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Black carbon aerosols affect the shortwave and longwave radiation in climate in a strong yet uncertain way. In aging process, black carbon particles coated by co-emitted aerosols tend to reduce the shortwave radiative forcing of freshly emitted black carbon at the top of atmosphere (TOA), however, this effect is still unclear in the longwave range. Here in this work, we investigate the effect of black carbon aging on longwave radiative forcing. The freshly emitted black carbon aerosols are simulated to be fractal aggregates consisting of hundreds of small spherical primary particles, and these aggregated black carbon aerosols tend to be fully coated by the large sulfate particles after aging. The optical properties of these freshly emitted and internally mixed black carbon aerosols are simulated using the numerically exact superposition T-matrix method, and their longwave radiative forcings are calculated by the radiative transfer equation solver. The results indicate that the black carbon longwave radiative forcing at TOA is remarkably amplified (up to 3) by coating the large sulfate particles, while the black carbon shortwave radiative forcings decrease during their aging. Moreover, the thicker sulfate coatings tend to increase the longwave radiative forcings of black carbon aerosols at TOA. These findings should improve our understanding of the effect of black carbon aging on their longwave radiative forcings and provide guidance for assessing the climate change.
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Keywords:
- aerosol /
- black carbon /
- longwave radiative forcing /
- absorption of particles
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-
[1] Jacobson M Z 2001 Nature 409 695
[2] Bellouin N, Boucher O, Haywood J, Reddy M S 2005 Nature 438 1138
[3] Shindell D, Faluvegi G 2009 Nature Geosci. 2 294
[4] Ramanathan V, Carmichael G 2008 Nature Geosci. 1 221
[5] Bond T C, Doherty S J, Fahey D W, Forster P M, Berntsen T, Boucher O, DeAngelo B J, Flanner M G, Ghan S, Krcher B, Koch D, Kinne S, Kondo Y, Quinn P K, Sarofim M C, Schultz M G, Schulz M, Venkataraman C, Zhang H, Zhang S, Bellouin N, Guttikunda S K, Hopke P K, Jacobson M Z, Kaiser J W, Klimont Z, Lohmann U, Schwarz J P, Shindell D, Storelvmo T, Warren S G, Zender C S 2013 J. Geophys. Res.:Atmos. 118 5380
[6] Adachi K, Buseck P R 2008 Atmos. Chem. Phys. 8 6469
[7] China S, Mazzoleni C, Gorkowski K, Aiken A C, Dubey M K 2013 Nat. Commun. 4 2122
[8] McFiggans G, Artaxo P, Baltensperger U, Coe H, Facchini M C, Feingold G, Fuzzi S, Gysel M, Laaksonen A, Lohmann U, Mentel T F, Murphy D M, O'Dowd C D, Snider J R, Weingartner E 2006 Atmos. Chem. Phys. 6 2593
[9] Zhou Y, Savijrvi H 2014 Atmos. Res. 135 102
[10] Ramana, M V, Ramanathan V, Feng Y, Yoon S C, Kim S W, Carmichael G R, Schauer J J 2010 Nature Geosci. 3 542
[11] Kahnert M, Nousiainen T, Lindqvist H, Ebert M 2012 Opt. Express 20 10042
[12] Cappa C D, Onasch T B, Massoli P, Worsnop D R, Bates T S, Cross E S, Davidovits P, Hakala J, Hayden K L, Jobson B T, Kolesar K R, Lack D A, Lerner B M, Li S M, Mellon D, Nuaaman I, Olfert J S, Petj T, Quinn P K, Song C, Subramanian R, Williams E J, Zaveri R A 2012 Science 337 1078
[13] Jacobson M Z 2013 Science 339 393
[14] Cappa C D, Onasch T B, Massoli P, Worsnop D R, Bates T S, Cross E S, Davidovits P, Hakala J, Hayden K L, Jobson B T, Kolesar K R, Lack D A, Lerner B M, Li S M, Mellon D, Nuaaman I, Olfert J S, Petj T, Quinn P K, Song C, Subramanian R, Williams E J, Zaveri R A 2013 Science 339 393
[15] Stocker T F, Qin D, Plattner G K, Tignor M, Allen S K, Boschung J, Nauels A, Xia Y, Bex V, Midgley P M 2013 Climate Change 2013:The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change (Cambridge:Cambridge University Press) p573
