搜索

x

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

基于磁集聚效应的系综NV色心磁检测增强

李中豪 王天宇 郭琦 郭浩 温焕飞 唐军 刘俊

引用本文:
Citation:

基于磁集聚效应的系综NV色心磁检测增强

李中豪, 王天宇, 郭琦, 郭浩, 温焕飞, 唐军, 刘俊

Enhancement of magnetic detection by ensemble NV color center based on magnetic flux concentration effect

Li Zhong-Hao, Wang Tian-Yu, Guo Qi, Guo Hao, Wen Huan-Fei, Tang Jun, Liu Jun
PDF
HTML
导出引用
  • 高灵敏色心量子自旋磁检测是弱磁、极弱磁检测及成像应用的关键. 本文通过搭建结合磁力线集聚结构(MFC)的系综金刚石氮空位(NV)色心的宽视场磁分布成像系统, 对系综金刚石NV色心磁检测增强进行了系统研究. 首先基于磁力线集聚效应仿真设计并制造了成对的T型薄片状MFC结构, 利用连续波光探测磁共振(ODMR)宽视场磁成像技术对MFC的磁增强效果进行验证. 实验测试的MFC间距的最小值为1.0 mm,此时磁增强倍数约为10.35, 通过进一步对比不同磁场强度以及不同间距条件下的MFC磁增强效果, 验证了MFC磁增强效果的有效性, 系统磁检测灵敏度由1.10 nT/Hz1/2提升至0.30 nT/Hz1/2. 通过进一步对比仿真与测量获得的磁增强倍数与间隙宽度的关系, 可对实验系统的磁增强及灵敏度进行有效估计. 在MFC间距为0.5 mm时, 对应的磁增强倍数可提升至约18.21, 磁灵敏度则可达0.25 nT/Hz1/2. 以上结果表明基于磁集聚效应可以实现系综金刚石氮空位色心磁检测灵敏度的有效提升, 为精密量子测量技术在弱磁、极弱磁检测应用方面提供了参考.
    The high-sensitivity magnetic sensor is the key to the weak magnetic and extremely weak magnetic detection imaging. In this paper, based on ensemble nitrogen-vacancy (NV) color center in diamond, a wide-field magnetic field distribution imaging system combined with the magnetic flux concentrator (MFC) is built for enhancing the magnetic detection. The paired T-shape chip MFC structures are designed and prepared based on the simulation of magnetic flux concentration effect, and the enhancement of magnetic field of MFC is verified by continuous wave optical detection magnetic resonance (CW-ODMR) imaging technology. When the gap width between the MFCs is 1.0 mm, the magnetic enhancement factor is about 10.35. To verify the effectiveness of the magnetic enhancement effect of the MFC, The magnetic enhancement effects are also measured under different magnetic field strengths and different gap widths. The magnetic sensitivity of the system increases from 1.10 nT/Hz1/2 to 0.30 nT/Hz1/2. By comparing the simulations with the measurements, the relationship between the measured magnetic enhancement multiple and the gap width can be obtained, and the better magnetic enhancement capability and sensitivity of the experimental system are also estimated. When the MFC’s gap width is 0.5 mm, the corresponding magnetic enhancement factor is increased to 18.21, and the corresponding magnetic sensitivity is 0.25 nT/Hz1/2. These results show that the magnetic detection sensitivity of the ensemble NV in diamond can be effectively improved based on magnetic flux concentration effect, which provides a reference for the applications of precision quantum measurement technology in weak magnetic and extremely weak magnetic detection.
      通信作者: 唐军, tangjun@nuc.edu.cn ; 刘俊, liuj@nuc.edu.cn
    • 基金项目: 国家重大科研仪器设备研制专项(批准号: 51727808, 61727804)、国家自然科学基金(批准号: 51635011, 51922009)、山西省应用基础研究计划(批准号: 201901D111011 (ZD), 201901D211254, 201801D221202, 201801D221213)、山西省重点研发项目(批准号: 201803D121067)、山西省高等学校科技创新项目(批准号: 2019L0558)、山西省重点实验室 (批准号: 201905D121001)和山西省“1331工程”重点学科建设计划经费资助的课题.
      Corresponding author: Tang Jun, tangjun@nuc.edu.cn ; Liu Jun, liuj@nuc.edu.cn
    • Funds: Project supported by the Special Fund for Research on National Major Research Instruments and Facilities of the National Natural Science Foundation of China (Grant Nos. 51727808, 61727804), the National Natural Science Foundation of China (Grant Nos. 51635011, 51922009), the Research Foundation for Basic Research of Shanxi Province, China (Grant Nos. 201901D111011(ZD), 201901D211254, 201801D221202, 201801D221213), the Key Research and Development Foundation of Shanxi Province, China (Grant No. 201803D121067), the Science and Technology Innovation Project of the Higher Education of Shanxi Province, China (Grant No. 2019L0558), the Key Laboratory of Shanxi Province, China (Grant No. 201905D121001), and the Fund for Shanxi “1331 Project” Key Subjects Construction, China
    [1]

