压-电-化学耦合增强策略及机理研究进展

贾艳敏; 王晓星; 张祺昌; 武峥

doi:10.7498/aps.72.20222078

摘要

压电材料能够收集环境中存在的微小的机械能, 具有将机械信号转换为电信号的强大能力. 利用压电材料的压电效应与电化学氧化还原效应二者的耦合可以实现压-电-化学耦合. 近年来, 压-电-化学耦合在收集清洁能源和处理废水保护环境方面受到国内外研究人员的广泛关注. 本文综述了增强压-电-化学耦合的策略, 从构建异质结、负载贵金属、构筑相界、混合碳或石墨烯和调控缺陷方面出发进行了总结梳理. 从电子的运输和转移、材料相变和氧空位的角度解释不同策略中的物理机理, 并对研究前景进行了展望.

关键词:

Abstract

Piezoelectric materials can harvest tiny mechanical energy existing in the environment, and have strong ability to convert mechanical signals into electrical signals. Piezo-electro-chemical coupling can be realized via combining piezoelectric effect of piezoelectric materials with electrochemical redox effect. In recent years, piezo-electro-chemical coupling has attracted a lot of attention from researchers in harvesting vibration energy to treat dye wastewater. The piezoelectric catalyst material dispersed in solution is deformed by ultrasonic vibrations. Owing to the piezoelectric effect and spontaneous polarization effects, positive and negative charges are generated at both ends of the catalyst, which can further react with dissolved oxygen and hydroxide ions in the solution to generate superoxide and hydroxyl radicals (·${}{\rm{O}}_2^- $ and ·OH) for decomposing organic dyes. However, ordinary piezoelectric catalytic materials are often difficult to meet people's pursuit of efficient treatment of organic dyes. Researchers have conducted a lot of researches on piezo-electro-chemical coupling, mainly focusing on the following two aspects: 1) the modification of piezoelectric catalysts to achieve extended carrier lifetime, accelerate carrier separation and high piezoelectric coefficients, and 2) the combination of piezo-electro-chemical coupling with photocatalysis to suppress photogenerated carrier compounding to obtain high synergistic catalytic performance. In this work, the following five strategies to enhance the piezo-electro-chemical coupling via modifying piezoelectric catalyst materials are introduced. The heterojunction structure is constructed to promote the separation of electron-hole pairs. The precious metal is coated on the surface of the catalyst to accelerate the transport and transfer of electrons. The catalyst composition is regulated and controlled to obtain an increased piezoelectric coefficient at the phase boundary. Carbon or graphene are mixed in the catalyst to accelerate the electron transfer on the surface of piezoelectric material. The number of active sites increases through introducing defects into the catalyst to increase the concentration of carriers. The physical mechanisms of five different strategies are described from the perspectives of electron transport and transfer, phase transition, and oxygen vacancies. In addition, the prospects for piezo-electro-chemical coupling in energy and biomedical applications such as hydrogen production, carbon dioxide reduction, tumor therapy and tooth whitening are presented.

Keywords:

作者及机构信息

1.
西安邮电大学理学院, 西安　710121

2.
西安工程大学环境与化学工程学院, 西安　710048

通信作者: 贾艳敏, jiayanmin@xupt.edu.cn ; 武峥, wuzheng@xpu.edu.cn

基金项目: 国家自然科学基金(批准号: 22179108)资助的课题.

Authors and contacts

1.
School of Science, Xi’an University of Posts and Telecommunications, Xi’an 710121, China

2.
School of Environmental and Chemical Engineering, Xi’an Polytechnic University, Xi’an, 710048, China

Corresponding author: Jia Yan-Min, jiayanmin@xupt.edu.cn ; Wu Zheng, wuzheng@xpu.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 22179108).

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参考文献

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施引文献

图 1 增强压-电-化学耦合5种策略, 异质结、贵金属负载、相界、缺陷、混合碳或石墨烯

Fig. 1. Five strategies to enhance piezo-electro-chemical coupling, including heterojunction, coating precious metal, phase boundary, defects, mixing carbon or graphene.

下载: 全尺寸图片幻灯片

图 2 BTO/CN异质结压-电-化学耦合的机理图^[39]

Fig. 2. Mechanism diagram for the piezo-electro-chemical coupling of BTO/CN heterostructures ^[39].

下载: 全尺寸图片幻灯片

图 3 异质结材料不同含量助剂对染料的降解率的影响　(a) CoO_x/BiFeO₃异质结^[38]; (b) BTO/CN异质结^[39]

Fig. 3. Effect of different content of cocatalyst in heterojunction materials on dye decomposition ratio: (a) CoO_x/BiFeO₃ heterostructure^[38]; (b) BTO/CN heterostructure^[39].

