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近几年对活性粒子的研究已成为很多领域研究者关注的重要课题之一，其中关于活性手征粒子的相分离问题具有重要的理论和实际意义.本文通过朗之万动力学研究了具有不同扩散系数的活性手征粒子组成的二元混合系统中粒子的相分离.较小的相对扩散系数有利于“冷”粒子形成大的团簇而分离，较大的相对扩散系数则会减弱分离效果.由于粒子特征（自驱动速度、自转角速度）和相对扩散系数对粒子间碰撞作用的影响，系统要使”冷””热”粒子达到相分离，自驱动速度和自转角速度的增加（或减小）不能是同步的，自驱动速度的相对变化率要小于自转角速度的相对变化率.通过分析“冷”粒子有效扩散系数的变化，系统相分离现象得到了很好的解释.有效扩散系数较小意味着“冷”粒子会聚集形成较大的团簇，系统可出现相分离现象，而当有效扩散系数较大时“冷”粒子的扩散较强，不会形成大的团簇产生相分离.另外，随着粒子填充率的增加“冷”粒子最大团簇粒子数占比曲线进行先增加后减小的非单调变化，每条曲线存在一段最优粒子填充率宽度.相对扩散系数和自驱动速度的增大，会使曲线的最优填充率宽度变窄并向右偏移.In recent years, the study of active particles has become one of the important topics of concern for researchers in many fields, among which the phase separation of active chiral particles has important theoretical and practical significance. This paper investigates the phase separation of binary mixed systems composed of active chiral particles with different diffusion coefficients through Langevin dynamics. A smaller relative diffusion coefficient is conducive to the formation of large clusters and separation of "cold" particles, while a larger relative diffusion coefficient will weaken the separation effect. Due to the influence of particle characteristics (self-driven velocity, self-rotational angular velocity) and relative diffusion coefficient on the collision between particles, if one wants the "cold" and "hot" particles to reach phase separation, the increase (or decrease) of self-driven velocity and self-rotational angular velocity cannot be synchronous, and the relative rate of change of self-driven velocity is smaller than that of the self-rotational angular velocity. By analyzing the changes of the effective diffusion coefficient of "cold" particles, the phenomenon of phase separation in the system can be better explained. A smaller effective diffusion coefficient means "cold" particles will aggregate into larger clusters, and the system may exhibit phase separation. However, when the effective diffusion coefficient is larger, the diffusion of "cold" particles is stronger and the "cold" particles will not form large clusters, which means the system could not aggregate into phase separation. In addition, with the filling rate of particle increases, the proportion curve of the number of cold particles in maximum cold particle cluster undergoes a non-monotonic change, which is first increasing and then decreasing, and each curve has an optimal filling rate with different widths.With the increase of the relative diffusion coefficient and self-driven velocity, the width of the optimal filling rate of the proportion curve will become narrower and shift to the right.
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Keywords:
- Active particles /
- Chirality /
- Langevin equation /
- Diffusion coefficient
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