    Shenton M E, Hamoda H M, Schneiderman J S, Bouix S, Pasternak O, Rathi Y, Vu M A, Purohit M P, Helmer K, Koerte I, Lin A P, Westin C F, Kikinis R, Kubicki M, Stern R A, Zafonte R 2012 Brain Imaging Behav. 6 137Google Scholar

    [2]

    Lenz J, Edelstein A S 2006 IEEE Sens. J. 6 631Google Scholar

    [3]

    Xia H, Baranga A B A, Hoffman D, Romalis M V 2006 Appl. Phys. Lett. 89 211104Google Scholar

    [4]

    Anahory Y, Reiner J, Embon L, Halbertal D, Yakovenko A, Myasoedov Y, Rappaport M L, Huber M E, Zeldov E 2014 Nano Lett. 14 6481Google Scholar

    [5]

    Pannetier M, Fermon C, Le Goff G, Simola J, Kerr E 2004 Science 304 1648Google Scholar

    [6]

    Yabukami S, Kato K, Ohtomo Y, Ozawa T, Arai K I 2009 J. Magn. Magn. Mater. 321 675Google Scholar

    [7]

    Wang Y, Gao J, Li M, Hasanyan D, Shen Y, Li J, Viehland D, Luo H 2012 Appl. Phys. Lett. 101 022903Google Scholar

    [8]

    Wang P F, Chen S Y, Guo M S, Peng S J, Wang M Q, Chen M, Ma W C, Zhang R, Su J H, Rong X, Shi F Z, Xu T, Du J F 2019 Sci. Adv. 5 eaau8038 6Google Scholar

    [9]

    Maze J R, Stanwix P L, Hodges J S, Hong S, Taylor J M, Cappellaro P, Jiang L, Dutt M V G, Togan E, Zibrov A S, Yacoby A, Walsworth R L, Lukin M D 2008 Nature 455 644Google Scholar

    [10]

    Barry J F, Schloss J M, Bauch E, Turner M J, Hart C A, Pham L M, Walsworth R L 2020 Rev. Mod. Phys. 92 015004Google Scholar

    [11]

    Davis H C, Ramesh P, Bhatnagar A, Lee-Gosselin A, Barry J F, Glenn D R, Walsworth R L, Shapiro M G 2018 Nat. Commun. 9 1319Google Scholar

    [12]

    Glenn D R, Fu R R, Kehayias P, Le Sage D, Lima E A, Weiss B P, Walsworth R L 2017 Geochem. Geophys. Geosyst. 18 3254Google Scholar

    [13]

    Jensen K, Leefer N, Jarmola A, Dumeige Y, Acosta V M, Kehayias P, Patton B, Budker D 2014 Phys. Rev. Lett. 112 160802Google Scholar

    [14]

    Fescenko I, Jarmola A, Savukov I, Kehayias P, Smits J, Damron J, Ristoff N, Mosavian N, Acosta V M 2020 Phys. Rev. Res. 2 023394Google Scholar

    [15]

    Griffith W C, Jimenez-Martinez R, Shah V, Knappe S, Kitching J 2009 Appl. Phys. Lett. 94 023502Google Scholar

    [16]

    Fan H, Li S, Nabaei V, Feng Q, Heidari H 2020 IEEE Sens. J. 20 9919Google Scholar

    [17]

