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铁硒基超导研究新进展:高质量(Li,Fe)OHFeSe单晶薄膜

董晓莉 袁洁 黄裕龙 冯中沛 倪顺利 田金朋 周放 金魁 赵忠贤

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铁硒基超导研究新进展:高质量(Li,Fe)OHFeSe单晶薄膜

董晓莉, 袁洁, 黄裕龙, 冯中沛, 倪顺利, 田金朋, 周放, 金魁, 赵忠贤

New progress on FeSe-based superconductors: high-quality and high-critical-parameter (Li, Fe)OHFeSe thin film

Dong Xiao-Li, Yuan Jie, Huang Yu-Long, Feng Zhong-Pei, Ni Shun-Li, Tian Jin-Peng, Zhou Fang, Jin Kui, Zhao Zhong-Xian
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  • 单晶薄膜形态的高温超导材料对于相关基础科学研究和应用开发都极为重要.多带的铁基高温超导体往往呈现丰富的物理现象,并具有较高的超导临界参数.特别是近年发现的插层(Li,Fe)OHFeSe超导体,无论对高温超导机理还是应用研究而言,都日益受到重视,已成为铁基家族中重要的典型材料.但是,该化合物含有OH键,加热易分解.因此,现有的常规高温成膜技术均不适用于生长该薄膜材料.为解决这一生长难题,我们最近发明了基体辅助水热外延生长法,实现了超导薄膜制备技术上的突破.本文简要介绍用此软化学成膜技术首次成功制备出(Li,Fe)OHFeSe单晶薄膜.该薄膜材料具有优良的结晶质量和较高的超导临界参数,特别是其高的临界电流密度和上临界场对应用开发有实际价值.因此,(Li,Fe)OHFeSe超导单晶薄膜的成功合成,为机理研究和应用开发分别提供了重要的实验载体和备选材料.另外,该薄膜技术也有望应用于其他功能材料的探索与合成,尤其是对常规手段难以获取的材料更具重大价值.
    High-quality superconducting thin films play an important role in the application and basic research of high-Tc superconductivity. In these aspects, iron-based superconductors feature the merits of rich physical phenomena and high superconducting critical parameters (including the transition temperature Tc, the upper critical field Hc2 and the critical current density Jc). The recently discovered high-Tc (Li,Fe)OHFeSe superconductor proves to be an important material for the studies of the mechanism and application of unconventional high-Tc superconductivity. However, due to the hydroxyl ion inherent in the compound, none of the conventional high-temperature synthesis methods is applicable for (Li,Fe)OHFeSe materials in bulk and thin film forms. Recently, by developing a hydrothermal ion-exchange technique, we have synthesized for the first time big and high-quality single crystals of (Li,Fe)OHFeSe (2015 Phys. Rev. B 92 064515). Here in this paper, we brief our most recent progress on growing a high-quality single-crystalline superconducting film of (Li,Fe)OHFeSe (2017 Chin. Phys. Lett. 34 077404). The film has been prepared on a LaAlO3 substrate by a hydrothermal epitaxial method. The high crystalline quality of the film is verified by X-ray diffraction (XRD). The XRD measurements show a single (001) orientation with a small crystal mosaic of 0.22 in terms of the full width at half maximum of the rocking curve, as well as an excellent in-plane orientation revealed by the -scan of (101) plane. Its bulk superconducting transition temperature Tc of 42.4 K is determined by both zero electrical resistance and diamagnetism measurements. Based on systematic magnetoresistance measurements, the upper critical field Hc2 is estimated to be 79.5 T and 443 T for the magnetic field perpendicular and parallel to the ab plane, respectively. Moreover, a large critical current density Jc of a value over 0.5 MA/cm2 is achieved at ~20 K. Such a (Li,Fe)OHFeSe film therefore is not only important for the fundamental research for understanding the high-Tc mechanism, but also promising for the applications in high-performance electronic devices and large scientific facilities such as superconducting accelerator.
      Corresponding author: Dong Xiao-Li, dong@iphy.ac.cn;kuijin@iphy.ac.cn;zhxzhao@iphy.ac.cn ; Jin Kui, dong@iphy.ac.cn;kuijin@iphy.ac.cn;zhxzhao@iphy.ac.cn ; Zhao Zhong-Xian, dong@iphy.ac.cn;kuijin@iphy.ac.cn;zhxzhao@iphy.ac.cn
    • Funds: Project supported by the National Key RD Program of China (Grant No. 2017YFA0303000), the National Natural Science Foundation of China (Grant No. 11574370), the Key Research Program of Frontier Sciences, Chinese Academy of Sciences (Grant Nos. QYZDY-SSW-SLH001, QYZDY-SSW-SLH008), and the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No. XDB07020100).
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    Khasanov R, Zhou H, Amato A, Guguchia Z, Morenzoni E, Dong X, Zhang G, Zhao Z 2016 Phys. Rev. B 93 224512

