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由绝缘体间隔的两个导体间的层间拖拽效应是研究准粒子耦合和探索层间关联物态的重要途径,而具有丰富可调物性的二维层状材料为研究拖拽效应提供了更多可能。本文制备了石墨烯-氮化硼-二硒化铌这一电双层结构,系统研究了二维半金属和二维超导体之间的拖拽效应。当石墨烯作为驱动层,二硒化铌作为被动层时,可以在二硒化铌超导转变温度区间发现显著的拖拽响应,表现出明显的超流拖拽特征;而当二硒化铌处于正常金属态时,拖拽信号消失。磁场、栅压调制下的测试进一步表明,拖拽响应与二硒化铌的超导转变直接相关,且其符号不依赖石墨烯载流子类型。更为重要的是,通过对比不同器件发现,这类超流拖拽响应仅出现在空气中解理的薄层二硒化铌中,因此二硒化铌中超导的不均匀性是产生该效应的关键。其机制可能源自非均匀超导体中量子涨落与二维半金属电荷密度波动之间的库伦耦合。In an electronic double-layer system composed of two spatially adjacent yet electrically insulated conductors, when a current flows through one conductor (drive layer), its charge carriers transfer energy/momentum to those in the other conductor (drag layer) via interlayer Coulomb coupling. This generates a measurable voltage or current in the drag layer, a phenomenon known as interlayer drag effect. This effect serves as a critical approach for studying quasiparticle interactions and investigating interlayer-correlated quantum states. Two-dimensional layered materials with highly tunable properties provide new opportunities for exploring the drag effect. In this study, we fabricate an electronic double-layer structure consisting of graphene and NbSe2 to systematically investigate the drag effect between a two-dimensional semimetal and a two-dimensional superconductor, wherein a thin hBN layer serves as the insulating spacer. When graphene acts as the drive layer and NbSe2 acts as the drag layer, a pronounced positive drag response is observed within the superconducting transition temperature range of NbSe2. In contrast, the drag signal vanishes when NbSe2 is in its normal metallic state. Magnetic field dependence measurements reveal that the drag response disappears under high fields where the superconductivity of NbSe2 is suppressed, further confirming its direct correlation with the superconducting transition. Gate-voltage modulation experiments reveal that the drag response peaks when tuning the Fermi level of graphene across the Dirac point. This is attributed to the reduced screening of interlayer interactions due to the ultra-low carrier concentration at this point. Notably, the sign of the supercurrent drag does not depend on the carrier type in graphene, ruling out the conventional momentum-transfer drag mechanism. Our results collectively demonstrate the realization of supercurrent drag effect, which has been attributed to Coulomb coupling between the quantum fluctuations of the superconducting phases in a superconductor and the charge densities in a normal conductor in previous study. Notably, comparative studies across devices show that supercurrent drag responses occur only in thin NbSe2 layers cleaved in air. No significant signals are detected in either thick NbSe2 layers or thin layers cleaved under argon protection. These results establish the importance of superconducting inhomogeneity in NbSe2 for generating supercurrent drag effect, suggesting that drag measurements could also serve as a novel probe for investigating superconducting properties. Further investigation into the polarity and intensity of supercurrent drag signals may advance our understanding of inhomogeneous superconductivity, as well as interactions between normal carriers and Cooper pairs.
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Keywords:
- two-dimensional materials /
- supercurrent drag effect /
- superconducting inhomogeneity /
- quantum fluctuations
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