    Szewczyk R, Ostaszewska-Lizewska A, Raback P 2020 Acta Phys. Pol. A 137 700Google Scholar

    [18]

    Hu J F, Ji M H, Qiu W C, Pan L, Li P S, Peng J P, Hu Y G, Liu H Y, Pan M C 2019 Sensors 19 4475Google Scholar

    [19]

    Feng Y L, Chen J Y, Wu K, Wang J P 2020 J. Magn. Magn. Mater. 511 166728Google Scholar

    [20]

    Doherty M W, Dolde F, Fedder H, Jelezko F, Wrachtrup J, Manson N B, Hollenberg L C L 2012 Phys. Rev. B 85 205203Google Scholar

    [21]

    Zhao B B, Guo H, Zhao R, Du F F, Li Z H, Wang L, Wu D J, Chen Y L, Tang J, Liu J 2019 IEEE Magn. Lett. 10 8101104Google Scholar

    [22]

    Marinho Z, Cardoso S, Chaves R, Ferreira R, Melo L V, Freitas P P 2011 J. Appl. Phys. 109 07e521Google Scholar

    [23]

    Zhang X M, Bi Y, Chen G B, Liu J, Li J, Feng K Q, Lv C, Wang W J 2018 AIP Adv. 8 125222Google Scholar

    [24]

    Sun X, Jiang L J, Pong P W T 2013 Microelectron. Eng. 111 77Google Scholar

    [25]

    Botsch L, Raatz N, Pezzagna S, Staacke R, John R, Abel B, Esquinazi P D, Meijer J, Diziain S 2020 Rev. Sci. Instrum. 91 125003Google Scholar

    [26]

    Schloss J M, Barry J F, Turner M J, Walsworth R L 2018 Phys. Rev. Appl. 10 034044Google Scholar

    [27]

    Barry J F, Turner M J, Schloss J M, Glenn D R, Song Y, Lukin M D, Park H, Walsworth R L 2016 Proc. Natl. Acad. Sci. U.S.A. 113 14133Google Scholar

    [28]

    Jensen K, Acosta V M, Jarmola A, Budker D 2013 Phys. Rev. B 87 014115Google Scholar

    [29]

    Leroy P, Coillot C, Roux A F, Chanteur G M 2006 IEEE Sens. J. 6 707Google Scholar

  • 图 1  (a)金刚石NV色心能级跃迁示意图; (b)沿(100)面生长的金刚石晶胞中一种NV轴朝向与磁场方向夹角示意图; (c) T型薄片状MFC及调节装置示意图; (d) MFC间距为0.5 mm的两永磁体间磁场仿真流线图; (e)无MFC的两永磁体间磁场仿真流线图

    Fig. 1.  (a) Related energy levels of NV color center in diamond; (b) schematic diagram of the angle between the direction of the magnetic field and the direction of the NV axis in the diamond cell grown along the (100) plane; (c) schematic diagram of the T-shaped flake MFC and adjusting system; (d) simulation of magnetic field streamline diagram with MFC gap width of 0.5 mm between two permanent magnets; (e) simulation of magnetic field streamline diagram without MFC between two permanent magnets

    图 2  (a) 实验装置示意图; (b) 用于仿真的几何结构俯视图, 红框为MFC间距0.5 mm时间隙部分放大示意图, 黑框为视场内的仿真磁场分布图

    Fig. 2.  (a) Schematic diagram of experimental setup; (b) top view of the geometric structure used in simulation, the red frame is the enlarged schematic diagram of the gap part when the MFC gap width is 0.5 mm, and the black frame is the simulated magnetic field distribution in the field of view.

    图 3  (a) 测量得到的1.0 mm间距MFC的测量位置磁场分布图(左)与同样位置处无MFC磁场分布图(右), 单位Gs; (b)仿真得到的图(a)的两个对应图; (c)三种状态的ODMR曲线, 只有背景磁场(黑线)、有待测磁场无MFC(橙线)、有间距1.0 mm 的MFC (蓝线); (d) MFC间距1.0 mm时改变待测磁场强度得到的增强磁场与基准磁场关系

    Fig. 3.  (a) Simulated magnetic field distribution diagram of the MFCs with a 1.0 mm gap (left) and without MFCs at the same position (right); (b) corresponding photos of panel (a) obtained by measurement; (c) ODMR curves under three conditions: only background magnetic field (black line), magnetic field without MFC (orange line), magnetic field with MFC of 1.0 mm gap (blue line); (d) relationship between the enhanced magnetic field and the reference magnetic field obtained by changing the intensity of the magnetic field to be measured when the MFCs gap is 1.0 mm.