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图 4 Ag负载的BTO压-电-化学耦合的机理图^[44]

Fig. 4. Mechanism diagram for the piezo-electro-chemical coupling of Ag-coated BTO^[44].

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图 5 不同Ag含量的BTO-Ag降解RhB染料的反应速率常数k值对比^[44]

Fig. 5. Comparison of reaction rate constant k of RhB dye decomposition by BTO-Ag with different Ag content^[44].

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图 6 通过调控组分, 构建两相共存区^[48]

Fig. 6. Schematic diagram of constructing two-phase coexistence zone through regulating components^[48].

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图 7 不同Sr含量的Ba_1–xSr_xTiO₃ 降解MO染料^[55]

Fig. 7. Decomposition of MO dye by Ba_1–xSr_xTiO₃ with different Sr content^[55].

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图 8 不同C含量对BaTiO₃降解RhB染料的影响^[56]

Fig. 8. Effects of RhB dye decomposition by BaTiO₃ with different C content^[56].

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图 9 BaTiO₃/C的压-电-化学耦合示意图^[56]

Fig. 9. Mechanism diagram for the piezo-electro-chemical coupling of BaTiO₃/C^[56].

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图 10 Graphene/BiVO₄的压-电-化学耦合示意图^[60]

Fig. 10. Mechanism diagram for the piezo-electro-chemical coupling of graphene/BiVO₄^[60].

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图 11 CNC 在热处理前后对RhB染料的降解率^[66]

Fig. 11. Decomposition ratio of RhB dye by CNC before and after heat treatment^[66]

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表 1 不同策略对有机染料降解结果汇总

Table 1. Summary of decomposition results of organic dyes via different strategies.

策略	复合材料	助剂	增强前的降解率D 或反应速率常数k	增强后的降解率D 或反应速率常数k
构建异质结	CoO_x/BiFeO₃	CoO(光沉积时间为3 h)	D = 50.76%	D = 81.2% ^[38]
构建异质结	BaTiO₃/g-C₃N₄	g-C₃N₄(质量分数为15%)	D = 57%	D = 82% ^[39]
负载贵金属	BaTiO₃-Ag	Ag(质量分数为2.09%)	D = 15%	D = 84% ^[44]
负载贵金属	Ag/PbBiO₂I	Ag(质量分数为0.2%)	k = 0.0024 min^–1	k = 0.0165 min^–1^[45]
构筑相界	(1–x)Na_0.5K_0.5NbO₃-xLiNbO₃	Li (x = 0.006)	D = 53%	D = 91% ^[48]
	(1–x)(Pb_0.9625Sm_0.025) (Mg_1/3Nb_2/3)O₃-xPbTiO₃	PbTiO₃(x = 0.29)		k = 0.0453 min^–1^[49]
	Ba_1–xSr_xTiO₃	Sr(x = 0.20)	k = 0.005 min^–1	k = 0.025 min^–1^[51]
	0.96(K_0.48Na_0.52)Nb_0.955Sb_0.045O₃-0.04(Bi_0.5Na_0.5)ZrO₃	0.04(Bi_0.5Na_0.5)ZrO₃	k = 0.043 min^–1	k = 0.091 min^–1^[73]
	0.82 Ba(Ti_0.89Sn_0.11)O₃-0.18(Ba_0.7Ca_0.3)TiO₃	0.18(Ba_0.7Ca_0.3)TiO₃	k = 0.0706 min^–1	k = 0.0094 min^–1^[74]
混合碳	BaTiO₃/C	C(质量分数为2%)	D = 48.4%	D = 75.5% ^[56]
混合石墨烯	BaTiO₃@Graphene	Graphene(质量比为2∶1)	k = 0.002 min^–1	k = 0.028 min^–1^[59]
混合石墨烯	Graphene/BiVO₄	Graphene(质量分数为2%)	D = 19%	D = 81% ^[60]
调控缺陷	BaTiO_3–x		k = 0.0084 min^–1	k = 0.0101 min^–1^[67]
	C₃N_5–x-O		D = 73.5%	D = 99%^[68]
	CNC		D = 34.58%	D = 96.65% ^[66]