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    Zhou X, Borg C K H, Lynn J W, Saha S R, Paglione J, Rodriguez E E 2016 J. Mater. Chem. C 4 3934

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    Ma M, Wang L, Bourges P, Sidis Y, Danilkin S, Li Y 2017 Phys. Rev. B 95 100504

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    Pan B, Shen Y, Hu D, Feng Y, Park J T, Christianson A D, Wang Q, Hao Y, Wo H, Yin Z, Maier T A, Zhao J 2017 Nat. Commun. 8 123

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    Wang Z, Yuan J, Wosnitza J, Zhou H, Huang Y, Jin K, Zhou F, Dong X, Zhao Z 2017 J. Phys.:Condens. Matter 29 025701

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    Sun J P, Shahi P, Zhou H X, Huang Y L, Chen K Y, Wang B S, Ni S L, Li N N, Zhang K, Yang W G, Uwatoko Y, Xing G, Sun J, Singh D J, Jin K, Zhou F, Zhang G M, Dong X L, Zhao Z X, Cheng J G 2018 Nat. Commun. 9 380

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  • [1]

    Johnston D C 2010 Adv. Phys. 59 803

    [2]

    Paglione J, Greene R L 2010 Nat. Phys. 6 645

    [3]

    Stewart G R 2011 Rev. Mod. Phys. 83 1589

    [4]

    Dagotto E 2013 Rev. Mod. Phys. 85 849

    [5]

    Chen X, Dai P, Feng D, Xiang T, Zhang F C 2014 Nat. Sci. Rev. 1 371

    [6]

    Putti M, Pallecchi I, Bellingeri E, Cimberle M R, Tropeano M, Ferdeghini C, Palenzona A, Tarantini C, Yamamoto A, Jiang J, Jaroszynski J, Kametani F, Abraimov D, Polyanskii A, Weiss J D, Hellstrom E E, Gurevich A, Larbalestier D C, Jin R, Sales B C, Sefat A S, McGuire M A, Mandrus D, Cheng P, Jia Y, Wen H H, Lee S, Eom C B 2010 Supercond. Sci. Technol. 23 034003

    [7]

    Hosono H, Tanabe K, Takayama-Muromachi E, Kageyama H, Yamanaka S, Kumakura H, Nohara M, Hiramatsu H, Fujitsu S 2015 Sci. Technol. Adv. Mater. 16 033503

    [8]

    Dong X, Zhou H, Yang H, Yuan J, Jin K, Zhou F, Yuan D, Wei L, Li J, Wang X, Zhang G, Zhao Z 2015 J. Am. Chem. Soc. 137 66

    [9]

    Hsu F C, Luo J Y, Yeh K W, Chen T K, Huang T W, Wu P M, Lee Y C, Huang Y L, Chu Y Y, Yan D C, Wu M K 2008 Proc. Natl. Acad. Sci. USA 105 14262

    [10]

    Guo J, Jin S, Wang G, Wang S, Zhu K, Zhou T, He M, Chen X 2010 Phys. Rev. B 82 180520R

    [11]

    Fang M H, Wang H D, Dong C H, Li Z J, Feng C M, Chen J, Yuan H Q 2011 Europhys. Lett. 94 27009

    [12]

    Medvedev S, McQueen T M, Troyan I A, Palasyuk T, Eremets M I, Cava R J, Naghavi S, Casper F, Ksenofontov V, Wortmann G, Felser C 2009 Nat. Mater. 8 630

    [13]

    Sun J P, Matsuura K, Ye G Z, Mizukami Y, Shimozawa M, Matsubayashi K, Yamashita M, Watashige T, Kasahara S, Matsuda Y, Yan J Q, Sales B C, Uwatoko Y, Cheng J G, Shibauchi T 2016 Nat. Commun. 7 12146

    [14]

    Lei B, Cui J H, Xiang Z J, Shang C, Wang N Z, Ye G J, Luo X G, Wu T, Sun Z, Chen X H 2016 Phys. Rev. Lett. 116 077002

    [15]