    图 4  (a) MFC不同间距下ODMR曲线; (b)仿真(红色圆圈)与测量(黑色方点)得到的不同间距MFC的磁场增强倍数曲线, 蓝线为拟合曲线.

    Fig. 4.  (a) ODMR curves of MFC with different gap widths; (b) magnetic field enhancement curve of MFC with different gap widths obtained by simulation (red circles) and measurement (black dots). The blue line is the fitting curve.

    图 5  黑色方点为测量得到的不同间距下的磁灵敏度, 红线为无MFC状态下的磁灵敏度, 蓝线为拟合曲线, 蓝色星形为估计得到的间距为0.5 mm的磁灵敏度

    Fig. 5.  The black square points are the measured magnetic sensitivity at different intervals, the red line is the magnetic sensitivity without MFC, the blue line is the fitting curve, and the blue star is the estimated magnetic sensitivity with a pitch of 0.5 mm.

  • [1]

    Shenton M E, Hamoda H M, Schneiderman J S, Bouix S, Pasternak O, Rathi Y, Vu M A, Purohit M P, Helmer K, Koerte I, Lin A P, Westin C F, Kikinis R, Kubicki M, Stern R A, Zafonte R 2012 Brain Imaging Behav. 6 137Google Scholar

    [2]

    Lenz J, Edelstein A S 2006 IEEE Sens. J. 6 631Google Scholar

    [3]

    Xia H, Baranga A B A, Hoffman D, Romalis M V 2006 Appl. Phys. Lett. 89 211104Google Scholar

    [4]

    Anahory Y, Reiner J, Embon L, Halbertal D, Yakovenko A, Myasoedov Y, Rappaport M L, Huber M E, Zeldov E 2014 Nano Lett. 14 6481Google Scholar

    [5]

    Pannetier M, Fermon C, Le Goff G, Simola J, Kerr E 2004 Science 304 1648Google Scholar

    [6]

    Yabukami S, Kato K, Ohtomo Y, Ozawa T, Arai K I 2009 J. Magn. Magn. Mater. 321 675Google Scholar

    [7]

    Wang Y, Gao J, Li M, Hasanyan D, Shen Y, Li J, Viehland D, Luo H 2012 Appl. Phys. Lett. 101 022903Google Scholar

    [8]

    Wang P F, Chen S Y, Guo M S, Peng S J, Wang M Q, Chen M, Ma W C, Zhang R, Su J H, Rong X, Shi F Z, Xu T, Du J F 2019 Sci. Adv. 5 eaau8038 6Google Scholar

    [9]

    Maze J R, Stanwix P L, Hodges J S, Hong S, Taylor J M, Cappellaro P, Jiang L, Dutt M V G, Togan E, Zibrov A S, Yacoby A, Walsworth R L, Lukin M D 2008 Nature 455 644Google Scholar

    [10]

    Barry J F, Schloss J M, Bauch E, Turner M J, Hart C A, Pham L M, Walsworth R L 2020 Rev. Mod. Phys. 92 015004Google Scholar

    [11]

    Davis H C, Ramesh P, Bhatnagar A, Lee-Gosselin A, Barry J F, Glenn D R, Walsworth R L, Shapiro M G 2018 Nat. Commun. 9 1319Google Scholar

    [12]

    Glenn D R, Fu R R, Kehayias P, Le Sage D, Lima E A, Weiss B P, Walsworth R L 2017 Geochem. Geophys. Geosyst. 18 3254Google Scholar

    [13]

    Jensen K, Leefer N, Jarmola A, Dumeige Y, Acosta V M, Kehayias P, Patton B, Budker D 2014 Phys. Rev. Lett. 112 160802Google Scholar

    [14]

    Fescenko I, Jarmola A, Savukov I, Kehayias P, Smits J, Damron J, Ristoff N, Mosavian N, Acosta V M 2020 Phys. Rev. Res. 2 023394Google Scholar

