Intrinsic stability of organic-inorganic hybrid perovskite

Zhang Yu; Zhou Huan-Ping

doi:10.7498/aps.68.20190343

Abstract

The power conversion efficiency of organic-inorganic hybrid perovskite solar cell has exceeded 24%. The rapid increase in efficiency coupled with its cost-effective fabrication has attracted tremendous attention toward the commercialization of perovskite solar cells. The biggest challenge that hinders the commercialization of perovskite solar cells is the long-term instability of materials and the corresponding devices, which cannot compete with other commercialized solar cells, such as Si cells, in terms of lifetime. The intrinsic instability of perovskite material itself is the most critical challenge faced by researchers. In this study, we discuss the intrinsic instability of organic-inorganic hybrid perovskite materials from the aspects of both chemical instability and phase instability. Suggestions for improving the stability of perovskite solar cell are provided from the perspective of composition design and fabrication process.

Keywords:

hybrid perovskite /
intrinsic stability

Authors and contacts

College of Engineering, Peking University, Beijing 100871, China

Corresponding author: Zhou Huan-Ping, happy_zhou@pku.edu.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 51722201, 51672008).

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Cited By

图 1 MA⁺, FA⁺, Cs⁺, Rb⁺结构示意图^[18]

Figure 1. Schematic diagram of MA⁺, FA⁺, Cs⁺, Rb⁺^[18].

DownLoad: Full-Size Img PowerPoint

图 2 RbCsFA三元钙钛矿太阳能电池最大功率点输出^[18]

Figure 2. Maximum power point tracking of RbCsFA hybrid perovskite solar cells^[18].

DownLoad: Full-Size Img PowerPoint

图 3 Eu³⁺/Eu²⁺催化消除铅、碘零价缺陷机理^[36]

Figure 3. Proposed mechanism diagram of cyclically elimination of Pb⁰ and I⁰ defects and regeneration of Eu³⁺-Eu²⁺ metal ion pair^[36].

DownLoad: Full-Size Img PowerPoint

图 4 PEA₂MA₂Pb₃I₁₀晶体结构示意图^[44]

Figure 4. Crystal structure of PEA₂MA₂Pb₃I₁₀^[44].

DownLoad: Full-Size Img PowerPoint

图 5 MAPbI₃中各类型点缺陷能级位置^[49]

Figure 5. Calculated transition energy levels of point defects in MAPbI₃^[49].

DownLoad: Full-Size Img PowerPoint

图 6 X射线荧光光谱显示出不同碱金属卤化物添加剂情况下的Br离子分布^[85]

Figure 6. X-ray fluorescence mapping indicates heterogeneous distribution of Br as a function of alkali metal incorporation of the perovskite films^[85].

DownLoad: Full-Size Img PowerPoint

图 7 (a) DMA掺杂薄膜与HI酸添加薄膜对比; (b) DMA掺杂薄膜与HI酸添加薄膜XRD对比; (c) DMA掺杂薄膜与DMF和HI反应所得产物DMAI的核磁共振对比^[87]

Figure 7. Film properties and component studies: (a) Photographs, (b) XRD spectra, (c) nuclear magnetic resonance spectra of the Cs_0.7DMA_0.3PbI₃ films and DMAI polycrystalline powder synthesized from DMF and HI^[87].

DownLoad: Full-Size Img PowerPoint

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