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空气激光: 面向大气遥感的高分辨光谱技术

张海粟 乔玲玲 程亚

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空气激光: 面向大气遥感的高分辨光谱技术

张海粟, 乔玲玲, 程亚

Air-lasing high-resolution spectroscopy for atmospheric remote sensing

Zhang Hai-Su, Qiao Ling-Ling, Cheng Ya
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  • 空气激光是以空气为增益介质产生的无谐振腔自由空间相干辐射, 具有高准直度、高相干性以及高强度等显著优势. 基于高功率超短激光脉冲非线性传输成丝过程, 可以远程诱导产生空气激光从而为大气遥感探测提供理想光源. 得益于空气激光产生时伴随的原子分子相干激发过程, 空气激光远程探测技术具有高光谱分辨率和高探测灵敏度, 为痕量分子探测、温室气体监测以及工业污染物检测等远程遥感应用提供了有力工具. 本文简单介绍空气激光的物理机制, 着重回顾空气激光远程探测的各种应用并对未来研究做出展望.
    Air-lasing is a cavityless coherent radiation generated in free space from air constituents as gain medium, featuring high collimation, high coherence, and high intensity. Benefited from the long-range filamentation of high-power ultrashort laser pulses propagating in air, the air-lasing can be induced remotely, providing an ideal light source for atmospheric remote sensing and chemical species-resolved detection. Owing to the coherent atomic/molecular excitation process accompanied with the generation of air laser, remote sensing based on air-lasing has high spectral resolution and high detection sensitivity, which recently proved to be a powerful tool for important applications such as in trace molecule detection, greenhouse gas monitoring and industrial pollutant detection. In this short review, the physical mechanism of air lasing is briefly introduced, and various applications of air laser remote sensing are reviewed emphatically, and the future research is prospected.
      通信作者: 程亚, ya.cheng@siom.ac.cn
    • 基金项目: 国家重点研发计划(批准号: 2019YFA0705000)和国家自然科学基金(批准号: 12192251, 12134001) 资助的课题
      Corresponding author: Cheng Ya, ya.cheng@siom.ac.cn
    • Funds: Project supported by the National Key R&D Program of China (Grant No. 2019YFA0705000) and the National Natural Science Foundation of China (Grant Nos. 12192251, 12134001).
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    Zhao X D, Nolte S, Ackermann R 2020 Opt. Lett. 45 3661Google Scholar

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    Zhang Z H, Zhang F B, Xu B, Xie H Q, Fu B T, Lu X, Zhang N, Yu S P, Yao J P, Cheng Y, Xu Z Z 2022 Ultrafast Sci. 2 9761458Google Scholar

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    Laurain A, Scheller M, Polynkin P 2014 Phys. Rev. Lett. 113 253901Google Scholar

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    Dogariu A, Miles R B 2016 Opt. Express 24 A544Google Scholar

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    Kartashov D, Ališauskas S, Andriukaitis G, Pugzlys A, Shneider M, Zheltikov A, Chin S L, Baltuska A 2012 Phys. Rev. A 86 033831Google Scholar

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    Mitryukovskiy S, Liu Y, Ding P J, Houard A, Mysyrowicz A 2014 Opt. Express 22 12750Google Scholar

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    Mitryukovskiy S, Liu Y, Ding P J, Houard A, Couairon A, Mysyrowicz A 2015 Phys. Rev. Lett. 114 063003Google Scholar

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    Yao J P, Chu W, Liu Z X, Chen J M, Xu B, Cheng Y 2018 Appl. Phys. B 124 73

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  • 图 1  $ {\rm{N}}_{2}^{+} $激光的时空特性[17] (a)中心波长为428 nm的$ {\rm{N}}_{2}^{+} $激光光谱, 插图为$ {\rm{N}}_{2}^{+} $激光的远场光斑形状; (b)$ {\rm{N}}_{2}^{+} $激光的时域波形, 红色箭头标明800 nm驱动激光脉冲入射时刻

    Fig. 1.  Spectral-temporal profiles of $ {\rm{N}}_{2}^{+} $ lasing[17]: (a) $ {\rm{N}}_{2}^{+} $ laser spectrum with the central wavelength of 428 nm, the inset is the far-field profile of $ {\rm{N}}_{2}^{+} $ laser; (b) $ {\rm{N}}_{2}^{+} $ laser temporal profile with the red arrow denoting the timing of the 800 nm driving pulse.

