of 0.08. The results show that AMAXDOAS can be used to measure the tropospheric NO2 in a large area within a short time.
    • 基金项目: 国家自然科学基金(批准号: 40805015, 40905010)和国家高技术研究发展计划(863)项目(批准号: 2006AA06A303)资助的课题.
    • Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 40805015, 40905010), and the National High Technology Research and Development Program of China (863 Program) (Grant No. 2006AA06A303).
    [1]

    Zhou B, Liu W Q, Qi F, Li Z B, Chui Y J 2001, Acta phys. sin. 50 1818 [周斌, 刘文清, 齐峰, 李振壁, 崔延军 2001 物理学报 50 1818]

    [2]

    Si F Q, Liu J G, Xie P H 2006 Acta phys. Sin. 55 3165 [司福祺, 刘建国, 谢品华 2006 物理学报 55 3165]

    [3]

    Pfeilsticker K, Platt U 1994 Geophysical Research Letters 21 1375

    [4]

    McElroy C T, McLinden C A, McConnell J C 1999 Nature 397 338

    [5]

    Melamed M L, Solomon S, Daniel J S, Langford A O, Portmann R W, Ryerson T B, Nicks D K, Jr, McKeen S A 2003, J. Environ. Monit 5 29

    [6]

    Wang P, Richter A, Bruns M, Rozanov V V, Burrows J P, Heue K P, Wagner T, Pundt I, Platt U 2005 Atmos. Chem. Phys. 5 337

    [7]

    Heue K P, Richter A, Bruns M, Burrows J P, Friedeburg C V, Platt U, Pundt I, Wang P, Wagner T 2005 Atmos. Chem. Phys. 5 1039

    [8]

    Bruns M, Buehler S A, Burrows J P, Richter A, Rozanov A, Wang P, Heue K P, Platt U, Pundt I,Wagner T 2006 Atmos. Chem. Phys. 6 3049

    [9]

    Wang P, Richter A, Bruns M, Burrows J P, Scheele R, Junkermann W, Heue K P,Wagner T, Platt U, Pundt I 2006 Atmos. Chem. Phys. 6 329

    [10]

    Rozanov A, Rozanov V, Burrows J P 2001 J. Quant. Spectrosc. Radiat. Transfer 69 491

    [11]

    Burrows, J P, Dehn A, Deters B, Himmelmann S, Richter A, Voigt S, Orphal J, 1998 Journal of Quantitative Spectroscopy and Radiative Transfer 60 1025

    [12]

    Burrow J P, Dehn A, Deters B, Himmelmann S, Richter A, Voigt S, Orphal J, 1999 Journal of Quantitative Spectroscopy and Radiative Transfer 61 509

    [13]

    Greenblatt G D, Orlando J J, Burkholder J B, Ravishankara A R 1990 J. Geophys. Res. 95 18577

    [14]

    Grainger J F, Ring J 1962 Nature 193 762

    [15]

    Fayt, C, Van Roozendael M 2001 WinDOAS 2.1 software User Manual

    [16]

    Feister U, Grewe R 1995 Photochem. Photobiol 62 736

    [17]

    Payne, Richard E 1972 Journal of Atmospheric Sciences 29 959

  • [1]

    Zhou B, Liu W Q, Qi F, Li Z B, Chui Y J 2001, Acta phys. sin. 50 1818 [周斌, 刘文清, 齐峰, 李振壁, 崔延军 2001 物理学报 50 1818]

    [2]

    Si F Q, Liu J G, Xie P H 2006 Acta phys. Sin. 55 3165 [司福祺, 刘建国, 谢品华 2006 物理学报 55 3165]

    [3]

    Pfeilsticker K, Platt U 1994 Geophysical Research Letters 21 1375

    [4]

    McElroy C T, McLinden C A, McConnell J C 1999 Nature 397 338

    [5]

    Melamed M L, Solomon S, Daniel J S, Langford A O, Portmann R W, Ryerson T B, Nicks D K, Jr, McKeen S A 2003, J. Environ. Monit 5 29

    [6]

    Wang P, Richter A, Bruns M, Rozanov V V, Burrows J P, Heue K P, Wagner T, Pundt I, Platt U 2005 Atmos. Chem. Phys. 5 337

    [7]

    Heue K P, Richter A, Bruns M, Burrows J P, Friedeburg C V, Platt U, Pundt I, Wang P, Wagner T 2005 Atmos. Chem. Phys. 5 1039

    [8]

    Bruns M, Buehler S A, Burrows J P, Richter A, Rozanov A, Wang P, Heue K P, Platt U, Pundt I,Wagner T 2006 Atmos. Chem. Phys. 6 3049

    [9]

    Wang P, Richter A, Bruns M, Burrows J P, Scheele R, Junkermann W, Heue K P,Wagner T, Platt U, Pundt I 2006 Atmos. Chem. Phys. 6 329

    [10]

    Rozanov A, Rozanov V, Burrows J P 2001 J. Quant. Spectrosc. Radiat. Transfer 69 491

    [11]

    Burrows, J P, Dehn A, Deters B, Himmelmann S, Richter A, Voigt S, Orphal J, 1998 Journal of Quantitative Spectroscopy and Radiative Transfer 60 1025

    [12]

    Burrow J P, Dehn A, Deters B, Himmelmann S, Richter A, Voigt S, Orphal J, 1999 Journal of Quantitative Spectroscopy and Radiative Transfer 61 509

    [13]

    Greenblatt G D, Orlando J J, Burkholder J B, Ravishankara A R 1990 J. Geophys. Res. 95 18577

    [14]

    Grainger J F, Ring J 1962 Nature 193 762

    [15]

    Fayt, C, Van Roozendael M 2001 WinDOAS 2.1 software User Manual

    [16]

    Feister U, Grewe R 1995 Photochem. Photobiol 62 736

    [17]

    Payne, Richard E 1972 Journal of Atmospheric Sciences 29 959

计量
  • 文章访问数:  5886
  • PDF下载量:  473
  • 被引次数: 0
出版历程
  • 收稿日期:  2011-03-03
  • 修回日期:  2011-05-04
  • 刊出日期:  2012-01-05

/

返回文章
返回