    [15]

    Griffith W C, Jimenez-Martinez R, Shah V, Knappe S, Kitching J 2009 Appl. Phys. Lett. 94 023502Google Scholar

    [16]

    Fan H, Li S, Nabaei V, Feng Q, Heidari H 2020 IEEE Sens. J. 20 9919Google Scholar

    [17]

    Szewczyk R, Ostaszewska-Lizewska A, Raback P 2020 Acta Phys. Pol. A 137 700Google Scholar

    [18]

    Hu J F, Ji M H, Qiu W C, Pan L, Li P S, Peng J P, Hu Y G, Liu H Y, Pan M C 2019 Sensors 19 4475Google Scholar

    [19]

    Feng Y L, Chen J Y, Wu K, Wang J P 2020 J. Magn. Magn. Mater. 511 166728Google Scholar

    [20]

    Doherty M W, Dolde F, Fedder H, Jelezko F, Wrachtrup J, Manson N B, Hollenberg L C L 2012 Phys. Rev. B 85 205203Google Scholar

    [21]

    Zhao B B, Guo H, Zhao R, Du F F, Li Z H, Wang L, Wu D J, Chen Y L, Tang J, Liu J 2019 IEEE Magn. Lett. 10 8101104Google Scholar

    [22]

    Marinho Z, Cardoso S, Chaves R, Ferreira R, Melo L V, Freitas P P 2011 J. Appl. Phys. 109 07e521Google Scholar

    [23]

    Zhang X M, Bi Y, Chen G B, Liu J, Li J, Feng K Q, Lv C, Wang W J 2018 AIP Adv. 8 125222Google Scholar

    [24]

    Sun X, Jiang L J, Pong P W T 2013 Microelectron. Eng. 111 77Google Scholar

    [25]

    Botsch L, Raatz N, Pezzagna S, Staacke R, John R, Abel B, Esquinazi P D, Meijer J, Diziain S 2020 Rev. Sci. Instrum. 91 125003Google Scholar

    [26]

    Schloss J M, Barry J F, Turner M J, Walsworth R L 2018 Phys. Rev. Appl. 10 034044Google Scholar

    [27]

    Barry J F, Turner M J, Schloss J M, Glenn D R, Song Y, Lukin M D, Park H, Walsworth R L 2016 Proc. Natl. Acad. Sci. U.S.A. 113 14133Google Scholar

    [28]

    Jensen K, Acosta V M, Jarmola A, Budker D 2013 Phys. Rev. B 87 014115Google Scholar

    [29]

    Leroy P, Coillot C, Roux A F, Chanteur G M 2006 IEEE Sens. J. 6 707Google Scholar