    图 2  $ {\rm{N}}_{2}^{+} $激光和$ {\rm{N}}_{2} $拉曼散射光谱[16] (a) $ {\rm{N}}_{2}^{+} $激光光谱; (b) $ {\rm{N}}_{2} $拉曼散射光谱

    Fig. 2.  Spectra of $ {\rm{N}}_{2}^{+} $ laser and $ {\rm{N}}_{2} $ Raman scattering[16]: (a) $ {\rm{N}}_{2}^{+} $ laser spectrum; (b) $ {\rm{N}}_{2} $ Raman scattering spectrum.

    图 3  利用$ {\rm{N}}_{2}^{+} $激光产生高阶拉曼散射[17] (a)实验装置示意图; (b) $ {\rm{N}}_{2}^{+} $激光在不同气压的CO2气体中产生的高阶转动拉曼散射光谱, 插图为1 atm (1 atm = 1.013×105 Pa)下的拉曼散射信号空间光斑形状

    Fig. 3.  High-order cascaded Raman scattering induced by $ {\rm{N}}_{2}^{+} $ laser[17]: (a) Experimental schematic; (b) measured high-order rotational Raman scattering spectra at various gas pressures of CO2, inset shows the spatial profile of Raman signals at 1 atm (1 atm = 1.013×105 Pa).

    图 4  $ {\rm{N}}_{2}^{+} $激光在CO2中产生拉曼散射[18] (a) CO2中对应的拉曼跃迁能级图; (b) N2, $ {\rm{N}}_{2}^{+} $, O2和 CO2的拉曼散射光谱

    Fig. 4.  Raman scattering induced by $ {\rm{N}}_{2}^{+} $ laser: (a) Relevant Raman transition levels in CO2; (b) Raman scattering spectra of N2, $ {\rm{N}}_{2}^{+} $, O2 and CO2.

    图 5  空气激光辅助相干拉曼散射[19] (a) 空气激光和相干拉曼散射产生机制示意图; (b), (c) 相干拉曼信号强度与气体浓度的定量关系, 插图为最小浓度下测得CO2和SF6的拉曼信号

    Fig. 5.  Air-lasing based coherent Raman scattering[19]: (a) Generation scheme of air-lasing and coherent Raman scattering; (b), (c) intensity of Raman signal as a function of gas pressure, inset shows the measured Raman signals of CO2 and SF6 at the minimum pressures.

  • [1]

    姚金平, 程亚 2020 中国激光 47 0500005Google Scholar

    Yao J, Cheng Y 2020 Chin. J. Laser 47 0500005Google Scholar

    [2]

    Chin S L, Xu H L, Cheng Y, Xu Z Z, Yamanouchi K 2013 Chin. Opt. Lett. 11 013201Google Scholar

    [3]

    Polynkin P, Cheng Y 2018 Air Lasing (Cham: Springer International Publishing) p139

    [4]

    Luo Q, Liu W W, Chin S L 2003 Appl. Phys. B 76 337Google Scholar

    [5]

    Dogariu A, Michael J B, Scully M O, Miles R B 2011 Science 331 442Google Scholar

    [6]

    Yao J P, Zeng B, Xu H L, Li G H, Chu W, Ni J L, Zhang H S, Chin S L, Cheng Y, Xu Z Z 2011 Phys. Rev. A 84 051802Google Scholar

    [7]

