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大气压低温等离子体在生物医学、环境保护、纳米制造等领域有广泛的应用，而这些应用中的核心理化过程通常是等离子体与水溶液的相互作用。等离子体与水溶液的相互作用非常复杂，既包含种类繁多的气液两相反应，也包含相互耦合的粒子传质过程，使得现有的实验技术难以系统地阐释内在机制，仿真研究至关重要。近10余年来，国内外对等离子体与水溶液相互作用的仿真研究取得了重要进展，基本解决了传质与反应参数缺乏的问题，从无到有建立了多种类型的仿真模型，并积极探索基于人工智能的新型仿真方法，显著提升了对该领域的认知水平。本文将从参数获取、模型构建到智能算法3个方面综述近年来的仿真研究进展，以期为国内同行和研究生提供参考。Atmospheric-pressure low-temperature plasma has been widely applied in various fields such as biomedicine, environmental protection, and nanomanufacturing, whereas key physicochemical processes in these applications involve the interactions between plasma and aqueous solutions. However, such plasma–liquid interactions are highly complex, encompassing a wide variety of gas– liquid phase reactions as well as coupled mass transfer processes. These intricate mechanisms make it difficult for existing experimental techniques to provide a systematic understanding, highlighting the critical role of simulation studies. Over the past decade, significant progress has been made both domestically and internationally in the simulation of plasma–solution interactions. Researchers have basically addressed the scarcity of data on transport and reaction parameters, established multiple types of simulation models, and are actively exploring new simulation approaches based on intelligence algorithm. These advances have greatly deepened our understanding of this field. Thus, this paper reviews recent developments in simulation studies of plasma–solution interactions from three perspectives, namely parameter acquisition, model construction, and intelligent algorithms, with the aim of providing useful insights for domestic researchers and graduate students.
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Keywords:
- Plasma treatment of aqueous solution /
- Basic parameter /
- Simulation models /
- Intelligence algorithm
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