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通过852 nm波长连续激光和509 nm波长纳秒脉冲激光级联激发,采用室温铯原子气室实现了铯里德伯原子电磁诱导透明(EIT)光谱。509 nm波长纳秒激光脉冲功率~176 W,脉冲重复频率在300 kHz-100 MHz范围连续可调,脉宽在1-100 ns范围连续可调。实验研究了里德伯EIT光谱与509nm波长纳秒脉冲激光参数的关系。时域周期脉冲光在频域上等效为相干频率梳,通过光脉冲参数调节实现了可控速度群铯原子的里德伯态激发。基于纳秒光脉冲激发的里德伯原子EIT光谱具有高信噪比,在量子传感和量子模拟领域有潜在的应用价值。By cascaded excitation using an 852-nm continuous-wave laser and a 509-nm nanosecond pulsed laser, the electromagnetically-induced transparency (EIT) spectroscopic signals of ladder type three-level cesium atoms with Rydberg state have been achieved using a room-temperature cesium vapor cell. The 509-nm pulsed laser beam’s power is ~176 W, while the pulse repetition frequency ranges from 300 kHz to 100 MHz and can be continuously adjusted. The laser pulse duration ranges from 1 to 100 ns and can be continuously adjusted. The relationship between Rydberg EIT spectroscopic signals and 509-nm nanosecond pulsed laser parameters have been experimentally investigated. By changing the pulse repetition frequency and the pulse duration of the 509-nm nanosecond pulsed laser, the comb-like Rydberg atomic spectroscopy has been achieved using a room-temperature cesium vapor cell. Under certain repetition frequency and pulse duration ranges, the envelope of the spectral lines shows a regular pattern, the spacing between the transmission peaks is consistent with the pulse repetition frequency, and atomic with the specific velocity group can be excited to Rydberg state by changing the values of the 509-nm laser pulse repetition frequency and pulse duration. Theoretically, the center peak frequency can be tuned to within ±100 MHz of the velocity group atoms' excitation in Rydberg state for the pulsed laser parameters.
Compared with finite velocity group pumping of cesium atoms by a continuous-wave laser, decreasing the repetition frequency of the 509-nm pulsed coupling laser can further increase the number of atoms in Rydberg state. When the repetition frequency of the 509-nm pulsed laser approaches the EIT linewidth, the number of cesium Rydberg atoms can be increased by up to 10 times. During the parameter optimization process, the dynamic characteristics of pulsed excitation in multi-level atoms, as well as the interaction characteristics between arbitrarily shaped laser pulses and multi-level atomic systems, should be considered. Pulsed laser pumping enables the interaction between the laser field, and a specific velocity group of atoms and the atomic frequency comb spectroscopy developed from it can be used for electric and magnetic field measurements. The multi-peak structure of the spectrum can be used to more accurately determine the intensity, frequency, and phase of the microwave electric field by measuring spectral variations. This high-sensitivity and high-resolution measurement capability is crucial for the precise measurement of microwave electric fields. The pulse coupling laser can excite atoms in a specific velocity group to the Rydberg state. High-density Rydberg atoms can improve the signal-to-noise ratio of the measured spectrum, which has potential application in quantum sensing and quantum measurement based on Rydberg atoms.-
Keywords:
- Rydberg atoms /
- Nanosecond pulse laser excitation /
- Electromagnetically induced transparency spectroscopy /
- Velocity selection spectroscopy
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