    Hemmer P R, Miles R B, Polynkin P, Siebert T, Sokolov A V, Sprangle P, Scully M O 2011 P. Natl. Acad. Sci. USA 108 3130Google Scholar

    [8]

    Traverso A J, Sanchez-Gonzalez R, Yuan L Q, Wang K, Voronine D V, Zheltikov A M, Rostovtsev Y, Sautenkov V A, Sokolov A V, North S W, Scully M O 2012 P. Natl. Acad. Sci. USA 109 15185Google Scholar

    [9]

    Malevich P N, Kartashov D, Pu Z, Alisauskas S, Pugzlys A, Baltuska A, Giniunas L, Danielius R, Zheltikov A, Marangoni M, Cerullo G 2012 Opt. Express 20 18784Google Scholar

    [10]

    Malevich P N, Maurer R, Kartashov D, Alisauskas S, Lanin A A, Zheltikov A M, Marangoni M, Cerullo G, Baltuska A, Pugzlys A 2015 Opt. Lett. 40 2469Google Scholar

    [11]

    Yuan L Q, Liu Y, Yao J P, Cheng Y 2019 Adv. Quantum Tech. 2 1900080Google Scholar

    [12]

    Braun A, Korn G, Liu X, Du D, Squier J, Mourou G 1995 Opt. Lett. 20 73Google Scholar

    [13]

    Couairon A, Mysyrowicz A 2007 Phys. Rep. 441 47Google Scholar

    [14]

    Fu Y, Cao J C, Yamanouchi K, Xu H L 2022 Ultrafast Sci. 4 9867028Google Scholar

    [15]

    Zhang F B, Xie H Q, Yuan L, Zhang Z H, Fu B T, Yu S P, Li G H, Zhang N, Lu X, Yao J P, Cheng Y, Xu Z Z 2022 Opt. Lett. 47 481Google Scholar

    [16]

    Ni J L, Chu W, Zhang H S, Zeng B, Yao J P, Qiao L L, Li G H, Jing C R, Xie H Q, Xu H L, Cheng Y, Xu Z Z 2014 Opt. Lett. 39 2250Google Scholar

    [17]

    Liu Z X, Yao J P, Zhang H S, Xu B, Chen J M, Zhang F B, Zhang Z H, Wan Y X, Chu W, Wang Z H, Cheng Y 2020 Phys. Rev. A 101 043404Google Scholar

    [18]

    Zhao X D, Nolte S, Ackermann R 2020 Opt. Lett. 45 3661Google Scholar

    [19]

    Zhang Z H, Zhang F B, Xu B, Xie H Q, Fu B T, Lu X, Zhang N, Yu S P, Yao J P, Cheng Y, Xu Z Z 2022 Ultrafast Sci. 2 9761458Google Scholar

    [20]

    Laurain A, Scheller M, Polynkin P 2014 Phys. Rev. Lett. 113 253901Google Scholar

    [21]

    Dogariu A, Miles R B 2016 Opt. Express 24 A544Google Scholar

    [22]

    Kartashov D, Ališauskas S, Andriukaitis G, Pugzlys A, Shneider M, Zheltikov A, Chin S L, Baltuska A 2012 Phys. Rev. A 86 033831Google Scholar

    [23]

    Mitryukovskiy S, Liu Y, Ding P J, Houard A, Mysyrowicz A 2014 Opt. Express 22 12750Google Scholar

    [24]

    Mitryukovskiy S, Liu Y, Ding P J, Houard A, Couairon A, Mysyrowicz A 2015 Phys. Rev. Lett. 114 063003Google Scholar

    [25]

    Yao J P, Li G H, Jing C R, Zeng B, Chu W, Ni J L, Zhang H S, Xie H Q, Zhang C J, Li H L, Xu H L, Chin S L, Cheng Y, Xu Z Z 2013 New J. Phys. 15 023046Google Scholar

    [26]

