Optimization strategies for energy storage properties of polyvinylidene fluoride composites

Zha Jun-Wei; Zha Lei-Jun; Zheng Ming-Sheng

doi:10.7498/aps.72.20222012

Abstract

Dielectric capacitors have been widely used in crucial energy storage systems of electronic power systems because of their advantages such as fast charge discharge rates, long cycle lifetimes, low losses, and flexible and convenient processingc. However, the dielectric capacitors have lower energy storage densities than electrochemical energy storage devices, which makes them difficult to meet higher application requirements for electrical engineering at the present stage. Polyvinylidene fluoride (PVDF) based polymers show great potential in achieving improved energy storage properties, which is attributed to their high dielectric constants and high breakdown strengths. This work systematically reviews PVDF-based nanocomposites for energy storage applications. Dielectric constant, breakdown strength and charge discharge efficiency are three main parameters related to energy storage properties, which are proposed to discuss their mechanisms of action and optimization strategies. Finally, the key scientific problems of PVDF-based high energy storage composites are summarized and considered, and the future development trend of dielectric capacitors is also prospected.

Keywords:

Authors and contacts

1.
School of Chemistry and Biological Engineering, University of Science and Technology Beijing, Beijing 100083, China
2.
Beijing Advanced Innovation Center for Materials Genome Engineering, University of Science and Technology Beijing, Beijing 100083, China

Corresponding author: Zha Jun-Wei, zhajw@ustb.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 51977114).

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References

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Cited By

图 1 介质电容器的应用

Figure 1. Application of Dielectric Capacitors.

DownLoad: Full-Size Img PowerPoint

图 2 D-E曲线示意图^[14]

Figure 2. Schematic illustration of electric displacement (D)-electric field (E) loop ^[14].

DownLoad: Full-Size Img PowerPoint

图 3 不同铁电结构电介质及其D-E曲线^[16]

Figure 3. Dielectrics with different ferroelectric structures and their D-E curves^16].

DownLoad: Full-Size Img PowerPoint

图 4 沿c轴观察的PVDF四种相的单胞^[28]

Figure 4. Unit cells of four PVDF phases observed along the c-axis^28].

DownLoad: Full-Size Img PowerPoint

图 5 (a) NH₂-GNDs/RGO/PVDF三元复合物制备流程; (b)不同PVDF基复合材料介电常数^[43]

Figure 5. (a) NH₂-GNDs/RGO/PVDF ternary complex preparation process; (b) different PVDF-based composite dielectric constants^[43].

DownLoad: Full-Size Img PowerPoint

图 6 (a) PDA表面改性减少漏电流示意图^[50]; (b)不同小分子改性剂改性后击穿强度^[52]

Figure 6. (a) schematic diagram of PDA surface modification to reduce leakage current ^[50]; (b) breakdown strength after modification with different small molecule modifiers ^[52].

DownLoad: Full-Size Img PowerPoint

图 7 (a) BTO@TO纳米纤维及其与聚合物复合材料示意图与元素图; (b) PVDF基复合材料能量密度; (c)P(VDF-HFP)基复合材料能量密度^[55,56]

Figure 7. (a) schematic and elemental diagrams of BTO@TO nanofibers and their composites with polymers; (b) energy density of PVDF-based composites; (c)energy density of P(VDF-HFP)-based composites ^[55,56].

DownLoad: Full-Size Img PowerPoint

图 8 复合材料阻挡效应模型示意图

Figure 8. Schematic diagram of barrier effect model of composite material

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图 9 (a) PVDF/ P(VDF-TrFE-CFE)共混膜的储能密度与充放电效率^[69]; (b)不同钛酸锶钡含量下单层膜与3层膜介电损耗; (c) TNF介电损耗降低示意图^[76]

Figure 9. (a) Energy storage density and charge/discharge efficiency of PVDF/ P(VDF-TrFE-CFE) blended films^[69]; (b) dielectric loss of monolayer and trilayer films with different barium strontium titanate content; (c) schematic diagram of TNF dielectric loss reduction ^[76]

DownLoad: Full-Size Img PowerPoint

[1]	Yu M P, Wang A J, Tian F Y, Song H Q, Wang Y S, Li C, Hong J D, Shi G Q 2015 Nanoscale 7 5292 Google Scholar
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[13]	Dang Z M, Yuan J K, Yao S H, Liao R J 2013 Adv. Mater. 25 6334 Google Scholar
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[15]	Diao C L, Liu H X, Lou G H, Zheng H W, Yao Z H, Hao H, Cao M H 2019 J. Alloys Compd. 781 378 Google Scholar
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[24]	Chen X Z, Li X Y, Qian X S, Lu S G, Gu H M, Lin M, Shen Q D, Zhang Q M 2013 Polymer 54 2373 Google Scholar
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[30]	Lovinger A J 1983 Science 220 1115 Google Scholar
[31]	Huang X Y, Sun B, Zhu Y K, Li S T, Jiang P K 2019 Prog. Mater. Sci. 100 187 Google Scholar
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[59]	Feng Y F, Wu Q, Deng Q H, Peng C, Hu J B, Xu Z C 2019 J. Mater. Chem. C 7 6744 Google Scholar
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[66]	Bharti V, Zhang Q M 2001 Phys. Rev. B 63 184103 Google Scholar
[67]	Li Z M, Arbatti M D, Cheng Z Y 2004 Macromolecules 37 79 Google Scholar
[68]	Wu S, Lin M, Lu S G, Zhu L, Zhang Q M 2011 Appl. Phys. Lett. 99 132901 Google Scholar
[69]	Zhang X, Shen Y, Shen Z H, Jiang J Y, Chen L Q, Nan C W 2016 ACS Appl. Mater. Interfaces 8 27236 Google Scholar
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