[16] Widmann J F, Yang J C, Smith T J, Manzello S L, Mulholland G W 2003 Combust. Flame 134 119
[17] Kahnert M 2010 Atmos. Chem. Phys. 10 8319
[18] Prasanna S, Rivire P H, Soufiani A 2014 J. Quant. Spectrosc. Radiat. Transfer 148 141
[19] Smith A J A, Peters D M, McPheat R, Lukanihins S, Grainger R G 2015 J. Geophys. Res.:Atmos. 120 9670
[20] Heinson W R, Chakrabarty R K 2016 Opt. Lett. 41 808
[21] Mikhailov E F, Vlasenko S S, Podgorny I A, Ramanathan V, Corrigan C E 2006 J. Geophy. Res.:Atmos. 111 D7
[22] Zhang R, Khalizov A F, Pagels J, Zhang D, Xue H, McMurry P H 2008 Proc. Natl. Acad. Sci. 105 10291
[23] Khalizov A F, Xue H, Wang L, Zheng J, Zhang R 2009 J. Phys. Chem. A 113 1066
[24] Bueno P A, Havey D K, Mulholland G W, Hodges J T, Gillis K A, Dickerson R R, Zachariah M R 2011 Aerosol. Sci. Tech. 45 1217
[25] Mishchenko M I, Dlugach J M 2012 Opt. Lett. 37 704
[26] Cheng T, Gu X, Wu Y, Chen H 2014 J. Quant. Spectrosc. Radiat. Transfer 147 196
[27] Wu Y, Cheng T, Zheng L, Chen H, Xu H 2015 J. Quant. Spectrosc. Radiat. Transfer 157 1
[28] Fierce L, Bond T C, Bauer S E, Mena F, Riemer N 2016 Nat. Commun. 7 1
[29] You R, Radney J G, Zachariah M R, Zangmeister C D 2016 Environ. Sci. Technol. 50 7982
[30] Schwarz J P, Gao R S, Spackman J R, Watts L A, Thomson D S, Fahey D W, Ryerson T B, Peischl J, Holloway J S, Trainer M, Frost G J, Baynard T, Lack D A, Gouw J A de, Warneke C, Del Negro L A 2008 Geophys. Res. Lett. 35 L13810
[31] Lack D A, Moosmller H, McMeeking G R, Chakrabarty R K, Baumgardner D 2014 Anal. Bioanal. Chem. 406 99
[32] Chakrabarty R K, Beres N D, Moosmller H, China S, Mazzoleni C, Dubey M K, Liu L, Mishchenko M I 2014 Sci. Rep. 4 1
[33] Li W, Shao L, Zhang D, Ro C, Hu M, Bi X, Geng H, Matsuki A, Niu H, Chen J 2016 J. Clean. Prod. 112 1330
[34] Liu L, Mishchenko M I, Arnott W P 2008 J. Quant. Spectrosc. Radiat. Transfer 109 2656
[35] Wu Y, Cheng T, Gu X, Zheng L, Chen H, Xu H 2014 J. Quant. Spectrosc. Radiat. Transfer 135 9
[36] Hentschel H G E 1984 Phys. Rev. Lett. 52 212
[37] Cheng T, Wu Y, Gu X, Chen H 2015 Opt. Express 23 10808
[38] Bond T C, Bergstrom R W 2006 Aerosol. Sci. Tech. 40 27
[39] John W, Wall S M, Ondo J L, Winklmayr W 1990 Atmos. Environ. Part A. General Topics 24 2349
[40] Chang H, Charalampopoulos T T 1990 Procee. Roy. Soc. Lon. Ser. A:Math. Phys. Sci. 430 577
[41] Toon O B, Pollack J B, Khare B N 1976 J. Geophys. Res. 81 5733
[42] Mackowski D W, Mishchenko M I 2011 J. Quant. Spectrosc. Radiat. Transfer 112 2182
[43] Mishchenko M I, Liu L, Mackowski D W 2013 J. Quant. Spectrosc. Radiat. Transfer 123 135
[44] Mackowski D W 2014 J. Quant. Spectrosc. Radiat. Transfer 133 264
[45] Buras R, Dowling T, Emde C 2011 J. Quant. Spectrosc. Radiat. Transfer 112 2028
[46] Mayer B, Kylling A 2005 Atmos. Chem. Phys. 5 1855
[47] Gasteiger J, Emde C, Mayer B, Buras R, Buehler S A, Lemke O 2014 J. Quant. Spectrosc. Radiat. Transfer 148 99
[48] Kahnert M, Nousiainen T, Lindqvist H 2013 Opt. Express 21 7974
[49] Wu Y, Cheng T, Zheng L, Chen H 2016 J. Quant. Spectrosc. Radiat. Transfer 179 139
[50] Cheng T, Wu Y, Chen H 2014 Opt. Express 22 15904
[51] Wu Y, Cheng T, Zheng L 2016 J. Quant. Spectrosc. Radiat. Transfer 182 1
[52] Wu Y, Cheng T, Zheng L, Chen H 2015 Aerosol. Sci. Tech. 49 941
[53] Lubin D, Satheesh S K, McFarquar G, Heymsfield A J 2007 J. Geophys. Res.:Atmos. 107 1
[54] Kahnert M, Devasthale A 2011 Atmos. Chem. Phys. 11 11745
[55] Adachi K, Chung S H 2010 J. Geophys. Res.:Atmos. 115 D15206
[56] Wu Y, Cheng T, Zheng L, Chen H 2016 Sci. Rep. 6 38592
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