    Liu Y, Ding P J, Lambert G, Houard A, Tikhonchuk V, Mysyrowicz A 2015 Phys. Rev. Lett. 115 133203Google Scholar

    [27]

    Xu H L, Lötstedt E, Iwasaki A, Yamanouchi K 2015 Nat. Commun. 6 8347Google Scholar

    [28]

    Yao J P, Jiang S C, Chu W, Zeng B, Wu C Y, Lu R F, Li Z T, Xie H Q, Li G H, Yu C, Wang Z S, Jiang H B, Gong Q H, Cheng Y 2016 Phys. Rev. Lett. 116 143007Google Scholar

    [29]

    Liu Y, Ding P J, Ibrakovic N, Bengtsson S, Chen S H, Danylo R, Simpson E R, Larsen E W, Zhang X, Fan Z Q 2017 Phys. Rev. Lett. 119 203205Google Scholar

    [30]

    Liu Z X, Yao J P, Chen J M, Xu B, Chu W, Cheng Y 2018 Phys. Rev. Lett. 120 083205Google Scholar

    [31]

    Britton M, Laferrière P, Ko D H, Li Z Y, Kong F Q, Brown G, Naumov A, Zhang C M, Arissian L, Corkum P B 2018 Phys. Rev. Lett. 120 133208Google Scholar

    [32]

    Yao J P, Chu W, Liu Z X, Chen J M, Xu B, Cheng Y 2018 Appl. Phys. B 124 73

    [33]

    Ando T, Lötstedt E, Iwasaki A, Li H L, Fu Y, Wang S Q, Xu H L, Yamanouchi K 2019 Phys. Rev. Lett. 123 203201Google Scholar

    [34]

    Li H L, Hou M Y, Zang H W, Fu Y, Lotstedt E, Ando T, Iwasaki A, Yamanouchi K, Xu H L 2019 Phys. Rev. Lett. 122 013202Google Scholar

    [35]

    Li H X, Lötstedt E, Li H L, Zhou Y, Dong N N, Deng L H, Lu P F, Ando T, Iwasaki A, Fu Y 2020 Phys. Rev. Lett. 125 053201Google Scholar

    [36]

    Zhang H S, Jing C R, Yao J P, Li G H, Zeng B, Chu W, Ni J L, Xie H Q, Xu H L, Chin S L, Yamanouchi K, Cheng Y, Xu Z Z 2013 Phys. Rev. X 3 041009Google Scholar

    [37]

    Jing C R, Zhang H S, Chu W, Xie H Q, Ni J L, Zeng B, Li G H, Yao J P, Xu H L, Cheng Y, Xu Z Z 2014 Opt. Express 22 3151Google Scholar

    [38]

    Jing C R, Yao J P, Li Z T, Ni J L, Zeng B, Chu W, Li G H, Xie H Q, Cheng Y 2015 J. Phys. B 48 094001Google Scholar

    [39]

    Li G H, Jing C R, Zeng B, Xie H Q, Yao J P, Chu W, Ni J L, Zhang H S, Xu H L, Cheng Y 2014 Phys. Rev. A 89 033833Google Scholar

    [40]

    Chen J M, Yao J P, Zhang H S, Liu Z X, Xu B, Chu W, Qiao L L, Wang Z H, Fatome J, Faucher O, Wu CY, Cheng Y 2019 Phys. Rev. A 100 031402Google Scholar

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    Xie H Q, Zeng B, Li G H, Chu W, Zhang H S, Jing C R, Yao J P, Ni J L, Wang Z H, Li Z T 2014 Phys. Rev. A 90 042504Google Scholar

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    Zeng B, Chu W, Li G H, Yao J P, Zhang H S, Ni J L, Jing C R, Xie H Q, Cheng Y 2014 Phys. Rev. A 89 042508Google Scholar

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出版历程
  • 收稿日期:  2022-10-05
  • 修回日期:  2022-11-14
  • 上网日期:  2022-11-28
  • 刊出日期:  2022-12-05

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