  • [1] 申圆圆, 王博, 柯冬倩, 郑斗斗, 李中豪, 温焕飞, 郭浩, 李鑫, 唐军, 马宗敏, 李艳君, 伊戈尔∙费拉基米罗维奇∙雅明斯基, 刘俊. 高频率分辨的金刚石氮-空位色心宽频谱成像技术. 物理学报, 2024, 73(6): 067601. doi: 10.7498/aps.73.20231833
    [2] 何健, 贾燕伟, 屠菊萍, 夏天, 朱肖华, 黄珂, 安康, 刘金龙, 陈良贤, 魏俊俊, 李成明. 碳离子注入金刚石制备氮空位色心的机理. 物理学报, 2022, 71(18): 188102. doi: 10.7498/aps.71.20220794
    [3] 吴建冬, 程智, 叶翔宇, 李兆凯, 王鹏飞, 田长麟, 陈宏伟. 金刚石氮-空位色心单电子自旋的电场驱动相干控制研究. 物理学报, 2022, 0(0): . doi: 10.7498/aps.71.20220410
    [4] 吴建冬, 程智, 叶翔宇, 李兆凯, 王鹏飞, 田长麟, 陈宏伟. 金刚石氮-空位色心单电子自旋的电场驱动相干控制. 物理学报, 2022, 71(11): 117601. doi: 10.7498/aps.70.20220410
    [5] 林豪彬, 张少春, 董杨, 郑瑜, 陈向东, 孙方稳. 基于金刚石氮-空位色心的温度传感. 物理学报, 2022, 71(6): 060302. doi: 10.7498/aps.71.20211822
    [6] 沈翔, 赵立业, 黄璞, 孔熙, 季鲁敏. 金刚石氮-空位色心的原子自旋声子耦合机理. 物理学报, 2021, 70(6): 068501. doi: 10.7498/aps.70.20201848
    [7] 冯园耀, 李中豪, 张扬, 崔凌霄, 郭琦, 郭浩, 温焕飞, 刘文耀, 唐军, 刘俊. 固态金刚石氮空位色心光学调控优化. 物理学报, 2020, 69(14): 147601. doi: 10.7498/aps.69.20200072
    [8] 张文杰, 刘郁松, 郭浩, 韩星程, 蔡安江, 李圣昆, 赵鹏飞, 刘俊. 双螺线圈射频共振结构增强硅空位自旋传感灵敏度方法. 物理学报, 2020, 69(23): 234206. doi: 10.7498/aps.69.20200765
    [9] 王磊, 郭浩, 陈宇雷, 伍大锦, 赵锐, 刘文耀, 李春明, 夏美晶, 赵彬彬, 朱强, 唐军, 刘俊. 基于金刚石色心自旋磁共振效应的微位移测量方法. 物理学报, 2018, 67(4): 047601. doi: 10.7498/aps.67.20171914
    [10] 廖庆洪, 叶杨, 李红珍, 周南润. 金刚石氮空位色心耦合机械振子和腔场系统中方差压缩研究. 物理学报, 2018, 67(4): 040302. doi: 10.7498/aps.67.20172170
    [11] 董杨, 杜博, 张少春, 陈向东, 孙方稳. 基于金刚石体系中氮-空位色心的固态量子传感. 物理学报, 2018, 67(16): 160301. doi: 10.7498/aps.67.20180788
    [12] 李雪琴, 赵云芳, 唐艳妮, 杨卫军. 基于金刚石氮-空位色心自旋系综与超导量子电路混合系统的量子节点纠缠. 物理学报, 2018, 67(7): 070302. doi: 10.7498/aps.67.20172634
    [13] 彭世杰, 刘颖, 马文超, 石发展, 杜江峰. 基于金刚石氮-空位色心的精密磁测量. 物理学报, 2018, 67(16): 167601. doi: 10.7498/aps.67.20181084
    [14] 李路思, 李红蕙, 周黎黎, 杨炙盛, 艾清. 利用金刚石氮-空位色心精确测量弱磁场的探索. 物理学报, 2017, 66(23): 230601. doi: 10.7498/aps.66.230601
    [15] 史生才, 李婧, 张文, 缪巍. 超高灵敏度太赫兹超导探测器. 物理学报, 2015, 64(22): 228501. doi: 10.7498/aps.64.228501
    [16] 顾源, 石荣晔, 王延辉. 分布式反馈激光抽运铯磁力仪灵敏度相关参数研究. 物理学报, 2014, 63(11): 110701. doi: 10.7498/aps.63.110701
    [17] 李楠, 黄凯凯, 陆璇辉. 提高激光抽运铯原子磁力仪灵敏度的研究. 物理学报, 2013, 62(13): 133201. doi: 10.7498/aps.62.133201
    [18] 刘东奇, 常彦春, 刘刚钦, 潘新宇. 金刚石纳米颗粒中氮空位色心的电子自旋研究. 物理学报, 2013, 62(16): 164208. doi: 10.7498/aps.62.164208
    [19] 李曙光, 周翔, 曹晓超, 盛继腾, 徐云飞, 王兆英, 林强. 全光学高灵敏度铷原子磁力仪的研究. 物理学报, 2010, 59(2): 877-882. doi: 10.7498/aps.59.877
    [20] 李鲠颖. 固态磁共振中提高四极核检测灵敏度的有效方法. 物理学报, 1994, 43(8): 1365-1370. doi: 10.7498/aps.43.1365
计量
  • 文章访问数:  6134
  • PDF下载量:  239
  • 被引次数: 0
出版历程
  • 收稿日期:  2021-01-20
  • 修回日期:  2021-03-08
  • 上网日期:  2021-07-14
  • 刊出日期:  2021-07-20

/

返回文章
返回