    Wang Q Y, Li Z, Zhang W H, Zhang Z C, Zhang J S, Li W, Ding H, Ou Y B, Deng P, Chang K, Wen J, Song C L, He K, Jia J F, Ji S H, Wang Y Y, Wang L L, Chen X, Ma X C, Xue Q K 2012 Chin. Phys. Lett. 29 037402

    [16]

    Liu D, Zhang W, Mou D, He J, Ou Y B, Wang Q Y, Li Z, Wang L, Zhao L, He S, Peng Y, Liu X, Chen C, Yu L, Liu G, Dong X, Zhang J, Chen C, Xu Z, Hu J, Chen X, Ma X, Xue Q, Zhou X J 2012 Nat. Commun. 3 931

    [17]

    Tan S Y, Zhang Y, Xia M, Ye Z R, Chen F, Xie X, Peng R, Xu D F, Fan Q, Xu H C, Jiang J, Zhang T, Lai X C, Xiang T, Hu J P, Xie B P, Feng D L 2013 Nat. Mater. 12 634

    [18]

    Lee J J, Schmitt F T, Moore R G, Johnston S, Cui Y T, Li W, Yi M, Liu Z K, Hashimoto M, Zhang Y, Lu D H, Devereaux T P, Lee D H, Shen Z X 2014 Nature 515 245

    [19]

    Shi X, Han Z Q, Peng X L, Richard P, Qian T, Wu X X, Qiu M W, Wang S C, Hu J P, Sun Y J, Ding H 2017 Nat. Commun. 8 14988

    [20]

    Lu X F, Wang N Z, Wu H, Wu Y P, Zhao D, Zeng X Z, Luo X G, Wu T, Bao W, Zhang G H, Huang F Q, Huang Q Z, Chen X H 2014 Nat. Mater. 14 325

    [21]

    Dong X, Jin K, Yuan D, Zhou H, Yuan J, Huang Y, Hua W, Sun J, Zheng P, Hu W, Mao Y, Ma M, Zhang G, Zhou F, Zhao Z 2015 Phys. Rev. B 92 064515

    [22]

    Du Z, Yang X, Lin H, Fang D, Du G, Xing J, Yang H, Zhu X, Wen H H 2016 Nat. Commun. 7 10565

    [23]

    Niu X H, Peng R, Xu H C, Yan Y J, Jiang J, Xu D F, Yu T L, Song Q, Huang Z C, Wang Y X, Xie B P, Lu X F, Wang N Z, Chen X H, Sun Z, Feng D L 2015 Phys. Rev. B 92 060504

    [24]

    Zhao L, Liang A, Yuan D, Hu Y, Liu D, Huang J, He S, Shen B, Xu Y, Liu X, Yu L, Liu G, Zhou H, Huang Y, Dong X, Zhou F, Liu K, Lu Z, Zhao Z, Chen C, Xu Z, Zhou X J 2016 Nat. Commun. 7 10608

    [25]

    Khasanov R, Zhou H, Amato A, Guguchia Z, Morenzoni E, Dong X, Zhang G, Zhao Z 2016 Phys. Rev. B 93 224512

    [26]

    Zhou X, Borg C K H, Lynn J W, Saha S R, Paglione J, Rodriguez E E 2016 J. Mater. Chem. C 4 3934

    [27]

    Ma M, Wang L, Bourges P, Sidis Y, Danilkin S, Li Y 2017 Phys. Rev. B 95 100504

    [28]

    Pan B, Shen Y, Hu D, Feng Y, Park J T, Christianson A D, Wang Q, Hao Y, Wo H, Yin Z, Maier T A, Zhao J 2017 Nat. Commun. 8 123

    [29]

    Wang Z, Yuan J, Wosnitza J, Zhou H, Huang Y, Jin K, Zhou F, Dong X, Zhao Z 2017 J. Phys.:Condens. Matter 29 025701

    [30]

    Sun J P, Shahi P, Zhou H X, Huang Y L, Chen K Y, Wang B S, Ni S L, Li N N, Zhang K, Yang W G, Uwatoko Y, Xing G, Sun J, Singh D J, Jin K, Zhou F, Zhang G M, Dong X L, Zhao Z X, Cheng J G 2018 Nat. Commun. 9 380

    [31]

    Huang Y, Feng Z, Ni S, Li J, Hu W, Liu S, Mao Y, Zhou H, Zhou F, Jin K, Wang H, Yuan J, Dong X, Zhao Z 2017 Chin. Phys. Lett. 34 077404

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出版历程
  • 收稿日期:  2018-04-22
  • 修回日期:  2018-05-04
  • 刊出日期:  2019-06-20

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