下载: 导出CSV

[1]	Dai X Q, Chen L, Li Z Y, Li X, Wang J F, Hu X, Zhao L H, Jia Y M, Sun S X, Wu Y, He Y M 2021 J. Colloid Interface Sci. 603 220 Google Scholar
[2]	Zhang W H, Wang X J, Zhang Y C, Bochove B, Mäkilä E, Seppälä J, Xu W Y, Willför S, Xu C L 2020 Sep. Purif. Technol. 242 116523 Google Scholar
[3]	Oliveira L V, Bennici S, Josien L, Limousy L, Bizeto M A, Camilo F F 2020 Carbohydr. Polym. 230 115621 Google Scholar
[4]	Wang S S, Wu Z, Chen J, Ma J P, Ying J S, Cui S C, Yu S G, Hu Y M, Zhao J H, Jia Y M 2019 Ceram. Int. 45 11703 Google Scholar
[5]	Muraro P C L, Mortari S R, Vizzotto B S, Chuy G, Dos Santos C, Brum L F W, da Silva W L 2020 Sci. Rep. 10 1 Google Scholar
[6]	Roy J S, Dugas G, Morency S, Messaddeq Y 2020 Physica E:Low Dimens. Syst. Nanostruct. 120 114114 Google Scholar
[7]	Van Tran C, La D D, Hoai P N T, Ninh H D, Hong P N T, Vu T H T, Nadda A K, Nguyen X C, Nguyen D D, Ngo H H 2021 J. Hazard. Mater. 420 126636 Google Scholar
[8]	李冬冬, 王丽莉 2012 物理学报 61 034212 Google Scholar Li D D, Wang L L 2012 Acta Phys. Sin. 61 034212 Google Scholar
[9]	Wu W, Yin X, Dai B Y, Kou J H, Ni Y, Lu C H 2020 Appl. Surf. Sci. 517 146119 Google Scholar
[10]	Lei H, Zhang H H, Zou Y, Dong X P, Jia Y M, Wang F F 2019 J. Alloys Compd. 809 151840 Google Scholar
[11]	佟建波, 黄茜, 张晓丹, 张存善, 赵颖 2012 物理学报 61 047801 Google Scholar Tong J B, Huang Q, Zhang X D, Zhang C S, Zhao Y 2012 Acta Phys. Sin. 61 047801 Google Scholar
[12]	Moghaddas S, Elahi B, Javanbakht V, 2020 J. Alloys Compd. 821 153519 Google Scholar
[13]	赵娟, 胡慧芳, 曾亚萍, 程彩萍 2013 物理学报 62 158104 Google Scholar Zhao J, Hu H F, Zeng Y P, Cheng C P 2013 Acta Phys. Sin. 62 158104 Google Scholar
[14]	Cha B J, Woo T G, Han S W, Saqlain S, Seo H O, Cho H K, Jee Y K, Kim Y D 2018 Catalysts 8 500 Google Scholar
[15]	Ni M, Leung M, Leung D, Sumathy K 2007 Renew. Sust. Energ. Rev. 11 401 Google Scholar
[16]	Xu X L, Xiao L B, Jia Y M, Hong Y T, Ma J P, Wu Z 2018 J. Electron. Mater. 47 536 Google Scholar
[17]	Ma J P, Chen L, Wu Z, Chen J, Jia Y M, Hu Y M 2019 Ceram. Int. 45 11934 Google Scholar
[18]	Yu D F, Liu Z H, Zhang J M, Li S, Zhao Z C, Zhu L F, Liu W S, Lin Y H, Liu H, Zhang Z T 2019 Nano Energy 58 695 Google Scholar
[19]	Ma J P, Wu Z, Luo W S, Zheng Y Q, Jia Y M, Wang L, Huang H T 2018 Ceram. Int. 44 21835 Google Scholar
[20]	李宗宝, 王霞, 樊帅伟 2014 物理学报 63 157102 Google Scholar Li Z B, Wang X, Fan S W 2014 Acta Phys. Sin. 63 157102 Google Scholar
[21]	You H L, Ma X X, Wu Z, Fei L F, Chen X Q, Yang J, Liu Y S, Jia Y M, Li H M, Wang F F, Huang H T 2018 Nano Energy 52 351 Google Scholar
[22]	Wu Y L, Ma Y L, Zheng H Y, Ramakrishna S 2021 Materials & Design 211 110164 Google Scholar
[23]	Hooper T E, Roscow J I, Mathieson A, Khanbareh H, Goetzee-Barral A J, Bell A J 2021 J. Eur. Ceram. Soc. 41 6115 Google Scholar
[24]	Hong K S, Xu H F, Konishi H, Li X C 2010 J. Phys. Chem. Lett. 1 997 Google Scholar
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