Magnetic field modulation of photocurrent in BiFeO<sub>3</sub> film

Huo Guan-Zhong; Su Chao; Wang Ke; Ye Qing-Ying; Zhuang Bin; Chen Shui-Yuan; Huang Zhi-Gao

doi:10.7498/aps.72.20222053

Abstract

BiFeO₃ (BFO) is a kind of room temperature multiferroic material with bulk photovoltaic effect, and it has been a research hotspot in the field of multifunctional materials in recent years. The coexistence of the coupling among magnetic, optical, electrical properties brings rich and complex physical connotations. In this work, BiFeO₃ thin film is deposited on FTO substrate by pulsed laser deposition, and the solar cell structure with BiFeO₃ film used as light absorption layer and Au film serving as electrode is constructed. X-ray diffraction and Raman spectra indicate that the BFO film grown on FTO substrate has a pure phase structure. The experimental results of physical properties indicate that the BFO film possesses good ferromagnetic and ferroelectric properties and obvious photoelectric effect. According to the hysteresis loop, the remanence (M_r) of the sample is 0.8 emu/cm³, and the coercivity (H_c) is 200 Oe at 300 K. In terms of ferroelectricity, the saturation polarization intensity of the sample can reach 0.997 μC/cm², the residual polarization intensity is 0.337 μC/cm², and the coercive electric field is 12.45 kV/cm. The above results show that the BFO film has good multiferroic properties. Under solar illumination conditions, the photocurrent density up to 208 mA/cm² is obtained when a bias voltage 1 V is applied. More importantly, magneto-photocurrent (MPC) effect is found in the BFO film. No matter whether the magnetic field starts to increase from the positive direction or the negative direction, the MPC usually changes with the magnitude of magnetization. When a 1.3 kOe magnetic field is applied, the magneto-photocurrent change rate up to 232.7% is observed under standard solar illumination condition. The results show that the photocurrent of BFO films is greatly improved by a positive magnetic field and negative magnetic field. This magneto-photocurrent effect in BFO thin film comes from the photo-magnetoresistance effect, that is, the photogenerated electrons become spin photoelectrons under the action of an external magnetic field and receive spin-dependent scattering during moving in the conductive band of the material, thus producing the photo-magnetoresistance effect. In addition, the magneto-photocurrent effect is further enhanced by weakening the domain wall scattering of the spin electrons by the magnetic field. This work provides a reference for the modulation effect of magnetic field and light field on the magnetic, optical and electrical properties in multiferroics, and presents a foundation for the research and application of devices in the field of multifunctional optoelectronic materials.

Keywords:

Authors and contacts

1.
Fujian Provincial Key Laboratory of Quantum Manipulation and New Energy Materials, Fujian Provincial Engineering Technology Research Center of Solar Energy Conversion and Energy Storage, Fuzhou 350117, China
2.
College of Physics and Energy, Fujian Normal University, Fuzhou 350117, China

Corresponding author: Chen Shui-Yuan, sychen@fjnu.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 11074031), the National Key R&D Program of China (Grant No. 2017YFE0301401), and the Natural Science Foundation of Fujian Province, China (Grant Nos. 2020J01192, 2021J01191).

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References

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Cited By

图 1 BFO薄膜在300 K温度下的(a) XRD图谱和(b)拉曼光谱

Figure 1. The XRD pattern (a) and Raman spectrum (b) of the BFO thin film at 300 K.

DownLoad: Full-Size Img PowerPoint

图 2 BFO薄膜在300 K温度下的(a)磁滞回线图和(b)电滞回线图

Figure 2. The M-H hysteresis loop (a) and the P-E hysteresis loops (b) of the BFO film at 300 K.

DownLoad: Full-Size Img PowerPoint

图 3 室温下样品J-V曲线在无磁场黑暗条件下及光照下随外磁场增强的响应情况

Figure 3. The J-V curves of the sample at room temperature under dark conditions without magnetic field and under light with the increase of external magnetic field.

DownLoad: Full-Size Img PowerPoint

图 4 在偏压分别为(a), (c) 0 V和(b), (d) 1 V时, 室温下样品的(a), (b)光电流随磁场变化曲线以及(c), (d) $ {D}_{{\rm{M}}{\rm{P}}{\rm{C}},{\rm{V}}} $值随磁场变化的响应曲线

Figure 4. Change curves of photocurrent (a), (b) and $ {D}_{{\rm{M}}{\rm{P}}{\rm{C}},{\rm{V}}} $(c), (d) with the alteration of magnetic field for the sample at room temperature with the bias of (a), (c) 0 V and (b), (d) 1 V.

DownLoad: Full-Size Img PowerPoint

图 5 (a) Fe³⁺简并轨道能量、自旋光电子与电子能带态密度示意图; (b)外磁场作用下Fe³⁺能带移动示意图

Figure 5. (a) Schematic diagram of the Fe³⁺ degenerate orbital energy, spin photoelectron and electron band density of state; (b) schematic diagram of the Fe³⁺ band movement under the external magnetic field.

DownLoad: Full-Size Img PowerPoint

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[17]	HOU CHUN-FENG, LI SHI-QUN, LI BIN, SUN XIU-DONG. INCOHERENTLY COUPLED BRIGHT-DARK SCREENING-PHOTOVOLTAIC SOLITON PAIRS IN BIASED PHOTOVOLTAIC PHOTOREFRACTIVE CRYSTALS. Acta Physica Sinica, 2001, 50(9): 1709-1712. doi: 10.7498/aps.50.1709
[18]	CHEN ZHENG-LIN, ZHANG JIE. CONFIGURATION OF MAGNETIC FIELDS INDUCED BY SUPERTHERMAL ELECTRONS. Acta Physica Sinica, 2001, 50(4): 735-740. doi: 10.7498/aps.50.735
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[20]	CHEN ZHENG-LIN, ZHANG JIE. CONFIGURATION OF MAGNETIC FIELDS INDUCED BY SUPERTHERMAL ELECTRONS. Acta Physica Sinica, 2000, 49(11): 2180-2185. doi: 10.7498/aps.49.2180

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Magnetic field modulation of photocurrent in BiFeO₃ film

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Magnetic field modulation of photocurrent in BiFeO3 film

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Magnetic field modulation of photocurrent in BiFeO₃ film